Kinetic fragility of binary and ternary glass forming liquid mixtures
详细信息 查看全文
- 作者：Hongxiang Gong (1)
Mingdao Sun (1)
Zijing Li (1)
Riping Liu (1)
Yongjun Tian (1)
Li-Min Wang (1) Limin_Wang@ysu.edu.cn - 刊名：The European Physical Journal E - Soft Matter
- 出版年：2011
- 出版时间：September 2011
- 年：2011
- 卷：34
- 期：9
- 页码：DOI: 10.1140/epje/i2
- 全文大小：517.2 KB
- 参考文献：1. C.A. Angell, J.M. Sare, E.J. Sare, J. Phys. Chem. 82, 2622 (1978).
2. J.M. Gordon, G.B. Rouse, J.H. Gibbs, W.M. Risen, J. Chem. Phys. 66, 4971 (1977).
3. P.R. Couchman, Nature (London) 298, 729 (1982).
4. Th. Blochowicz, C. Karle, A. Kudlik, P. Medick, I. Roggatz, M. Vogel, Ch. Tschirwitz, J. Wolber, J. Senker, E. R枚ssler, J. Phys. Chem. B 103, 4032 (1999).
5. A.L. Greer, Nature (London) 366, 303 (1993).
6. G. Foffi, W. Gotze, F. Sciortino, P. Tartaglia, Th. Voigtmann, Phys. Rev. Lett. 91, 085701 (2007).
7. P.K. Gupta, J.C. Mauro, J. Chem. Phys. 130, 094503 (2009).
8. A. Inoue, Acta Mater. 48, 279 (2000).
9. D. Turnbull, Contemp. Phys. 10, 473 (1969).
10. L.-M. Wang, Z. Li, Z. Chen, Y. Zhao, R. Liu, Y. Tian, J. Phys. Chem. B 114, 12080 (2010).
11. O.N. Senkov, Phys. Rev. B 76, 104202 (2007).
12. E.S. Park, J.H. Na, D.H. Kim, Appl. Phys. Lett. 91, 031907 (2007).
13. C.A. Angell, K.L. Ngai, G.B. McKenna, P.F. McMillan, S.W. Martin, J. Appl. Phys. 88, 3113 (2000).
14. S. Sastry, Nature (London) 409, 164 (2001).
15. L.M. Wang, R. Richert, Phys. Rev. Lett. 99, 185701 (2007).
16. L.-M. Wang, Y. Tian, R. Liu, Appl. Phys. Lett. 97, 181901 (2010).
17. H. Senapati, R.K. Kadiyala, C.A. Angell, J. Phys. Chem. 95, 7050 (1991).
18. L. Battezzati, A.L. Greer, Acta Metall. 37, 1791 (1989).
19. S. Mukherjee, Z. Zhou, J. Schroers, W.L. Johnson, W.K. Rhim, Appl. Phys. Lett. 84, 5010 (2004).
20. S. Mukherjee, J. Schroers, W.L. Johnson, W.-K. Rhim, Phys. Rev. Lett. 94, 245501 (2005).
21. S. Kojima, V.N. Novikov, M. Kodama, J. Chem. Phys. 113, 6344 (2000).
22. R. Fabian Jr., D.L. Sidebottom, Phys. Rev. B 80, 064201 (2009).
23. P.G. Santangelo, C.M. Roland, K.L. Ngai, A.K. Rizos, H. Katerinopoulos, J. Non-Cryst. Solids 172-174, 1084 (1994).
24. M. Cutroni, A. Mandanici, L. De Francesco, J. Non-Cryst. Solids 307-310, 449 (2002).
25. W. Huang, S. Shahriari, R. Richert, J. Chem. Phys. 123, 164504 (2005).
26. A. Minoguchi, K. Kitai, R. Nozaki, Phys. Rev. E 68, 031501 (2003).
27. M.S. Beevers, J. Crossley, D.C. Garrington, G. Williams, J. Chem. Soc. Fraday Trans. 73, 458 (1977).
28. B. Gerharz, G. Meier, E.W. Fischer, J. Chem. Phys. 92, 7110 (1990).
29. L.-M. Wang, Y. Tian, R. Liu, R. Richert, J. Phys. Chem. B 144, 3618 (2010).
30. L.-M. Wang, Y. Zhao, M. Sun, R. Liu, Y. Tian, Phys. Rev. E 82, 062502 (2010).
31. C.A. Angell, Chem. Rev. 102, 2627 (2002).
32. E.J. Sutter, C.A. Angell, J. Phys. Chem. 75, 1826 (1971).
