Depth profile of persistent and emerging organic pollutants upstream of the Three Gorges Dam gathered in 2012/2013

详细信息    查看全文

• 作者：Dominik Deyerling ; Jingxian Wang…
• 关键词：Monitoring ; Depth profile ; Persistent organic compounds ; Perfluoroalkylic acids ; Pharmaceutical residues ; Environmental fate
• 刊名：Environmental Science and Pollution Research
• 出版年：2016
• 出版时间：March 2016
• 年：2016
• 卷：23
• 期：6
• 页码：5782-5794
• 全文大小：847 KB
• 参考文献：Ahrens L, Yeung LWY, Taniyasu S, Lam PKS, Yamashita N (2011) Partitioning of perfluorooctanoate (PFOA), perfluorooctane sulfonate (PFOS) and perfluorooctane sulfonamide (PFOSA) between water and sediment. Chemosphere 85:731–737CrossRef
  Ali U, Syed JH, Junwen L, Sánchez-García L, Malik RN, Chaudhry MJI, Arshad M, Li J, Zhang G, Jones KC (2014) Assessing the relationship and influence of black carbon on distribution status of organochlorines in the coastal sediments from Pakistan. Environ Pollut 190:82–90CrossRef
  Bao L-J, Maruya KA, Snyder SA, Zeng EY (2012) China’s water pollution by persistent organic pollutants. Environ Pollut 163:100–108CrossRef
  Bergmann A et al (2012) The Yangtze-Hydro Project: a Chinese–German environmental program. Environ Sci Pollut Res 19:1341–1344CrossRef
  Bu Q, Wang B, Huang J, Deng S, Yu G (2013) Pharmaceuticals and personal care products in the aquatic environment in China: a review. J Hazard Mater 262:189–211CrossRef
  Campbell CG, Borglin SE, Green FB, Grayson A, Wozei E, Stringfellow WT (2006) Biologically directed environmental monitoring, fate, and transport of estrogenic endocrine disrupting compounds in water: a review. Chemosphere 65:1265–1280CrossRef
  Chang X, Meyer MT, Liu X, Zhao Q, Chen H, J-a C, Qiu Z, Yang L, Cao J, Shu W (2010) Determination of antibiotics in sewage from hospitals, nursery and slaughter house, wastewater treatment plant and source water in Chongqing region of Three Gorge Reservoir in China. Environ Pollut 158:1444–1450CrossRef
  CNEMC (2011) Bulletin on the Ecological and Environmental Monitoring Results of the Three Gorges Project 2011, China National Environmental Monitoring Center
  Daughton CG (2004) Non-regulated water contaminants: emerging research. Environ Impact Assess Rev 24:711–732CrossRef
  Deyerling D, Wang J, Hu W, Westrich B, Peng C, Bi Y, Henkelmann B, Schramm K-W (2014) PAH distribution and mass fluxes in the Three Gorges Reservoir after impoundment of the Three Gorges Dam. Sci Environ 491–492:123–130
  Duan Y-P, Meng X-Z, Wen Z-H, Chen L (2013) Acidic pharmaceuticals in domestic wastewater and receiving water from hyper-urbanization city of China (Shanghai): environmental release and ecological risk. Environ Sci Pollut Res 20:108–116CrossRef
  EPA (2008) Facts Sheet on Polycyclic Aromatic Hydrocarbons, United States Environmental Protection Agency
  Floehr T, Xiao H, Scholz-Starke B, Wu L, Hou J, Yin D, Zhang X, Ji R, Yuan X, Ottermanns R, Roß-Nickoll M, Schäffer A, Hollert H (2013) Solution by dilution?—A review on the pollution status of the Yangtze River. Environ Sci Pollut Res 20:6934–6971CrossRef
  Gao L, Shi Y, Li W, Niu H, Liu J, Cai Y (2012) Occurrence of antibiotics in eight sewage treatment plants in Beijing, China. Chemosphere 86:665–671CrossRef
  Heeb F, Singer H, Pernet-Coudrier B, Qi W, Liu H, Longrée P, Müller B, Berg M (2012) Organic micropollutants in rivers downstream of the Megacity Beijing: sources and mass fluxes in a large-scale wastewater irrigation system. Environ Sci Technol 46:8680–8688CrossRef
  Hobbs JJ (2008) World Regional Geography. Cengage Learning
  Jia H, Liu L, Sun Y, Li Y-F (2011) Endosulfan in China: Usage, Emissions and Residues. InTech
  Kannan K, Reiner JL, Yun SH, Perrotta EE, Tao L, Johnson-Restrepo B, Rodan BD (2005) Polycyclic musk compounds in higher trophic level aquatic organisms and humans from the United States. Chemosphere 61:693–700CrossRef
  Liu J-L, Wong M-H (2013) Pharmaceuticals and personal care products (PPCPs): a review on environmental contamination in China. Environ Int 59:208–224CrossRef
  Müller A, Schulz W, Ruck WKL, Weber WH (2011) A new approach to data evaluation in the non-target screening of organic trace substances in water analysis. Chemosphere 85:1211–1219CrossRef
  Pandelova M, Stanev I, Henkelmann B, Lenoir D, Schramm K-W (2009) Correlation of PCDD/F and PCB at combustion experiments using wood and hospital waste. Influence of (NH4)2SO4 as additive on PCDD/F and PCB emissions. Chemosphere 75:685–691CrossRef
  Qi P, Wang Y, Mu J, Wang J (2011) Aquatic predicted no-effect-concentration derivation for perfluorooctane sulfonic acid. Environ Toxicol Chem 30:836–842CrossRef
  Qi W, Müller B, Pernet-Coudrier B, Singer H, Liu H, Qu J, Berg M (2014) Organic micropollutants in the Yangtze River: seasonal occurrence and annual loads. Sci Total Environ 472:789–799CrossRef
  Sánchez-García L, Cato I, Gustafsson Ö (2010) Evaluation of the influence of black carbon on the distribution of PAHs in sediments from along the entire Swedish continental shelf. Mar Chem 119:44–51CrossRef
