Treatment of simulated berberine wastewater by electrochemical process with Pt/Ti anode
详细信息 查看全文
- 作者：Xiang Tu ; Shuhu Xiao ; Yonghui Song ; Dongsheng Zhang…
- 关键词：Berberine wastewater ; Electrochemical treatment ; Pt/Ti anode ; Active chlorines ; Removal efficiency
- 刊名：Environmental Earth Sciences
- 出版年：2015
- 出版时间：May 2015
- 年：2015
- 卷：73
- 期：9
- 页码：4957-4966
- 全文大小：794 KB
- 参考文献：Baquero F (2001) Low-level antibacterial resistance: a gateway to clinical resistance. Drug Resist Update Rev comment Antimicrob Anticancer Chemother 4(2):93-05View Article
Basha CA, Chithra E, Sripriyalakshmi NK (2009) Electro-degradation and biological oxidation of non-biodegradable organic contaminants. Chem Eng J 149(1-):25-4View Article
Bensalah N, Quiroz Alfaro MA, Martínez-Huitle CA (2009) Electrochemical treatment of synthetic wastewaters containing Alphazurine A dye. Chem Eng J 149(1-):348-52View Article
Bosco MV, Callao MP, Larrechi MS (2006) Simultaneous analysis of the photocatalytic degradation of polycyclic aromatic hydrocarbons using three-dimensional excitation–emission matrix fluorescence and parallel factor analysis. Anal Chim Acta 576(2):184-91View Article
Bu HM, Wan J, Zhang Y, Meng W (2013) Spatial characteristics of surface water quality in the Haicheng River (Liao River basin) in Northeast China. Environ Earth Sci 70(6):2865-872View Article
Bundschuh M, Pierstorf R, Schreiber WH, Schulz R (2011) Positive effects of wastewater ozonation displayed by in situ bioassays in the receiving stream. Environ Sci Technol 45(8):3774-780View Article
?erňáková M, Ko??álová D (2002) Antimicrobial activity of berberine–a constituent of mahonia aquifolium. Folia Microbiol 47(4):375-78View Article
Cilenti A, Provenzano MR, Senesi N (2005) Characterization of dissolved organic matter from saline soils by fluorescence spectroscopy. Environ Chem Lett 3(2):53-6View Article
da Silva BF, Jelic A, Lopez-Serna R, Mozeto AA, Petrovic M, Barcelo D (2011) Occurrence and distribution of pharmaceuticals in surface water, suspended solids and sediments of the Ebro river basin Spain. Chemosphere 85(8):1331-339View Article
Daneshvar N, Khataee AR, Ghadim ARA, Rasoulifard MH (2007) Decolorization of CI Acid Yellow 23 solution by electrocoagulation process: investigation of operational parameters and evaluation of specific electrical energy consumption (SEEC). Journal Hazardous Materials 148(3):566-72View Article
de Oliveira GR, Fernandes NS, de Melo JV, da Silva DR, Urgeghe C, Martínez-Huitle CA (2011) Electrocatalytic properties of Ti-supported Pt for decolorizing and removing dye from synthetic textile wastewaters. Chem Eng J 168(1):208-14View Article
Drlica K (2003) The mutant selection window and antimicrobial resistance. J Antimicrob Chemother 52(1):11-7View Article
Ellis JB (2006) Pharmaceutical and personal care products (PPCPs) in urban receiving waters. Environ Pollut 144(1):184-89View Article
Ghernaout D, Naceur MW, Aouabed A (2011) On the dependence of chlorine byproducts generated species formation of the electrode material and applied charge during electrochemical water treatment. Desalination 270(1-):9-2View Article
González T, Domínguez JR, Palo P, Sánchez-Martín J, Cuerda-Correa EM (2011) Development and optimization of the BDD-electrochemical oxidation of the antibiotic trimethoprim in aqueous solution. Desalination 280(1-):197-02
Güven G, Perendeci A, Tanyola? A (2009) Electrochemical treatment of simulated beet sugar factory wastewater. Chem Eng J 151(1-):149-59View Article
He PJ, Zheng Z, Zhang H, Shao LM, Tang QY (2009) PAEs and BPA removal in landfill leachate with Fenton process and its relationship with leachate DOM composition. Sci Total Environ 407(17):4928-933View Article
