Selective formation of aniline over nanogold incorporated cobalt loaded SBA 15 catalysts

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• 作者：Suraja Viswanathan (1)
  Binitha Narayanan (2)
  Zahira Yaakob (1)
  Pradeepan Periyat (3)
  Silija Padikkaparambil (1)
  
• 关键词：Nitrobenzene ; Selective reduction ; Aniline ; Nanogold catalysts
• 刊名：Journal of Porous Materials
• 出版年：2014
• 出版时间：June 2014
• 年：2014
• 卷：21
• 期：3
• 页码：251-262
• 全文大小：
• 参考文献：1. G.C. Muller, U.H. Kim, Endocrinology 102, 1429-435 (1978) CrossRef
  2. R. White, S. Jobling, S.A. Hoare, J.P. Sumpter, M.G. Parker, Endocrinology 135, 175-82 (1994)
  3. C. Furuta, A.K. Suzuki, S. Taneda, K. Kamata, H. Hayashi, Y. Mori, C. Li, G. Watanabe, K. Taya, Biol. Reprod. 70, 1527-533 (2004) CrossRef
  4. N. Mahata, A.F. Cunha, J.J.M. órfao, J.L. Figueiredo, Appl. Catal. A: Gen. 351, 204-09 (2008) CrossRef
  5. P. Sangeetha, P. Seetharamulu, K. Shanthi, S. Narayanan, K.S. Rama Rao, J. Mol. Catal. A: Chem. 273, 244-49 (2007) CrossRef
  6. E.A. Gelder, S.D. Jackson, C.M. Lok, Catal. Lett. 84, 205-06 (2002) CrossRef
  7. F. Figueras, B. Coq, J. Mol. Catal. A: Chem. 173, 223 (2001) CrossRef
  8. C.C. Torres, E.L. Jablonski, G.T. Baronetti, A.A. Castro, S.R. de Miguel, O.A. Scelza, M.D. Blanco, M.A. Pena Jimenez, L.G. Fierro, Appl. Catal. A 161, 213 (1997) CrossRef
  9. M.C. Macias Perez, C. Salinas Martinez de Lecea, A. Linares Solano, Appl. Catal. A 151, 461-75 (1997) CrossRef
  10. X.D. Wang, M.H. Liang, J.L. Zhang, Y. Wang, Curr. Org. Chem. 11, 299-14 (2007) CrossRef
  11. X. Yan, J. Sun, Y. Wang, J. Yang, J. Mol. Catal. A: Chem. 252, 17-2 (2006) CrossRef
  12. H. Liu, J. Deng, W. Li, Catal. Lett. 137, 261-66 (2010) CrossRef
  13. H.U. Blaser, H. Steiner, M. Studer, Chem. Cat. Chem. 1, 210-21 (2009)
  14. F.C. Lizana, S.G. Quero, M.A. Keane, Appl. Catal. A 334, 199-06 (2008) CrossRef
  15. E. Baumgarten, A. Fiebes, A. Stumpe, React. Funct. Polym. 33, 71-9 (1997) CrossRef
  16. H. Li, Q. Zhao, H. Li, J. Mol. Catal. A: Chem. 285, 29-5 (2008) CrossRef
  17. N. Yao, J. Chen, J. Zhang, J. Zhang, Catal. Commun. 9, 1510-516 (2008) CrossRef
  18. X.X. Han, Q. Chen, R.X. Zhou, J. Mol. Catal. A: Chem. 277, 210-14 (2007) CrossRef
  19. X. Yang, H. Liu, H. Zhong, J. Mol. Catal. A: Chem. 147, 55-2 (1999) CrossRef
  20. A. Corma, P. Sema, P. Concepcion, J.J. Calvino, J. Am. Chem. Soc. 130, 8748-753 (2008) CrossRef
  21. G.C. Bond, D.T. Thompson, Catal. Rev. 41, 319-88 (1999) CrossRef
  22. C. Mohr, H. Hofmeister, P. Claus, J. Catal. 213, 86-4 (2003) CrossRef
  23. C. Milone, C. Crisafulli, R. Ingoglia, L. Schipilliti, S. Galvagno, Catal. Today 122, 341-51 (2007) CrossRef
  24. X. Zhang, A. Corma, Angew. Chem. Int. Ed. 47, 4358-361 (2008) CrossRef
  25. M. Boronat, P. Concepcion, A. Corma, S. Gonzalez, F. Illas, P. Serna, J. Am. Chem. Soc. 129, 16230-6237 (2007) CrossRef
  26. L.F. Liotta, Catalysts 2, 299-02 (2012) CrossRef
  27. M. Shekhar, J. Wang, W.S. Lee, W.D. Williams, S.M. Kim, E.A. Stach, J.T. Miller, W.N. Delgass, F.H. Ribeiro, J. Am. Chem. Soc. 134, 4700-708 (2012) CrossRef
  28. P. Claus, Appl. Catal. A 291, 222-29 (2005) CrossRef
  29. X. Wang, N. Perret, J.J. Delgado, G. Blanco, X. Chen, C.M. Olmos, S. Bernal, M.A. Keane, J. Phys. Chem. C 117, 994-005 (2013) CrossRef
  30. F. Cárdenas-Lizana, S. Gómez-Quero, N. Perret, M.A. Keane, Catal. Sci. Technol. 1, 652-61 (2011) CrossRef
  31. N. Perret, X. Wang, L. Delannoy, C. Potvin, C. Louis, M.A. Keane, J. Catal. 286, 172-83 (2012) CrossRef
  32. F. Cardenas-Lizana, S. Gomez-Quero, N. Perret, M.A. Keane, Gold Bull. 42, 124-32 (2009) CrossRef
  33. F. Cardenas-Lizana, S. Gomez-Quero, A. Hugon, L. Delannoy, C. Louis, M.A. Keane, J. Catal. 262, 235-43 (2009) CrossRef
  34. F. Cardenas-Lizana, S. Gomez-Quero, M.A. Keane, Catal. Commun. 9, 475-81 (2008) CrossRef
  35. F. Cardenas-Lizana, S. Gomez-Quero, M.A. Keane, Chem. Sus. Chem. 1, 215-21 (2008) CrossRef