  Seth R, Mackay D, Muncke J (1999) Estimating the organic carbon partition coefficient and its variability for hydrophobic chemicals. Environ Sci Technol 33:2390–2394CrossRef
  Stahl T, Mattern D, Brunn H (2011) Toxicology of perfluorinated compounds. Environ Sci Europe 23:38CrossRef
  Tang JYM, McCarty S, Glenn E, Neale PA, Warne MSJ, Escher BI (2013) Mixture effects of organic micropollutants present in water: towards the development of effect-based water quality trigger values for baseline toxicity. Water Res 47:3300–3314CrossRef
  Tang JYM, Busetti F, Charrois JWA, Escher BI (2014) Which chemicals drive biological effects in wastewater and recycled water? Water Res 60:289–299CrossRef
  Tobiszewski M, Namieśnik J (2012) PAH diagnostic ratios for the identification of pollution emission sources. Environ Pollut 162:110–119CrossRef
  UNEP (2009) Governments unite to step-up reduction on global DDT reliance and add nine new chemicals under international treaty
  Wang B, Iino F, Yu G, Huang J, Morita M (2010) The pollution status of emerging persistent organic pollutants in China. Environ Eng Sci 27:215–225CrossRef
  Wang B, Cao M, Zhu H, Chen J, Wang L, Liu G, Gu X, Lu X (2013a) Distribution of perfluorinated compounds in surface water from Hanjiang River in Wuhan, China. Chemosphere 93:468–473CrossRef
  Wang J, Bi Y, Pfister G, Henkelmann B, Zhu K, Schramm K-W (2009) Determination of PAH, PCB, and OCP in water from the Three Gorges Reservoir accumulated by semipermeable membrane devices (SPMD). Chemosphere 75:1119–1127CrossRef
  Wang J, Bi Y, Pfister G, Henkelmann B, Zhu K, Schramm K-W (2013b) Erratum to “Determination of PAH, PCB, and OCP in water from the Three Gorges Reservoir accumulated by semipermeable membrane devices (SPMD)” [Chemosphere 75 (2009) 1119–1127]. Chemosphere 90:2483–2484CrossRef
  Wang J, Bernhöft S, Pfister G, Schramm K-W (2014) Water exposure assessment of aryl hydrocarbon receptor agonists in Three Gorges Reservoir, China using SPMD-based virtual organisms. Sci Total Environ 496:26–34CrossRef
  Weber J, Halsall CJ, Muir D, Teixeira C, Small J, Solomon K, Hermanson M, Hung H, Bidleman T (2010) Endosulfan, a global pesticide: a review of its fate in the environment and occurrence in the Arctic. Sci Total Environ 408:2966–2984CrossRef
  Wode F, Reilich C, van Baar P, Dünnbier U, Jekel M, Reemtsma T (2012) Multiresidue analytical method for the simultaneous determination of 72 micropollutants in aqueous samples with ultra high performance liquid chromatography–high resolution mass spectrometry. J Chromatogr A 1270:118–126CrossRef
  Wolf A, Bergmann A, Wilken R-D, Gao X, Bi Y, Chen H, Schüth C (2013) Occurrence and distribution of organic trace substances in waters from the Three Gorges Reservoir, China. Environ Sci Pollut Res, 1-16
  Xie S, Wang T, Liu S, Jones KC, Sweetman AJ, Lu Y (2013) Industrial source identification and emission estimation of perfluorooctane sulfonate in China. Environ Int 52:1–8CrossRef
  Xing Y, Lu Y, Dawson RW, Shi Y, Zhang H, Wang T, Liu W, Ren H (2005) A spatial temporal assessment of pollution from PCBs in China. Chemosphere 60:731–739CrossRef
  Xu X, Tan Y, Yang G, Li H, Su W (2011) Impacts of China’s Three Gorges Dam Project on net primary productivity in the reservoir area. Sci Total Environ 409:4656–4662CrossRef
  Xu X, Tan Y, Yang G (2013) Environmental impact assessments of the Three Gorges Project in China: issues and interventions. Earth-Sci Rev 124:115–125CrossRef
  Yan Q, Gao X, Chen Y-P, Peng X-Y, Zhang Y-X, Gan X-M, Zi C-F, Guo J-S (2014) Occurrence, fate and ecotoxicological assessment of pharmaceutically active compounds in wastewater and sludge from wastewater treatment plants in Chongqing, the Three Gorges Reservoir Area. Sci Total Environ 470–471:618–630CrossRef
  Yang S, Xu F, Wu F, Wang S, Zheng B (2014) Development of PFOS and PFOA criteria for the protection of freshwater aquatic life in China. Sci Total Environ 470–471:677–683CrossRef
  Yang Y, Cao X, Zhang M, Wang J (2015) Occurrence and distribution of endocrine-disrupting compounds in the Honghu Lake and East Dongting Lake along the Central Yangtze River, China. Environ Sci Pollut Res, 1-9
  Yang Z, Shen Z, Gao F, Tang Z, Niu J (2009) Occurrence and possible sources of polychlorinated biphenyls in surface sediments from the Wuhan reach of the Yangtze River, China. Chemosphere 74:1522–1530CrossRef
  Yunker MB, Macdonald RW, Vingarzan R, Mitchell RH, Goyette D, Sylvestre S (2002) PAHs in the Fraser River basin: a critical appraisal of PAH ratios as indicators of PAH source and composition. Org Geochem 33:489–515CrossRef
  Zhang L, Shi S, Dong L, Zhang T, Zhou L, Huang Y (2011) Concentrations and possible sources of polychlorinated biphenyls in the surface water of the Yangtze River Delta, China. Chemosphere 85:399–405CrossRef
  Zhang X-X, Zhang T, Fang HP (2009) Antibiotic resistance genes in water environment. Appl Microbiol Biotechnol 82:397–414CrossRef
  Zhou H, Zhang Q, Wang X, Zhang Q, Ma L, Zhan Y (2014) Systematic screening of common wastewater-marking pharmaceuticals in urban aquatic environments: implications for environmental risk control. Environ Sci Pollut Res 21:7113–7129CrossRef
  
