Multi-color luminescence of hybrids based with lanthanide functionalized zeolite A and titania

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• 作者：Lei Chen ; Bing Yan
• 关键词：Hybrids ; Lanthanide polyoxometalate ; Lanthanide complex ; Functionalized zeolite A ; Ionic liquid ; Luminescence
• 刊名：Colloid & Polymer Science
• 出版年：2015
• 出版时间：June 2015
• 年：2015
• 卷：293
• 期：6
• 页码：1847-1853
• 全文大小：2,899 KB
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• 作者单位：Lei Chen (1)
  Bing Yan (1)
  
  1. Department of Chemistry, Tongji University, Siping Road 1239, Shanghai, 200092, China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Polymer Sciences
  Physical Chemistry
  Soft Matter and Complex Fluids
  Characterization and Evaluation Materials
  Food Science
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1435-1536

文摘

A so-called inside-outside double modification path is used to functionalize zeolite A (ZA) with two kinds of luminescent lanthanide species (Eu3+/Tb3+ complex of thenoyltrifluoroacetylacetone (TAA) and acetylacetone (AA), and lanthanide polyoxometalate (NaLnW₁₀O₃₆?2H₂O (LnW₁₀, Ln-?Eu, Tb, Dy)) to prepare the multi-component hybrid materials. ZA is functionalized with Eu3+/Tb3+ through ion exchange reaction, and then TTA/AA ligands are introduced through gas dispersion (ship in bottle) method to the inside channel or pore structure of ZA. On the other hand, another species, LnW₁₀, is fabricated onto the surface of ZA through ionic liquid (1-methyl-3-propionyloxy imidazolium bromide) coordinated to titania as linker. The prepared hybrids show the multi-color luminescence for different composition and excitation. The results provide a useful path to obtain multi-component lanthanide hybrids.