Computational fluid dynamics modeling and analysis of Pd-based membrane module for CO2 capture from H2/CO2 binary gas mixture

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• 作者：Dong-Yoon Shin ; Kyung-Ran Hwang ; Jong-Soo Park…
• 关键词：Pd ; based Membrane ; CO2 Capture ; Computational Fluid Dynamics Model ; H2 Flux ; Module Structure
• 刊名：Korean Journal of Chemical Engineering
• 出版年：2015
• 出版时间：July 2015
• 年：2015
• 卷：32
• 期：7
• 页码：1414-1421
• 全文大小：1,042 KB
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• 作者单位：Dong-Yoon Shin (1)
  Kyung-Ran Hwang (2)
  Jong-Soo Park (3)
  Myung-June Park (1) (4)
  
  1. Department of Energy Systems Research, Ajou University, Suwon, 443-749, Korea
  2. Clean Fuel Department, Korea Institute of Energy Research, Daejeon, 305-343, Korea
  3. Energy Materials Center, Korea Institute of Energy Research, Daejeon, 305-343, Korea
  4. Department of Chemical Engineering, Ajou University, Suwon, 443-749, Korea
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Industrial Chemistry and Chemical Engineering
  Catalysis
  Materials Science
  Biotechnology
  
• 出版者：Springer New York
• ISSN：1975-7220

文摘

A Pd-based membrane module for the capture of CO2 from a H2/CO2 binary gas mixture was considered, and computational fluid dynamics modeling was used to predict the module performance. Detailed models of momentum and mass balances, including local flux as a function of local linear velocity, satisfactorily described CO2 fraction in a retentate tube when compared to the experimental data under various feed flow rates. By using the model, several cases having different geometries, including the location and diameter of feed tube and the number and location of the feed and retentate tubes, were considered. Among tested geometries, the case of two feed tubes with each offset by an angle, θ, of 45° from the center line, and a feed tube diameter of 2.45mm showed the increase of the feed flow rate up to 11.80% compared to the reference case while a CO2 fraction of 90% in the retentate, which was the criterion for effective CO2 capture in the present study, was guaranteed. This would result in a plausible reduction in capital expenditures for the CO2 capture process.