  36. H. Sakurai, M. Haruta, Appl. Catal. A 127, 93-05 (1995) CrossRef
  37. C. Milone, R. Ingoglia, L. Schipilliti, C. Crisafulli, G. Neri, S. Galvagno, J. Catal. 236, 80-0 (2005) CrossRef
  38. S. Schimpf, M. Lucas, C. Mohr, U. Rodemerck, A. Bruckner, J. Radnick, H. Hofmeister, P. Claus, Catal. Today 72, 63-8 (2002) CrossRef
  39. J.E. Bailie, H.A. Abdullah, J.A. Anderson, C.H. Rochester, N.V. Richardson, N. Hodge, J.G. Zhang, A. Burrows, C.J. Kiely, G.J. Hutchings, Phys. Chem. Chem. Phys. 3, 4113-121 (2001) CrossRef
  40. E. Klemm, B. Amon, H. Redlingshofer, E. Dieterich, G. Emig, Chem. Eng. Sci. 56, 1347-353 (2001) CrossRef
  41. V. Vishwanathan, V. Jayasri, P.M. Basha, N. Mahata, L.M. Sikhwivhilu, N.J. Coville, Catal. Commun. 9, 453-58 (2008) CrossRef
  42. K.K. Yeong, A. Gavriilidis, R. Zapf, V. Hessel, Catal. Today 81, 641-51 (2003) CrossRef
  43. S. Diao, W. Qian, G. Luo, F. Wei, Y. Wang, Appl. Catal. A 286, 30-5 (2005) CrossRef
  44. L. Petrov, K. Kumbilieva, N. Kirkov, Appl. Catal. 59, 31-3 (1990) CrossRef
  45. A.M. Venezia, G. Pantaleo, A. Longo, G. Di Carlo, M. Casaletto, F.L. Liotta, G. Deganello, J. Phys. Chem. B 109, 2821-827 (2005) CrossRef
  46. K.C. Wu, Y.L. Tung, Y.L. Chen, Y.W. Chen, Appl. Catal. B: Environ. 53, 111-16 (2004) CrossRef
  47. N. Lopez, T.V.W. Janssens, B.S. Clausen, Y. Xu, M. Mavrikakis, T. Bligaard, J.K. Norskov, J. Catal. 223, 232-35 (2004) CrossRef
  48. S.H. Overbury, L. Ortiz-Soto, H. Zhu, B. Lee, M.D. Amiridis, S. Dai, Catal. Lett. 95, 99-06 (2004) CrossRef
  49. J.T. Richardson, J.L. Propp, J. Catal. 98, 457-67 (1986) CrossRef
  50. H.K. Kuo, R.J. De Angelis, J. Catal. 68, 203-08 (1981) CrossRef
  51. S. Parambadath, A.P. Sing, Catal. Today 141, 161-67 (2009) CrossRef
  52. M.A. Keane, Appl. Catal. A: Gen. 271, 109-18 (2004) CrossRef
  53. M.A. Keane, P.M. Patterson, J. Chem. Soc., Faraday Trans. 92, 1413-421 (1996) CrossRef
  54. G. Tavoularis, M.A. Keane, J. Chem. Technol. Biotechnol. 74, 60-0 (1999) CrossRef
  55. M.M. Thackeray, W.I.F. David, J.B. Goodenough, Mater. Res. Bull. 17, 785-93 (1982) CrossRef
  56. L. Li, C. Jin, X.C. Wang, W.J. Ji, Y. Pan, T. van der Knaap, R. van der Stoel, C.T. Au, Catal. Lett. 129, 303-11 (2009) CrossRef
  57. B. Klingenberg, M.A. Vannice, Chem. Mater. 8, 2755-768 (1996) CrossRef
  58. M. Primeau, C. Vautey, M. Langlet, Thin Solid Films 310, 47-6 (1997) CrossRef
  59. P. Nkeng, F. Koening, L. Gautier, P. Chartier, G. Poillerat, J. Electroanal. Chem. 402, 81-9 (1996) CrossRef
  60. S. Wang, B. Zhang, C. Zhao, S. Li, M. Zhang, L. Yan, Appl. Surf. Sci. 257, 3358-362 (2011) CrossRef
  61. Y. Brik, M. Kacimi, M. Ziyad, F. Bozon-Verduraz, J. Catal. 202, 118-28 (2001) CrossRef
  62. B.A. Sexton, A.E. Hughes, T.W. Turney, J. Catal. 97, 390-06 (1986) CrossRef
  63. M.A. Langell, J.G. Kim, D.L. Pugmire, W. McCarroll, J. Vac. Sci. Technol., A 19, 1977-982 (2001) CrossRef
  64. Y. Mikhlin, M. Likhatski, Y. Tomashevich, A. Romanchenko, S. Erenburg, S. Trubina, J. Electron Spectrosc. 177, 24-9 (2010) CrossRef
  65. L. Makhova, Y. Mikhlin, A. Romanchenko, Nucl. Instrum. Methods A. 575, 75-7 (2007) CrossRef
  66. J.F. Moulder, W.F. Sticke, P.E. Sobol, K.D. Bomben, in: / Handbook of X- / Ray Photoelectron Spectroscopy, eds. by J. Chastain, R.C. King (Physical Electronics, Eden Prairie, MN, 1995)
  67. E.D. Park, J.S. Lee, J. Catal. 186, 1-1 (1999) CrossRef
  68. M.P. Casaletto, A. Longo, A. Martorana, A. Prestianni, A.M. Venezia, Surf. Interf. Anal. 38, 215-18 (2006) CrossRef
  69. S. Panigrahi, S. Basu, S. Praharaj, S. Pande, S. Jana, A. Pal, S.K. Gosh, T. Pal, J. Phys. Chem. C 111, 4596-605 (2007) CrossRef
  70. X. Zhang, H. Shi, B.Q. Xu, Angew. Chem. Int. Ed. 44, 7132-135 (2005) CrossRef
  71. T. Tsoncheva, L. Ivanova, J. Rosenholm, M. Linden, Appl. Catal. B: Environ. 89, 365-74 (2009) CrossRef
  72. X. Xu, J. Li, Z. Hao, W. Zhao, C. Hu, Mater. Res. Bull. 41, 406-13 (2006) CrossRef
  73. R.M. Koros, E.J. Nowak, Chem. Eng. Sci. 22, 470 (1967) CrossRef
  
