CO2 mineral sequestration by wollastonite carbonation
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- 作者：Wenjin Ding (1) (2)
Liangjie Fu (1) (2)
Jing Ouyang (1) (2)
Huaming Yang (1) (2) - 关键词：Wollastonite ; Mineral carbonation ; CO2 sequestration ; Sulfuric acid ; Ammonia
- 刊名：Physics and Chemistry of Minerals
- 出版年：2014
- 出版时间：July 2014
- 年：2014
- 卷：41
- 期：7
- 页码：489-496
- 全文大小：994 KB
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Liangjie Fu (1) (2)
Jing Ouyang (1) (2)
Huaming Yang (1) (2)
1. School of Minerals Processing and Bioengineering, Central South University, Changsha, 410083, China
2. Research Center for Mineral Materials, Central South University, Changsha, 410083, China - ISSN：1432-2021
文摘
In this paper, we demonstrated a new approach to CO2 mineral sequestration using wollastonite carbonation assisted by sulfuric acid and ammonia. Samples were characterized by X-ray diffraction, scanning electron microscopy, Fourier transform infrared spectroscopy, and 29Si nuclear magnetic resonance. The change in Gibbs free energy from ?23?kJ/mol for the leaching reaction of wollastonite to ?01?kJ/mol for the carbonation reaction indicated that these two reactions can proceed spontaneously. The leached and carbonated wollastonite showed fibrous bassanite and granular calcium carbonate, respectively, while the crystal structure of pristine wollastonite was destroyed and the majority of the Ca2+ in pristine wollastonite leached. The chemical changes in the phases were monitored during the whole process. A high carbonation rate of 91.1?% could be obtained under the action of sulfuric acid and ammonia at 30?°C at normal atmospheric pressure, indicating its potential use for CO2 sequestration.