Interpenetrated polymer networks in composites with poly(vinyl alcohol), micro- and nano-fibrillated cellulose (M/NFC) and polyHEMA to develop packaging materials
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- 作者：Huiyu Bai ; Yufei Li ; Wei Wang ; Guangliang Chen ; Orlando J. Rojas ; Weifu Dong…
- 关键词：Poly(vinyl alcohol) ; Micro ; and nano ; fibrillated cellulose ; Photo ; crosslinking ; Composite films ; Packaging
- 刊名：Cellulose
- 出版年：2015
- 出版时间：December 2015
- 年：2015
- 卷：22
- 期：6
- 页码：3877-3894
- 全文大小：2,456 KB
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Fortunati - 作者单位：Huiyu Bai (1) (2)
Yufei Li (1)
Wei Wang (1)
Guangliang Chen (3)
Orlando J. Rojas (4) (5)
Weifu Dong (1)
Xiaoya Liu (1)
1. The Key Laboratory of Food Colloids and Biotechnology, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, Wuxi, 214122, Jiangsu, China
2. State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Donghua University, Shanghai, 201620, China
3. Key Laboratory of Advanced Textile Materials and Manufacturing Technology, and Engineering Research Center for Eco-Dyeing and Finishing of Textiles, Ministry of Education, Zhejiang Sci-Tech University, Hangzhou, 310018, Zhejiang, China
4. Department of Forest Products Technology, School of Chemical Technology, Aalto University, P.O. Box 16300, 00076, Aalto, Finland
5. Departments of Forest Biomaterials and Chemical and Biomolecular Engineering, North Carolina State University, Raleigh, NC, 27695, USA - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Bioorganic Chemistry
Physical Chemistry
Organic Chemistry
Polymer Sciences - 出版者：Springer Netherlands
- ISSN：1572-882X
文摘
A novel method for the preparation of composites based on poly(vinyl alcohol) (PVA) and micro- and nano-fibrillated cellulose (M/NFC) is reported. The addition of crosslinking HEMA monomers and a photo-initiator enabled the formation of an interpenetrated polymer network that displayed enhanced interfacial adhesion and dispersion of (M/NFC) in the matrix. Photo-crosslinked PVA/(M/NFC)/polyHEMA composite films produced by casting followed by UV polymerization of HEMA were characterized by using several approaches. These included Fourier transform infrared and UV–Vis spectroscopies, differential scanning calorimetry, X-ray diffractometry, thermogravimetric analysis and dynamic mechanical analysis. The thermo-mechanical and optical properties as well as water absorption and vapor barrier abilities of the developed photo-crosslinked PVA/(M/NFC)/polyHEMA films were measured and the benefit of photo-crosslinking determined. The major degradation peak of photo-crosslinked PVA/(M/NFC)/polyHEMA composites increased substantially compared to that of the PVA/(M/NFC) system (from ~300 to ~350 °C). The water vapor permeability of PVA/(M/NFC)/polyHEMA composite films was reduced with HEMA loading (5.44 × 10?1, 5.10 × 10?1, 4.12 × 10?1, 4.31 × 10?1 g/m h Pa for 0, 5, 10 and 15 % HEMA, respectively). Overall, a new and facile method for the synthesis of PVA/(M/NFC)-based composite networks interpenetrated with cross-linked poly(HEMA) is demonstrated, offering excellent prospects for packaging applications. Keywords Poly(vinyl alcohol) Micro- and nano-fibrillated cellulose Photo-crosslinking Composite films Packaging