Assessment of the Detrimental Effects of Steam on Al2O3-Scale Establishment

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• 作者：Wei Zhao ; Brian Gleeson
• 关键词：Steam effect ; Wagner’s theory ; Scale establishment ; Ni ; base alloy ; Critical volume fraction ; Hydrogen effect
• 刊名：Oxidation of Metals
• 出版年：2015
• 出版时间：June 2015
• 年：2015
• 卷：83
• 期：5-6
• 页码：607-627
• 全文大小：2,019 KB
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• 作者单位：Wei Zhao (1)
  Brian Gleeson (1)
  
  1. Department of Mechanical Engineering and Materials Science, University of Pittsburgh, Pittsburgh, PA, 15261, USA
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Inorganic Chemistry
  Tribology, Corrosion and Coatings
  Metallic Materials
  
• 出版者：Springer Netherlands
• ISSN：1573-4889

文摘

The effects of steam on the oxidation behavior of model Al₂O₃-scale forming Ni-base alloys at 1000?°C were studied. This was done by conducting tests using dry air and air +30?% H₂O (“wet air-in short) gas environments. It was found that the critical concentration of Al (N _Al * ) to form a continuous and protective alumina scale on Ni–Al–Cr alloys is increased when the environment is wet air. Based on a rigorous assessment of the parameters contained in Maak’s modification (Z Met 52:545, 1961) of Wagner’s criterion (Z Elektrochem 63:772, 1959) for the transition from internal oxidation to external scale formation, it was deduced that the factor that can change the critical concentration N _Al * to the extent measured is the critical volume fraction f _v * .