Selective hydrogenation of maleic anhydride over Pd/Al2O3 catalysts prepared via colloid deposition

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• 作者：HONGJING YUAN (1)
  CHUNLEI ZHANG (2)
  WEITAO HUO (1)
  CHUNLI NING (2)
  YONG TANG (2)
  YI ZHANG (2)
  DEQUAN CONG (1)
  WENXIANG ZHANG (1)
  JIAHUAN LUO (3)
  SU LI (1)
  ZHENLU WANG (1)
  
• 关键词：Pd/Al2O3 catalyst ; maleic anhydride ; selective hydrogenation ; succinic anhydride
• 刊名：Journal of Chemical Sciences
• 出版年：2014
• 出版时间：January 2014
• 年：2014
• 卷：126
• 期：1
• 页码：141-145
• 全文大小：528 KB
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• 作者单位：HONGJING YUAN (1)
  CHUNLEI ZHANG (2)
  WEITAO HUO (1)
  CHUNLI NING (2)
  YONG TANG (2)
  YI ZHANG (2)
  DEQUAN CONG (1)
  WENXIANG ZHANG (1)
  JIAHUAN LUO (3)
  SU LI (1)
  ZHENLU WANG (1)
  
  1. Key Laboratory of Surface and Interface Chemistry of Jilin Province, College of Chemistry, Jilin University, Qianjin Road 2699, Changchun, 130012, PR China
  2. Shanghai Huayi (Group) Company Technology Research Institute, Longwu Road 4600, Shanghai, 200241, PR China
  3. State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, College of Chemistry, Jilin University, Qianjin Road 2699, Changchun, 130012, PR China
  
• ISSN：0973-7103

文摘

Pd/Al2O3 catalysts were prepared via colloid deposition and the performance of the catalysts was examined in the selective hydrogenation of maleic anhydride to succinic anhydride. When the reaction was carried on in a batch system with 1,4-dioxane as the solvent (353?K and 1.0?MPa), high conversion of maleic anhydride (>98%) and high selectivity (>99%) for succinic anhydride were observed after 5?h. The as-prepared Pd/Al2O3 catalyst also showed excellent performance in solvent-free system and fixed-bed systems. The maleic anhydride (MA) conversion was greater than 98%, and high selectivity (>99%) for succinic anhydride was obtained after 1600?h in a fixed bed reacter. The results showed that the activity of the Pd/Al2O3 catalysts was excellent due to its high active surface area. Graphical Abstract Pd/Al2O3 catalysts were prepared via colloid deposition and the performance of the catalysts was examined in the selective hydrogenation of maleic anhydride (MA) to succinic anhydride (SA). The MA conversion was >98%, and selectivity for SA was >99%.