Construction and Luminescence Properties of 4f and d-4f Clusters with Salen-Type Schiff Base Ligands

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• 关键词：4f and d ; 4f clusters ; Crystal structures ; Luminescence properties ; Salen ; type Schiff base ligands ; Synthesis
• 刊名：Structure & Bonding
• 出版年：2017
• 出版时间：2017
• 年：2017
• 卷：173
• 期：1
• 页码：155-187
• 全文大小：2,487 KB
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• 作者单位：Xiaoping Yang (3)
  Shiqing Wang (3)
  Chengri Wang (3)
  Shaoming Huang (3)
  Richard A. Jones (4)
  
  3. College of Chemistry and Materials Engineering, Wenzhou University, Wenzhou, 325035, China
  4. Department of Chemistry and Biochemistry, The University of Texas at Austin, 1 University Station A5300, Austin, TX, 78712, USA
  
• 丛书名：Recent Development in Clusters of Rare Earths and Actinides: Chemistry and Materials
• ISBN：978-3-662-53303-1
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Inorganic Chemistry
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1616-8550
• 卷排序：173

文摘

The synthesis, crystal structures, and photophysical properties of twenty-three 4f and d-4f clusters based on eight salen-type Schiff base ligands are described in this chapter. Most of these lanthanide-based clusters exhibit interesting “enclosed” structures, such as multi-decker, “twisted,” and drum-like structures. In these polynuclear complexes, the multidentate salen-type ligands can efficiently sensitize lanthanide emissions by serving as antennas that absorb excitation light and transfer the energy to the lanthanide centers. With the lanthanide ions encapsulated by chromophoric salen-type ligands and shielded from solvent molecules which can quench the emissions from lanthanide ions, those lanthanide-based clusters with “enclosed” structures show impressive luminescence properties.