Development of surface imprinting polymer as a selective adsorbent for adsorbing and separating dibenzothiophene from fuel oil

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• 作者：Wenming Yang ; Lukuan Liu ; Zhiping Zhou ; Yang Cao…
• 关键词：Surface imprinting polymer ; Titanium dioxide ; Dibenzothiophene ; Desulfurization ; Adsorbent
• 刊名：Research on Chemical Intermediates
• 出版年：2015
• 出版时间：April 2015
• 年：2015
• 卷：41
• 期：4
• 页码：2619-2633
• 全文大小：491 KB
• 参考文献：1. Babich, IV, Moulijn, JA (2003) Fuel 82: pp. 607 CrossRef
  2. Jeon, HJ, Ko, CH, Kim, SH, Kim, JN (2009) Energy Fuel 23: pp. 2537 CrossRef
  3. Li, C, Jiang, ZX, Gao, JB, Yang, YX, Wang, SJ, Tian, FP, Sun, FX, Sun, XP, Ying, PL, Han, CR (2004) Chem. Eur. J. 10: pp. 2277 CrossRef
  4. Li, HM, He, LN, Lu, JD, Zhu, WS, Jiang, X, Wang, Y, Yan, YS (2009) Energy Fuel 23: pp. 1354 CrossRef
  5. Takahashi, A, Yang, FH, Yang, RT (2002) Ind. Eng. Chem. Res. 41: pp. 2487 CrossRef
  6. Tam, PS, Kittrell, JR, Eldridge, JW (1990) Ind. Eng. Chem. Res. 29: pp. 321 CrossRef
  7. Qian, EW (2008) J. Jpn. Petrol. Inst. 51: pp. 14 CrossRef
  8. Fang, YM, Hu, HQ (2007) Catal. Commun. 8: pp. 817 CrossRef
  9. Chang, JH, Kim, YJ, Lee, BH, Cho, KS, Ryu, HW, Chang, YK, Chang, HN (2001) Biotechnol. Prog. 17: pp. 876 CrossRef
  10. Shiomi, T, Matsui, M, Mizukami, F, Sakaguchi, K (2005) Biomaterials 26: pp. 5564 CrossRef
  11. Baggiani, C, Giraudi, G, Giovannoli, C, Tozzi, C, Anfossi, L (2004) Anal. Chim. Acta 504: pp. 43 CrossRef
  12. Kubo, T, Hosoya, K, Watabe, Y, Ikegami, T, Tanaka, N, Sano, T, Kaya, K (2004) J. Chromatogr. A 1029: pp. 37 CrossRef
  13. Say, R, Birlik, E, Ers?z, A, Y?lmaz, F, Gedikbey, T, Denizli, A (2003) Anal. Chim. Acta 480: pp. 251 CrossRef
  14. Gao, BJ, Lu, JH, Chen, ZP, Guo, JF (2009) Polymer 50: pp. 3275 CrossRef
  15. Han, DM, Fang, GZ, Yan, XP (2005) J. Chromatogr. A 1100: pp. 131 CrossRef
  16. Lu, C, Zhou, W, Han, B, Yang, H, Chen, X, Wang, X (2007) Anal. Chem. 79: pp. 5457 CrossRef
  17. Gao, D, Zhang, Z, Wu, M, Xie, C, Guan, G, Wang, D (2007) J. Am. Chem. Soc. 129: pp. 7859 CrossRef
  18. Schmidt, RH, Mosbach, K, Haupt, K (2004) Adv. Mater. 16: pp. 719 CrossRef
  19. Titirici, MM, Sellergren, B (2006) Chem. Mater. 18: pp. 1773 CrossRef
  20. Kodakari, N, Katada, N, Niwa, M (1997) Appl. Surf. Sci. 121-22: pp. 292 CrossRef
  21. Wu, GH, Wang, ZQ, Wang, J, He, CY (2007) Anal. Chim. Acta 582: pp. 304 CrossRef
  22. Pérez, N, Whitcombe, MJ, Vulfson, EN (2001) Macromolecules 34: pp. 830 CrossRef
  23. Li, F, Li, XM, Zhang, SS (2006) J. Chromatogr. A 1129: pp. 223 CrossRef
  24. Diltemiz, SE, Say, R, Büyüktiryaki, S, Hür, D, Den
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Catalysis
  Physical Chemistry
  Inorganic Chemistry
  
• 出版者：Springer Netherlands
• ISSN：1568-5675

文摘

A novel surface molecular imprinting approach was used to synthesize a desulfurization imprinting polymer (MIP-a href='/search?dc.title=SiO&facet-content-type=ReferenceWorkEntry&sortOrder=relevance' class='reference-link webtrekk-track' gaCategory="Internal link" gaLabel="SiO" gaAction="reference keyword">SiO2/TiO2). Its structure and characters were investigated by using infrared spectrophotometry, X-ray diffraction, field emission scanning electron microscopy, and nitrogen sorption measurements. The structural superiority of MIP-a href='/search?dc.title=SiO&facet-content-type=ReferenceWorkEntry&sortOrder=relevance' class='reference-link webtrekk-track' gaCategory="Internal link" gaLabel="SiO" gaAction="reference keyword">SiO2/TiO2 was reflected by the above measurements. The adsorption behavior of MIP-a href='/search?dc.title=SiO&facet-content-type=ReferenceWorkEntry&sortOrder=relevance' class='reference-link webtrekk-track' gaCategory="Internal link" gaLabel="SiO" gaAction="reference keyword">SiO2/TiO2 was evaluated by using batch static adsorption experiments by the kinetic, isotherm, and thermodynamic analyses. The experimental results show that the adsorption process follows a pseudo-second-order kinetic model and that the experimental data are well fitted with the Freundlich isothermal equation. The thermodynamic analysis indicate that the adsorption process is endothermic in nature. Meanwhile, it was further demonstrated that the prepared adsorbent has high specificity for dibenzothiophene. The approach we described would provide a new opportunity in the deep desulfurization field.