Distribution and fate of synthetic musks in the Songhua River, Northeastern China: influence of environmental variables

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• 作者：Binyu Lu ; Yujie Feng ; Peng Gao…
• 关键词：Synthetic musk ; Spatial and temporal distribution ; Fate ; Risk assessment ; Surface water and sediment
• 刊名：Environmental Science and Pollution Research
• 出版年：2015
• 出版时间：June 2015
• 年：2015
• 卷：22
• 期：12
• 页码：9090-9099
• 全文大小：2,090 KB
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  R
• 作者单位：Binyu Lu (1)
  Yujie Feng (1)
  Peng Gao (1) (2)
  Zhaohan Zhang (1)
  Nan Lin (1)
  
  1. State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, No. 73 Huanghe Road, Nangang District, Harbin, 150090, China
  2. Stockbridge School of Agriculture, University of Massachusetts, Amherst, MA, 01003, USA
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：Environment
  Environment
  Atmospheric Protection, Air Quality Control and Air Pollution
  Waste Water Technology, Water Pollution Control, Water Management and Aquatic Pollution
  Industrial Pollution Prevention
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1614-7499

文摘

Contamination levels and spatial and temporal distributions of six typical synthetic musks (SMs) in water and sediment of the Songhua River in Northeastern China were investigated. Experimental data for 72 water and 52 sediment samples collected at 29 sampling sites over 12?months spanning 2011-012 showed that the Songhua River had been contaminated to different degrees at various sites separately from the river’s source. The polycyclic musks 1,3,4,6,7,8-hexahydro-4,6,6,7,8,8-hexamethylcyclopenta-(g)-2-benzopyran (HHCB) (Galaxolide) and 7-acetyl-1,1,3,4,4,6-hexamethyl-1,2,3,4-tetrahydronaphthalene (AHTN) (Tonalide) were found most frequently and at the highest levels. Concentrations of HHCB were <2-7?ng/L in water and <0.5-7.5?ng/g dry weight (dw) in sediment. AHTN was <1-?ng/L in water and <0.5-.7?ng/g dw in sediment. Statistical relationships between SM concentrations and four environmental variables (temperature, illumination, runoff, and population density) in the Songhua River Basin were formulated. Concentration levels varied proportionately with the size of the city along the river, while the distribution patterns showed clear seasonal variations. HHCB/AHTN ratios mirrored the transfer and transmitting process of SMs. Concentrations of target compounds were correlated with each other, suggesting similar exposure sources. Environmental risk assessment of SMs presented seasonal variations and provided baseline information on SM exposure in the Songhua River Basin.