• 作者单位：Suraja Viswanathan (1)
  Binitha Narayanan (2)
  Zahira Yaakob (1)
  Pradeepan Periyat (3)
  Silija Padikkaparambil (1)
  
  1. Department of Chemical and Process Engineering, Universiti Kebangsaan Malaysia (UKM), 43600, Bangi, Selangor, Malaysia
  2. Department of Chemistry, Sree Neelakanta Government Sanskrit College, Pattambi, Palakkad, 679306, Kerala, India
  3. Department of Chemistry, University of Calicut, Calicut, India
  
• ISSN：1573-4854

文摘

Nanogold was dispersed over cobalt-loaded SBA 15 to create an effective redox catalyst. The support was identified as spinel Co3O4 attached to mesoporous SBA 15 based on XRD, FTIR and TEM analyses. The gold crystallites were found to be in the nanosize range (8-5?nm) by the application of the Scherrer equation to the XRD data. XPS analysis provided insight into the state of the gold nanoparticles. The selective hydrogenation of nitrobenzene over nanogold doped cobalt-loaded SBA 15 catalysts was investigated in a fixed bed down flow reactor. The selectivity for the desired product, aniline, was very high with a maximum conversion of 98.9?% of nitrobenzene. The high catalytic performance is attributed to the efficient dispersion of gold nanoparticles over the support. Performing the reaction in the flow reactor maximizes the access of the reactants to the catalysts without the aid of any solvent, which further eliminates the filtration steps required to remove the catalyst after the reaction. Conducting the reaction at 200?°C facilitates the recovery of the product (aniline), from the catalyst, as soon as it is formed.