Study of photodegradation and photooxidation of p-arsanilic acid in water solutions at pH = 7: kinetics and by-products
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- 作者：Marianna Czaplicka ; Katarzyna Jaworek…
- 关键词：p ; Arsanilic acid ; Photodegradation ; Advanced oxidation ; Kinetics ; By ; products
- 刊名：Environmental Science and Pollution Research
- 出版年：2015
- 出版时间：November 2015
- 年：2015
- 卷：22
- 期：21
- 页码：16927-16935
- 全文大小：568 KB
- 参考文献：Arroyo-Abad U, Elizalde-Gonzalez MP, Hidalogo-Moreno CM, Mattusch J, Wennrich R (2011) Retention of phenylarsenicals in soils derived from volcanic metrials. J Hazard Mater 186:1328–1334CrossRef
B’Hymer C, Caruso JA (2004) Arsenic and its speciation analysis using high – performance liquid chromatography and inductively coupled plasma mass spectrometry. J Chromatogr A 1045:1–13CrossRef
Bednar AJ, Garbarino JR, Ferrer I, Rutherford DW, Wershaw RL, Ranville JF, Wildeman TR (2003) Photodegradation of roxarsone in poultry litter leachates. Sci Total Environ 302:237–245CrossRef
Blaser HU (2006) A golden boost to an old reaction. Science 313(5785):312–313CrossRef
Briviba K, Devasagayam TP, Sies H, Steenken S (1993) Selective para hydroxylation of phenol and aniline by singlet molecular oxygen. Chem Res Toxicol 6(4):548–553CrossRef
Burns EA, Strenli CA, Averell PR (1970) The analytical chemistry of nitrogen and its compounds. Wiley – Interscience, New York, p 51
Casiot C, Morin G, Juillot F, Bruneela O, Personn JC, Leblanc M, Duquesne K, Bonnefoy V, Elbaz-Poulichet F (2003) Bacterial immobilization and oxidation of arsenic in acid mine drainage (Carnoul"es creek, France). Water Res 37:2929–2936CrossRef
Chappel J, Chiswell B, Olszowy H (1995) Speciation of arsenic in a contaminated soil by solvent extraction. Talanta 43(3):323–329CrossRef
Chatterjee A (1999) Behaviour of anionic arsenic compounds in microwave system with nitric acid and hydrogen peroxide – preliminary laboratory study. Sci Total Environ 228:25–34CrossRef
Czaplicka M, Manko T, Wypych J (2005) Determination of chlorophenols and their photodegradation products in aqueous solutions using liquid-liquid extraction and solid phase microextraction - a comparison. Chem Anal (Warsaw) 50(5):887–896
Czaplicka M, Mańko T, Czarnul J, Wypych J (2009) Application of solid phase microextraction for determination of dihydroxybenzenes, trihydroxybenzenes and chlorohydroxybenzenes in water and wastewater. Fresenius Environ Bull 18(4):491–498
Czaplicka M, Kurowski R, Jaworek K, Bratek Ł (2013) Application of advanced oxidation processes for cleaning of industrial water generated in wet dedusting of shaft furnace gases. Environ Technol 34(9-12):1455–1462CrossRef
Czaplicka M, Bratek Ł, Jaworek K, Bonarski J, Pawlak S (2014) Photooxidation of p-arsanilic acid in acidic solutions: kinetics and the identification of by- products and reaction pathways. Chem Eng J 243:364–371CrossRef
EPA – 454/R-98-013, Locating and estimating air emissions from sources of arsenic and arsenic compounds. Office of Air Quality Planning and Standards, U.S. Environmental Protection Agency, Triangle Park, NC (June 1998)
Fendler JH, Gasowski GL (1968) Radiation-induced hydroxylation of nitrobenzene in dilute aqueous solution. J Org Chem 33(5):1865–1868CrossRef
Furusho Y, Maki T, Hasegawa H (2011) Selective separation of arsenic species from aqueos solutions with immobilized macrocyclic material containing solid phase extraction columns. Chemosphere 82:549–556CrossRef