• 作者单位：Dominik Deyerling (1) (2)
  Jingxian Wang (1) (3)
  Yonghong Bi (3)
  Chengrong Peng (3)
  Gerd Pfister (2)
  Bernhard Henkelmann (2)
  Karl–Werner Schramm (2) (4)
  
  1. Technische Universität München, Wissenschaftszentrum Weihenstephan für Ernährung, Landnutzung und Umwelt, Lehrstuhl für analytische Lebensmittelchemie, Alte Akademie 10, 85354, Freising, Germany
  2. Helmholtz Zentrum München – German Research Center for Environmental Health, Molecular EXposomics, Ingolstaedter Landstr. 1, 85764, Neuherberg, Germany
  3. The State Key Laboratory of Freshwater Ecology and Biotechnology, Institute of Hydrobiology, Chinese Academy of Sciences, Wuhan, 430072, China
  4. Department für Biowissenschaften, Technische Universität München, Wissenschaftszentrum Weihenstephan für Ernährung, Landnutzung und Umwelt, Weihenstephaner Steig 23, 85350, Freising, Germany
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：Environment
  Environment
  Atmospheric Protection, Air Quality Control and Air Pollution
  Waste Water Technology, Water Pollution Control, Water Management and Aquatic Pollution
  Industrial Pollution Prevention
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1614-7499

文摘

Persistent and emerging organic pollutants were sampled in September 2012 and 2013 at a sampling site in front of the Three Gorges Dam near Maoping (China) in a water depth between 11 and 61 m to generate a depth profile of analytes. A novel compact water sampling system with self-packed glass cartridges was employed for the on-site enrichment of approximately 300 L of water per sample to enable the detection of low analytes levels in the picogram per liter-scale in the large water body. The overall performance of the sampling system was acceptable for the qualitative detection of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), organochlorine pesticides (OCPs), perfluoroalkylic acids (PFAAs), pharmaceutical residues and polar pesticides. Strongly particle-associated analytes like PAHs and PCBs resided mainly in the glass wool filter of the sampling system, whereas all other compounds have mainly been enriched on the XAD-resin of the self-packed glass cartridges. The sampling results revealed qualitative information on the presence, depth distribution and origin of the investigated compounds. Although the depth profile of PAHs, PCBs, OCPs, and PFAAs appeared to be homogeneous, pharmaceuticals and polar pesticides were detected in distinct different patterns with water depth. Source analysis with diagnostic ratios for PAHs revealed their origin to be pyrogenic (burning of coal, wood and grass). In contrast, most PCBs and OCPs had to be regarded as legacy pollutants which have been released into the environment in former times and still remain present due to their persistence. The abundance of emerging organic pollutants could be confirmed, and their most abundant compounds could be identified as perfluorooctanoic acid, diclofenac and atrazine among investigated PFAAs, pharmaceuticals and polar pesticides, respectively.