33. A. M霉gica, M.E. Calahorra, M. Cort谩zar, Macromol. Chem. Phys. 203, 1088 (2002).
34. A.V. Lesikar, J. Phys. Chem. 80, 1005 (1976).
35. A.V. Lesikar, J. Chem. Phys. 66, 4263 (1977).
36. K. Takeda, O. Yamamuro, H. Suga, J. Therm. Anal. 38, 1847 (1992).
37. K. Takeda, K. Murata, S. Yamashita, J. Non-Cryst. Solids 231, 273 (1998).
38. K. Takeda, K. Murata, S. Yamashita, J. Phys. Chem. B 103, 3457 (1998).
39. G.G. Naumis, Phys. Rev. B 73, 172202 (2006).
40. K. Duvvuri, R. Richert, J. Phys. Chem. B 108, 10451 (2004).
41. L.-M. Wang, R. Richert, J. Phys. Chem. B 109, 11091 (2005).
42. K. Putz, P.F. Green, J. Non-Cryst. Solids 337, 254 (2004).
43. L.A. Shadowspeaker, R. Busch, Appl. Phys. Lett. 85, 2508 (2004).
44. H.-J. Fecht, W.L. Johnson, Mater. Sci. Eng. A 375-377, 2 (2004).
45. S. Pedersen, Viscosity, structure and glass formation in the AlCl_3-ZnCl_2 system, PhD thesis, Norges Teknisknaturvitenskaplige Universitet, Avhandling NR (2001).
46. Q. Qin, G.B. McKenna, J. Non-Cryst. Solids 352, 2977 (2006).
47. D. Cubicciotti, H. Eding, J. Chem. Phys. 40, 978 (1994).
48. P. Patnaik (Editor), Handbook of Inorganic Materials (McGraw-Hill, New York, 2003).
49. S. Jabrane, J.M. Letoffe, J.J. Counioux, P. Claudy, Thermochim. Acta 290, 31 (1996).
50. S. Sudo, M. Shimomura, N. Shinyashiki, S. Yagihara, J. Non-Cryst. Solids 307-310, 356 (2002).
51. P. Walstra, Physical Chemistry of Foods (Marcel Dekker Inc. New York, 2001).
52. P.M. Mehl, Thermochim. Acta 324, 215 (1998). - 作者单位：1. State Key Lab of Metastable Materials Science and Technology, and College of Materials Science and Engineering, Yanshan University, 066004 Qinhuangdao, Hebei, China
- 刊物类别：Physics and Astronomy
- 刊物主题：Physics
Soft Matter and Complex Fluids
Biotechnology
Physical Chemistry
Polymer Sciences - 出版者：Springer Berlin / Heidelberg
- ISSN：1292-895X
文摘
The experimental studies of liquid fragility in miscible binary and ternary glass forming mixtures reveal a general observation of the negative deviation in fragility upon mixing from the linear average of those of the components. Further analyses from ideal, near ideal to non-ideal mixing modes show that the deviation magnitude does not increase monotonically with mixing enthalpy, and a moderate intermolecular interaction would generate a largest reduction in fragility. Four eutectic systems, methyl-o-toluate-methyl-p-toluate, ZnCl2-AlCl3, glycerol-water, and fructose-water, are studied to locate the composition where the largest fragility deviation occurs in phase diagrams. It is found that the compositions with the fragility minima do not coincide with the eutectic points. The results partly explain the experimental observation that the best glass forming region is not located at the eutectic composition.