Gong Z, Lu X, Ma M, Watt C, Le X (2002) Arsenic speciation analysis. Talanta 58:77–96CrossRef
Habuda-Stanić M, Kules M, Kalajdzi B, Romić Z (2007) Quality of graundwater in eastern Croatia. The problem of arsenic pollution. Desalination 210:157–162CrossRef
Hering JG (1996) Risk assessment for arsenic in drinking water: limits to achievable risk levels. J Hazard Mater 45:175–184CrossRef
Huang JH, Hu KN, Decker B (2011) Organic arsenic in yhe soil environment: speciation, occurrence, transformation and adsorption behaviour. Water Air Soil Pollut 219:401–415CrossRef
Jain CK, Ali J (2000) Arsenic: occurance, toxicity and speciation techniques. Water Res 34:4304–4312CrossRef
Jaworek K, Czaplicka M, Bratek Ł (2014) Decomposition of phenylarsonic acid by AOP processes: degradation rate constants and by products. Environ Sci Pollut Res 21:11917–11923CrossRef
Karabulut B, Tapramaz R (1999) EPR study of gamma irradiated arsanilic acid single crystal. Radiat Phys Chem 55:331–335CrossRef
Kenyon EM, Hughes MF (2001) A concise review of the toxicity and carcinogenicity of dimethylarsinic acid. Toxicology 160:227–236CrossRef
Kochany EL (1992) Degradation of nitrobenzene and nitrophenols by means of advanced oxidation processes in a homogeneous phase: photolysis in the presence of hydrogen peroxide versus the Fenton reaction. Chemosphere 24(7):1369–1380CrossRef
Kohler M, Hofmann K, Volsgen F, Thurow K, Koch A (2001) Bacterial relese of arsenic ions and organoarsenic compounds from soil contaminated by chemical warfare agents. Chemosphere 42:425–429CrossRef
Leermakers M, Morabito R, Quevauviller P (2006) Toxic arsenic compounds in environmental samples: Speciation and validation. Trends Anal Chem 25:1–10CrossRef
Melamed D (2005) Monitoring arsenic in the environment: a review of science and technologies with the potential for field measurements. Anal Chim Acta 532:1–13CrossRef
Miguel R, Andreas K, Sandra C, Esther C, Santiago E (2000) Influence of H2O2 and Fe(III) in the photodegradation of nitrobenzene. J Photochem Photobiol A 133(1–2):123–127
Patric JS, Ayala-Ferro F, Cullen WR, Carter DE, Aposhian HV (2000) Monomethylarsenous acid (MMAIII) is more toxic than arsenite in Chang Human Hepatocytes. Toxicol Appl Pharmacol 163:203–207CrossRef
Ringmann S, Boch K, Marquardt W, Schuster M, Schlemmer G, Kainrath P (2002) Microwave – assisted digestion of organoarsenic compounds for the determination of total arsenic in aqueous, biological, and sediment samples using flow injection hydride generation electrothermal atomic absorption spectrometry. Anal Chim Acta 452:207–215CrossRef
Romero A, Santos A, Vicente F, Rodriguez S, Lafuente L (2009) In situ oxidation remediation technologies: Kinetic of hydrogen peroxide decomposition on soil organic matter. J Hazard Mater 170:627–632CrossRef
Rubio R, Alberti J, Pedro A, Rauret G (1995) On – line photolytic decomposition for the determination of organoarsenic compounds. Trends Anal Chem 14(6):274–279CrossRef
Schaeffer R, Francesconi KA, Kienzl N, Soeroes C, Fodor P, Váradi L, Raml R, Goessler W, Kuehnelt D (2006) Arsenic speciation in freshwater organisms from the river Danube in Hungary. Talanta 69(4):856–865CrossRef
Schoene K, Bruckert HJ, Jurling H, Steinhanses J (1996) Derivatization of 10- chloro – 5, 10 – dihydrophenarsazine (Adamsite) for gas chromatographic analysis. J Chromatogr A 719:401–409CrossRef
