Evaluation of the potential impact of fluorine-rich fertilizers on the Guarani Aquifer System, Rio Grande do Sul, Southern Brazil
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- 作者：Maria Paula Casagrande Marimon (1)
Ari Roisenberg (2)
Antonio Pedro Viero (2)
Flávio Anastacio de Oliveira Camargo (3)
Alexandra Vieira Suhogusoff (2) - 关键词：Adsorption ; Clay ; Fertilizers ; Fluorine ; Guarani Aquifer System
- 刊名：Environmental Earth Sciences
- 出版年：2013
- 出版时间：May 2013
- 年：2013
- 卷：69
- 期：1
- 页码：77-84
- 全文大小：411KB
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Ari Roisenberg (2)
Antonio Pedro Viero (2)
Flávio Anastacio de Oliveira Camargo (3)
Alexandra Vieira Suhogusoff (2)
1. Departamento de Geografia, Universidade do Estado de Santa Catarina, Avenida Madre Benvenuta, 2007, Florianópolis, SC, 88035-001, Brazil
2. Departamento de Geologia, Instituto de Geociências, Universidade Federal do Rio Grande do Sul, Avenida Bento Gon?alves, 9500, Porto Alegre, RS, 91501-970, Brazil
3. Departamento de Ciências do Solo, Faculdade de Agronomia, Universidade Federal do Rio Grande do Sul, Avenida Bento Gon?alves, 7712, Porto Alegre, RS, 91540-000, Brazil - ISSN：1866-6299
文摘
It has been determined that the fluorine concentration reaches up to 11?mg?L? in the porous-confined Santa Maria Aquifer, Guarani Aquifer System, in the central region of the state of Rio Grande do Sul, southern Brazil. Due to the elevated fluorine content in the groundwater, which is the major supply for drinking water, several incidences of dental fluorosis occurred. This area is the largest tobacco producer in Brazil and has a long history of fertilizer application. The fluorine in the local groundwater is likely to have come from the use of apatite-based fertilizers. This hypothesis was tested by soil and water analyses. Fluorine concentration has been monitored in the field for 2?years. The data combined with laboratory experiments on the adsorption and leaching of fluorine in soils showed that fluorine is easily retained by adsorption on aluminum clay-rich soils (Udults). The local clay-rich soils present high cation exchange capacity, aluminum content, and low pH; they act as a trap for fluorine derived from fertilizer and play an important role in the mobility of fluorine.