Mineralogical characteristics of airborne particles collected in Beijing during a severe Asian dust storm period in spring 2002
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  • 作者:LongYi Shao (1) (2)
    WeiJun Li (1) (2)
    ShuShen Yang (1) (2)
    ZongBo Shi (3)
    SenLin Lü (1) (2)
  • 关键词:Asian dust storm (ADS) ; inhalable particle (PM10) ; X ; ray diffraction (XRD) ; individual particles analysis ; Beijing
  • 刊名:Science China Earth Sciences
  • 出版年:2007
  • 出版时间:June 2007
  • 年:2007
  • 卷:50
  • 期:6
  • 页码:953-959
  • 全文大小:3857KB
  • 参考文献:1. Duce R A, Unni C K, Ray B J, et al. Long-range atmospheric transport of soil dust from Asia to the tropical North Pacific: temporal variability. Science, 1980, 209: 1522-524 CrossRef
    2. Iwasaka Y, Yamato M, Imasu R, et al. Transport of Asian dust (KOSA) particles; importance of weak KOSA events on the geochemical cycle of soil particles. Tellus, 1988, 40B: 494-03 CrossRef
    3. Husar R B, Tratt D M, Schichtel B A, et al. Asian dust events of April 1998. J Geophys Res, 2001, 106: 18317-8330 CrossRef
    4. Andreae M O. Climate effects of changing atmospheric aerosol levels. In Future Climates of the World: A Modeling Perspective, ed. A. Henderson-Sellers, New York: Elsevier, 1995. 341-92
    5. Buseck P R, Pósfai M. Airborne minerals and related aerosol particles: Effects on climate and the environment. Proc Natl Acad Sci USA, 1999, 96: 3372-379 CrossRef
    6. Prospero J M. Long-range transport of mineral dust in the global atmosphere: Impact of African dust on the environment of the southeastern United States. Proc Natl Acad Sci USA, 1999, 96: 3396-403 CrossRef
    7. Bishop J K B, Davis R E, Sherman J T. Robotic observations of dust storm enhancement of carbon biomass in the North Pacific. Science, 2002, 298: 817-21 CrossRef
    8. Zhang D, Iwasaka Y, Shi G, et al. Separated status of the natural dust plume and polluted air masses in an Asian dust storm event at coastal areas of China. J Geophys Res, 2005, 110, D06302, doi:10.1029/2004JD005305 CrossRef
    9. Davis B L, Guo J. Airborne particulate study in five cities of China, Atmos Environ, 2000, 34, 2703-711 CrossRef
    10. Zhang X Y, Zhang G, Zhu D, et al. Elemental tracers for Chinese source dust. Sci China Ser D-Earth Sci, 1996, 39(5): 512-21
    11. Zhang D Z, Zhao C S, Qin Y. Composition and morphology analyses of dust particles. Acta Sci Circumst, 1998, 18(5): 450-56
    12. Zhuang G S, Guo J H, Yuan H, et al. The compositions, sources, size distribution of dust particles and the influence of global environment during dust storm in 2000 in China. Chin Sci Bull (in Chinese), 2001, 46(3): 191-97
    13. Zhang R J, Xue Y F, Han Z W. The chemical characteristics and sources of PM2.5 in Beijing during ACE-Asia. Chin Sci Bull. (in Chinese), 2003, 48(7): 730-33
    14. Shi Z, Shao L, Jones T P, et al. Microscopy and mineralogy of airborne particles collected during severe dust storm episodes in Beijing, China. J Geophys Res, 110, 2005, D01303, doi:10.1029/2004 JD005073 CrossRef
    15. Shao L Y, Shi Z B. Microscopic characteristics and size distribution of summer PM10 in the air of a northwestern urban site and a clean air site in Beijing. Environ Sci (in Chinese), 2003, 24(5): 11-6
    16. Lü S L, Shao L Y, Jones T P. Mineralogy studies on Beijing urban inhalable particulate matter (PM10). China Environ Sci (in Chinese), 2005, 25(2): 129-32
