Three 2D mixed-ligand Co(II) coordination polymers containing flexible bis(benzimidazole) ligands with different spacers

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• 作者：Xu Zhang ; Yong Guang Liu ; BaoYi Yu ; Guang Hua Cui
• 刊名：Transition Metal Chemistry
• 出版年：2016
• 出版时间：March 2016
• 年：2016
• 卷：41
• 期：2
• 页码：213-223
• 全文大小：1,984 KB
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• 作者单位：Xu Zhang (1)
  Yong Guang Liu (1)
  BaoYi Yu (2)
  Guang Hua Cui (1)
  
  1. College of Chemical Engineering, North China University of Science and Technology, Tangshan, 063009, Hebei, China
  2. Department of Inorganic and Physical Chemistry, Ghent University, Krijgslaan 281 S3, 9000, Ghent, Belgium
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Catalysis
  Physical Chemistry
  Inorganic Chemistry
  
• 出版者：Springer Netherlands
• ISSN：1572-901X

文摘

Three new Co(II) coordination polymers, [Co(L1)(bpdc)] _n (1), [Co(L2)(ndc)(H₂O)·2H₂O] _n (2) and [Co(L3)(ndc)(H₂O)·H₂O] _n (3) (L1 = 1,2-bis(5,6-dimethylbenzimidazole)ethane, L2 = 1,3-bis(5,6-dimethylbenzimidazole)propane, L3 = 1,4-bis(5,6-dimethylbenzimidazole)butane, H₂bpdc = 4,4′-biphenyldicarboxylic acid, H₂ndc = 2,6-naphthalenedicarboxylic acid) have been synthesized under hydrothermal conditions and structurally characterized by X-ray crystallography. All three complexes feature (4,4) networks that extend into 3D supramolecular frameworks via hydrogen bonding interactions. The luminescence properties and catalytic activities of these complexes with respect to the degradation of methyl orange in a Fenton-like process have been investigated.