Sources of and variations in tropospheric CO in Central Siberia: Numerical experiments and observations at the Zotino Tall Tower Observatory

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• 作者：Yu. A. Shtabkin ; K. B. Moiseenko…
• 关键词：carbon monoxide ; Zotino Tall Tower Observatory (ZOTTO) station ; natural fires ; anthropogenic pollution ; regional transport
• 刊名：Izvestiya, Atmospheric and Oceanic Physics
• 出版年：2016
• 出版时间：January 2016
• 年：2016
• 卷：52
• 期：1
• 页码：45-56
• 全文大小：1,119 KB
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• 作者单位：Yu. A. Shtabkin (1)
  K. B. Moiseenko (1)
  A. I. Skorokhod (1)
  A. V. Vasileva (1)
  M. Heimann (2)
  
  1. A. M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences, Pyzhevskii per. 3, Moscow, 119017, Russia
  2. Max Planck Institute for Biogeochemistry, Jena, Germany
  
• 刊物主题：Geophysics/Geodesy; Climatology;
• 出版者：Springer US
• ISSN：1555-628X

文摘

Contributions of climatically significant natural and anthropogenic emission sources in northern Eurasia to seasonal carbon monoxide (CO) variations observed at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia in 2007–2011 have quantitatively been estimated using the GEOS-Chem chemical transport model. It is shown that the formation of a stable continental pollution plume from sources in Western Europe, European Russia and southern Siberia during winter plays an important role in the regional balance of surface CO and allows one to explain 55–80% of the amplitude of the CO annual cycle observed at the ZOTTO station (~70–90 ppbv). During the warm period, the effect of the anthropogenic factor is weakly pronounced, and the background concentration of CO is regulated, first and foremost, by the oxidation of biogenic volatile organic compounds and fire activity in the region.