Synthesis of polyamidoxime-functionalized nanoparticles for uranium(VI) removal from neutral aqueous solutions

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• 作者：Li Huang ; Lixia Zhang ; Daoben Hua
• 关键词：Uranium(VI) ; Nanoparticles ; Polyamidoxime ; Sorption
• 刊名：Journal of Radioanalytical and Nuclear Chemistry
• 出版年：2015
• 出版时间：August 2015
• 年：2015
• 卷：305
• 期：2
• 页码：445-453
• 全文大小：1,335 KB
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• 作者单位：Li Huang (1)
  Lixia Zhang (2)
  Daoben Hua (1) (2) (3)
  
  1. College of Chemistry, Chemical Engineering and Materials Science & School for Radiological and Interdisciplinary Sciences (RAD–X), Soochow University, Suzhou, 215123, China
  2. Collaborative Innovation Center of Radiological Medicine of Jiangsu Higher Education Institutions, Suzhou, 215123, China
  3. School of Radiation Medicine and Protection, Medical College, Soochow University, Suzhou, 215123, China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Nuclear Chemistry
  Physical Chemistry
  Nuclear Physics, Heavy Ions and Hadrons
  Diagnostic Radiology
  Inorganic Chemistry
  
• 出版者：Akad茅miai Kiad贸, co-published with Springer Science+Business Media B.V., Formerly Kluwer Academic
• ISSN：1588-2780

文摘

It is important to separate uranium(VI) from water environment due to its high toxicity and radioactivity. A new kind of polystyrene nanoparticles with polyamidoxime is reported here for removal of uranium(VI) from aqueous solutions. The obtained PSt nanoparticles have a tunable sorption capacity. The sorption process follows pseudo-second-order kinetics, and the equilibrium can be reached within 6?h. Furthermore, the optimal pH value of sorption process is 6.5, and the adsorbents can be recycled well for uranium(VI) sorption from aqueous solution. This work indicates that the polyamidoxime-functionalized PSt nanoparticles may be used as a good adsorbent for the removal of uranium(VI) from neutral aqueous solution.