Synthetic Bioinorganic Chemistry: Scorpionates Turn 50

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• 关键词：Bioinorganic chemistry ; Carbonic anhydrase ; Copper ; Gold ; Iron ; Manganese ; Mercury ; Molybdenum ; Nickel ; Scorpionates ; Silver ; Synthesis ; Thiolate complexes ; Tris(carbene)borates ; Tris(mercaptoimidazolyl)borates ; Tris(phosphino)borates ; Tris(pyrazolyl)borate ; Tris(thioether)borates ; Tris(triazolyl)borates ; Tungsten ; Vanadium ; Zinc
• 刊名：Structure & Bonding
• 出版年：2016
• 出版时间：2016
• 年：2016
• 卷：172
• 期：1
• 页码：139-157
• 全文大小：615 KB
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• 作者单位：Daniel Rabinovich (3)
  
  3. Department of Chemistry, The University of North Carolina at Charlotte, 9201 University City Boulevard, Charlotte, NC, 28223, USA
  
• 丛书名：50 Years of Structure and Bonding – The Anniversary Volume
• ISBN：978-3-319-35138-4
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Inorganic Chemistry
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1616-8550
• 卷排序：172

文摘

The coordination chemistry of scorpionates, anionic tripodal boron-centered ligands that readily bind to virtually all main group, transition, and f-block metals, has had a profound effect in the development of synthetic bioinorganic chemistry during the past 50 years. Highlighted in this article are some of the most meaningful results published in the area, primarily in the preparation of structural and functional model compounds for the active sites in metalloproteins and metalloenzymes, a theme that encompasses topics as diverse as nitrogen fixation and heavy metal poisoning. It has also been 50 years since the genesis of Structure and Bonding, so let this account also be a celebration of the many contributions that the staunch serial has had on the entire field of inorganic chemistry during the past half century.