Immobilization of photosystem I or II complexes on electrodes for preparation of photoenergy-conversion devices

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• 作者：Masaharu Kondo (1)
  Mizuki Amano (2)
  Takashi Joke (2)
  Shuichi Ishigure (2)
  Tomoyasu Noji (2)
  Takehisa Dewa (2)
  Yutaka Amao (3)
  Mamoru Nango (2) (3)
  
• 关键词：Photosystem ; Electrode ; Photoenergy conversion
• 刊名：Research on Chemical Intermediates
• 出版年：2014
• 出版时间：November 2014
• 年：2014
• 卷：40
• 期：9
• 页码：3287-3293
• 全文大小：543 KB
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• 作者单位：Masaharu Kondo (1)
  Mizuki Amano (2)
  Takashi Joke (2)
  Shuichi Ishigure (2)
  Tomoyasu Noji (2)
  Takehisa Dewa (2)
  Yutaka Amao (3)
  Mamoru Nango (2) (3)
  
  1. Center for Fostering Young and Innovative Researchers, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya, 466-8555, Japan
  2. Materials Science and Engineering, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya, 466-8555, Japan
  3. OCARINA, Osaka City University, 3-3-138 Sugimoto, Sumiyoshi-ku, Osaka, 558 8585, Japan
  
• ISSN：1568-5675

文摘

Photosystems, PSI and PSII isolated from Thermosynechococcus elongatus were successfully immobilized on a TiO2 nanostructured film for use in dye-sensitized biosolar cells (DSBCs). The photosystem complexes were also immobilized on an ITO electrode modified with 3-aminopropyltriethoxysilane by utilizing the interactions between the electrode and the surface of the PSI or PSII polypeptide. Illumination of the PSI and PSII complexes immobilized on the ITO electrode resulted in action spectra?in the presence of methyl viologen, which corresponded to the absorption spectra of the complexes. Compared with the ITO electrode, PSI or PSII complexes assembled on the TiO2 electrode had much higher energy-conversion efficiency in the presence of an iodide/triiodide redox system of an ionic-liquid-based electrolyte. This could have interesting applications in the development of DSBCs.