Tuning Side Chain and Main Chain Order in a Prototypical Donor–Acceptor Copolymer: Implications for Optical, Electronic, and Photovoltaic Characteristics

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• 关键词：Aggregate states ; All‐polymer heterojunctions ; Alternating copolymers ; Ambipolar charge transport ; Ambipolar materials ; Backbone modifications ; Bilayer solar cells ; Charge separation ; Conformational disorder ; Crystalline phases ; Donor–acceptor copolymers ; Electron traps ; Energetic disorder ; Energy‐level alignment ; Fermi‐level alignment ; Fermi‐level pinning ; Interface dipole ; Interlayer ; Intrachain order ; Intragap states ; Microscopic morphology ; Mobility imbalance ; Mobility relaxation ; Monte Carl
• 刊名：Advances in Polymer Science
• 出版年：2017
• 出版时间：2017
• 年：2017
• 卷：272
• 期：1
• 页码：243-265
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• 作者单位：Marcel Schubert (20)
  Johannes Frisch (21)
  Sybille Allard (22)
  Eduard Preis (22)
  Ullrich Scherf (22)
  Norbert Koch (21) (23)
  Dieter Neher (24)
  
  20. Soft Matter Photonics, School of Physics and Astronomy, University of St Andrews, KY16 9SS, St Andrews, UK
  21. Institut für Physik and IRIS Adlershof, Humboldt-Universität zu Berlin, Brook-Taylor-Straße 6, 12489, Berlin, Germany
  22. Macromolecular Chemistry and Institute for Polymer Technology, Bergische Universität Wuppertal, Gaußstraße 20, 42119, Wuppertal, Germany
  23. Helmholtz Zentrum Berlin für Materialien und Energie GmbH, Albert-Einstein-Straße 15, 12489, Berlin, Germany
  24. Physics of Soft Matter, School of Physics and Astronomy, University of Potsdam, 14476, Potsdam, Germany
  
• 丛书名：Elementary Processes in Organic Photovoltaics
• ISBN：978-3-319-28338-8
• 卷排序：272

文摘

The recent development of donor–acceptor copolymers has led to an enormous improvement in the performance of organic solar cells and organic field-effect transistors. Here we describe the synthesis, detailed characterisation, and application of a series of structurally modified copolymers to investigate fundamental structure–property relationships in this class of conjugated polymers. The interplay between chemical structure and optoelectronic properties is investigated. These are further correlated to the charge transport and solar cell performance, which allows us to link their chemical structure to the observed physical properties.