Synthesis of Conjugated Polymers with Complex Architecture for Photovoltaic Applications

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• 关键词：Catalyst ; transfer polycondensation ; Covalent preorganization ; Donor ; acceptor block copolymer ; Grafting ; from ; Grafting ; through ; Grafting ; to ; Hairy particles ; Morphology ; PCBM ; Self ; assembly ; Suzuki chain ; growth polycondensation
• 刊名：Advances in Polymer Science
• 出版年：2017
• 出版时间：2017
• 年：2017
• 卷：272
• 期：1
• 页码：351-376
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• 作者单位：Anton Kiriy (20)
  Frederik C. Krebs (21)
  
  20. Department of Polymer Structures, Leibniz-Institut für Polymerforschung Dresden e.V., Hohe Str. 6, 01069, Dresden, Germany
  21. DTU ENERGY, Department of Energy Conversion and Storage, Technical University of Denmark, Frederiksborgvej 399, Building 111, Room S05, 4000, Roskilde, Denmark
  
• 丛书名：Elementary Processes in Organic Photovoltaics
• ISBN：978-3-319-28338-8
• 卷排序：272

文摘

A common approach to bulk heterojunction solar cells involves a “trial-and-error” approach in finding optimal kinetically unstable morphologies. An alternative approach assumes the utilization of complex polymer architectures, such as donor–acceptor block copolymers. Because of a covalent preorganization of the donor and acceptor components, these materials may form desirable morphologies at thermodynamic equilibrium. This chapter reviews synthetic approaches to such architectures and shows the first photovoltaic results.