Heeb F, Singer H, Pernet-Coudrier B, Qi W, Liu H, Longree P, Mueller B, Berg M (2012) Organic micropollutants in rivers downstream of the megacity Beijing: sources and mass fluxes in a large-scale wastewater irrigation system. Environ Sci Technol 46(16):8680-688View Article
Jara CC, Fino D, Specchia V, Saracco G, Spinelli P (2007) Electrochemical removal of antibiotics from wastewaters. Appl Catal B 70(1-):479-87View Article
Kosma CI, Lambropoulou DA, Albanis TA (2010) Occurrence and removal of PPCPs in municipal and hospital wastewaters in Greece. J Hazard Mater 179(1-):804-17View Article
Lahkimi A, Oturan MA, Oturan N, Chaouch M (2007) Removal of textile dyes from water by the electro-Fenton process. Environ Chem Lett 5(1):35-9View Article
Li Y, Fu J, Deng SG, Lu XY (2014) Optimization of mesoporous carbons for efficient adsorption of berberine hydrochloride from aqueous solutions. J Colloid Interface Sci 424:104-12View Article
Lin H, Niu JF, Xu JL, Huang HO, Li D, Yue ZH, Feng CH (2013a) Highly efficient and mild electrochemical mineralization of long-chain perfluorocarboxylic acids (C9–C10) by Ti/SnO2–Sb–Ce, Ti/SnO2–Sb/Ce–PbO2, and Ti/BDD Electrodes. Environ Sci Technol 47(22):13039-3046View Article
Lin H, Niu JF, Xu JL, Li Y, Pan YH (2013b) Electrochemical mineralization of sulfamethoxazole by Ti/SnO2-Sb/Ce-PbO2 anode: kinetics, reaction pathways, and energy cost evolution. Electrochim Acta 97:167-74View Article
Martins RC, Rossi AF, Quinta-Ferreira RM (2010) Fenton’s oxidation process for phenol - 作者单位：Xiang Tu (1) (2)
Shuhu Xiao (1) (2)
Yonghui Song (1) (2)
Dongsheng Zhang (1) (2)
Ping Zeng (1) (2)
1. State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China
2. Department of Urban Water Environmental Research, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China - 刊物类别：Earth and Environmental Science
- 刊物主题：None Assigned
- 出版者：Springer Berlin Heidelberg
- ISSN：1866-6299
文摘
The emergence of antibiotics in aquatic environment has led to an increasing concern about the potential environmental risks and the spread of antibacterial resistance among microorganisms. Electrochemical oxidation processes are promising technologies to treat low contents of toxic and bio-refractory pollutants in water. Anodic oxidation of berberine, the frequently detected antibiotic in surface waters, was carried out by using RuO2/Ti, IrO2/Ti, RuIrO2/Ti, and Pt/Ti electrodes. It showed that with Pt/Ti anode, the removal efficiency of berberine was significantly higher than that with the other electrodes. Moreover, all the four electrodes showed 3- times higher reaction rate constant in NaCl solution than in Na2SO4 solution. The addition of chloride salts increased the oxidation rate of berberines due to the formation of active chlorines. In the case of Pt/Ti anode and simulated berberine wastewater, the effects of applied anodic bias, initial pH, Cl?/sup> and berberine concentrations, and reaction time on the removal efficiency of berberines were investigated. Under the optimal conditions of applied bias of 2.0?V, initial pH of 5.0, and Cl?/sup> concentration of 0.1?mol/L, the removal efficiency was higher than 90.0?% after 1-h reaction when the berberine concentration was lower than 50?mg/L. The acute toxicity of the simulated berberine wastewater could be largely reduced under the optimum conditions. Ultraviolet–visible adsorption spectra and excitation–emission matrix fluorescence spectra also confirmed that although berberines could not be fully mineralized after 1?h of electrochemical treatment, most of them were easily oxidized and decomposed by the electrolysis, thus forming some intermediate products with simple aromatic structures. Based on the results obtained, the electrochemical process with Pt/Ti electrode can be a feasible alternative as a post-treatment or treatment for berberine wastewater.