    17. Chung Y, Kim H, Dulam J, et al. On heavy dustfall observed with explosive sandstorms in Chongwon-Chongju, Korea in 2002. Atmos Environ, 2003, 37: 3425-433 CrossRef
    18. Ren Z H, Gao Q X, Su F Q, et al. The regional characteristics and dust influence of atmospheric environment in Beijing. Eng Sci (in Chinese), 2003, 5(2): 49-6
    19. Xu X F, Zhang X L. The process and situation of a severely dust storm in Beijing area. The Ninth National Atmospheric Environment Conference (in Chinese), Beijing, 2002, 40-5
    20. Alfaro S C, Gomes L, Rajot J L, et al. Chemical and optical characterization of aerosols measured in spring 2002 at the ACE-Asia supersite, Zhenbeitai, China. J Geophys Res, 2003,108(D23): 8641, doi:10.1029/2002JD003214 CrossRef
    21. Li W J, Shao L Y, Lü S L, Size distribution of airborne inhalable particles in northwestern urban Beijing during spring 2002. J Chin Electron Microscopy Soc (in Chinese), 2004, 23(5): 589-93
    22. Welton J E, SEM Petronlogy Atlas. Methods in Exploration Series (4). The American Association of Petroleum Geologists, Oklahoma, 1984. 1-37
    23. Avila A, Queralt-Mitjans I, Alarcón M. Mineralogical composition of African dust delivered by red rains over northeastern Spain. J Geophys Res, 1997, 102: 21868-1977 CrossRef
    24. Caquineau S, Gaudichet A, Gomes L, et al. Saharan dust: clay ratio as a relevant tracer to assess the origin of soil-derived aerosols. Geophys Res Lett, 1998, 25: 983-86 CrossRef
    25. Chamley, H., Clay Sedimentology. New York: Berlin. Heidelberg: Springer-Verlag, 1989. 1-21
  • 作者单位:LongYi Shao (1) (2)
    WeiJun Li (1) (2)
    ShuShen Yang (1) (2)
    ZongBo Shi (3)
    SenLin Lü (1) (2)

    1. The State Key Laboratory of Coal Resources and Safety Mining, China University of Mining and Technology, Beijing, 100083, China
    2. Department of Resources and Earth Sciences, China University of Mining and Technology, Beijing, 100083, China
    3. Faculty of Environmental and Symbiotic Sciences, Prefectural University of Kumamoto, Kumamoto, 862-8502, Japan
  • ISSN:1869-1897
文摘
Asian dust storm (ADS) samples were collected on March 20, 2002 in Beijing, China. High-resolution field emission scanning electron microscopy with energy dispersive X-ray detector (FESEM-EDX) and X-ray diffraction (XRD) were used to study the morphology, chemical compositions, number-size distributions and mineralogical compositions of ADS particles. The mineral particles were major components in the ADS samples, accounting for 94% by number. The XRD analysis indicated that the dust particles were dominated by clay (40.3%), and quartz (19.5%), followed by plagioclase (8.4%), calcite (7.5%), K-feldspar (1.5%), hematite (0.9%), pyrite (0.9%), hornblende (0.4%) and gypsum (0.3%), with a certain amount of noncrystalline materials (20.3%). Clay minerals were mainly illite/smectite mixed layers (78%), followed by illite (9%), kaolinite (6%), and chlorite (7%). In addition to these main minerals, FESEM-EDX also detected some trace minerals, such as dolomite, pyrite, thenardite, as well as heavy minerals represented by rutile, ilmenite and apatite. The mineralogical compositions of the 2002-03-20 Asian dust storm and the Saharan dust plumes were similar but the clay mineralogy showed a great distinction, with the illite/smectite mixed layers being common in the Asian dust storm but illite being common in the Saharan dust plumes.

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