Sheppard SC (1992) Summary of phytotoxic levels of soil arsenic. Water Air Soil Pollut 64:539–550CrossRef
Sierra-Alvarez R, Cortinas I, Field JA (2010) Methanogenic inhibition by roxarsone (4-hydroxy – 3 – nitro – phenylarsonic acid) and related aromatic arsenic compounds. J Hazard Mater 175:352–358CrossRef
Szostek B, Aldstadt JH (1998) Determination of organoarsenicals in the environment by solid-phase microextraction–gas chromatography–mass spectrometry. J Chromatogr A 807:253–263CrossRef
Tornes JA, Opstad AM, Johnsen BA (2006) Determination of organoarsenic warfare agents in sediment samples from Skagerrak by gas chromatography – mass spectrometry. Sci Total Environ 356:235–246CrossRef
Wang A, Chun HU, Jiuhui Q, Yang MY, Huijuan L, Jia R, Rong Q, Jingfang S (2008) Phototransformation of nitrobenzene in the Songhua River: Kinetics and photoproduct analysis. J Environ Sci 20:787–795CrossRef
Xu T, Kamat PV, Joshi S, Mebel AM, Cai Y, O’Shea KE (2007) Hydroxyl radical mediated degradation of phenylarsonic acid. J Phys Chem A 111:7819–7824CrossRef
Zhang Q, Minami H, Inoue S, Atsuya I (2004) Differential determination of trance amounts of As (III) and As (V) in seawater by solid sampling atomic absorption spectrometry. Anal Chim Acta 508:99–105CrossRef
Zheng S, Jiang W, Cai Y, Donysiou D, O’Shea KE (2014) Adsorption and photocatalytic degradation of aromatic organoarsenic compounds in TiO2 suspension. Catal Today 224:83–88CrossRef
Zheng S, Jiang W, Rashid M, Cai Y, Donysiou D, O’Shea KE (2015) Selective reduction of Cr (VI) in Chromium, Copper and Arsenic (CCA) mixed waste streams using UV/TiO2photocatalysis. Molecules 20(2):2622–2635CrossRef
Ziołek M (2004) Catalytic liquid-phase oxidation in heterogeneous system as green chemistry goal - Advantages and disadvantages of MCM-41 used as catalyst. Catal Today 90:145–150CrossRef - 作者单位：Marianna Czaplicka (1)
Katarzyna Jaworek (1)
Marta Bąk (1)
1. Institute of Non-Ferrous Metals, Gliwice, Sowinskiego 5, Poland - 刊物类别：Earth and Environmental Science
- 刊物主题：Environment
Environment
Atmospheric Protection, Air Quality Control and Air Pollution
Waste Water Technology, Water Pollution Control, Water Management and Aquatic Pollution
Industrial Pollution Prevention - 出版者：Springer Berlin / Heidelberg
- ISSN：1614-7499
文摘
The paper presents the kinetics and proposed pathways photodegradation and photooxidation of p-arsanilic acid, in a neutral environment by ozone and hydrogen peroxide. The results showed that in a neutral environment, photoozonation process was characterized by the highest decomposition rate constant (k) (k = 31.8 × 10−3 min−1). The rate constants decreased in the order UV/O3 > O3 > UV/H2O2 > H2O2 > UV. It was also found that under pH = 7, decomposition of p-arsanilic acid leads mainly to the formation of aniline, which undergoes secondary reactions. Intermediate products of oxidation and photooxidation by hydrogen peroxide like nitrobenzene, nitrophenol, azobenzenes, and phenylazophenol were identified depending on processes. However, in the photodegradation process, formation of nitrasone as a reaction product of p-arsanilic acid with oxygen in the singlet state was observed. In the case of ozonation and photoozonation, in addition, aniline formation of carboxylic acids was observed.