Infrared planar laser-induced fluorescence with a CW quantum-cascade laser for spatially resolved CO2 and gas properties

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• 作者：Christopher S. Goldenstein ; Victor A. Miller ; Ronald K. Hanson
• 关键词：Laser ; induced fluorescence ; Quantum ; cascade laser ; Infrared photophysics ; CO2
• 刊名：Applied Physics B: Lasers and Optics
• 出版年：2015
• 出版时间：August 2015
• 年：2015
• 卷：120
• 期：2
• 页码：185-199
• 全文大小：3,373 KB
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• 作者单位：Christopher S. Goldenstein (1)
  Victor A. Miller (1)
  Ronald K. Hanson (1)
  
  1. High Temperature Gasdynamics Laboratory, Stanford University, Stanford, CA, 94305, USA
  
• 刊物类别：Physics and Astronomy
• 刊物主题：Physics
  Electromagnetism, Optics and Lasers
  Physical Chemistry
  Laser Technology and Physics and Photonics
  Quantum Optics, Quantum Electronics and Nonlinear Optics
  Optical Spectroscopy and Ultrafast Optics
  Physics and Applied Physics in Engineering
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1432-0649

文摘

The design and demonstration of a new infrared laser-induced fluorescence (IR-LIF) technique that enables spatially resolved measurements of CO2, temperature, and pressure, with potential for velocity, are presented. A continuous-wave, wavelength-tunable, quantum-cascade laser (QCL) near \(4.3\,\upmu \hbox {m}\) with up to 120mW was used to directly excite the asymmetric-stretch fundamental-vibration band of CO2 for approximately 200 to \(10^5\) times more absorbance compared with previous IR-LIF techniques. This enabled LIF detection limits (signal-to-noise ratio of 1) of 20 and 70ppm of CO2 in Ar and \(\hbox {N}_2\), respectively, at 1 bar and 296K in static-cell experiments. Simplified and detailed kinetic models for simulating the LIF signal as a function of gas properties are presented and enable quantitative, calibration-free, IR-LIF measurements of CO2 mole fraction within 1of known values at 0.5r. By scanning the laser across two absorption transitions and performing a multi-line Voigt fit to the LIF signal, measurements of temperature, pressure, and \(\chi _{\hbox {CO}_2}\) within 2% of known values were obtained. LIF measurements of gas pressure at a repetition rate up to 200Hz (in argon) are also presented. Planar-LIF (PLIF) was used to image steady and unsteady CO2–Ar jets at 330 frames per second with a spatial signal-to-noise ratio (SNR) up to 25, corresponding to a detection limit (SNR=1) of 200 ppm with a projected pixel size of \(40\,\upmu \hbox {m}\). The gas pressure was measured within \(3 \pm 2\)% of the known value (1 bar) at 5Hz by scanning the QCL across the P(42) absorption transition and least-squares fitting a Voigt profile to the PLIF signal. Spatially resolved measurements of absolute CO2 mole fraction in a laminar jet are also presented.