Novel D-em class="a-plus-plus">π–A dye sensitizers of polymeric metal complexes with triphenylamine derivatives as donor for dye-sensitized solar cells: synthesis, characterization and application

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• 作者：GUIPENG TANG ; JUN ZHOU ; WEI ZHANG ; JIAOMEI HU ; DAHAI PENG…
• 关键词：Transition metal ; dye sensitizer ; polymeric metal complex ; triphenylamine ; dye ; sensitized solar cells
• 刊名：Bulletin of Materials Science
• 出版年：2015
• 出版时间：April 2015
• 年：2015
• 卷：38
• 期：2
• 页码：467-474
• 全文大小：780 KB
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• 作者单位：GUIPENG TANG (1)
  JUN ZHOU (1)
  WEI ZHANG (1)
  JIAOMEI HU (1)
  DAHAI PENG (1)
  QIUFANG XIE (1)
  CHAOFAN ZHONG (1)
  
  1. Key Laboratory of Environmentally Friendly Chemistry and Applications of Ministry of Education, College of Chemistry, Xiangtan University, Xiangtan, Hunan, 411105, China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Materials Science
  Engineering, general
  
• 出版者：Springer India
• ISSN：0973-7669

文摘

Because of being the key component of dye-sensitized solar cells and acting as an important role, dye sensitizer and its synthesis and application has been extensively researched. In this paper, four novel polymeric metal complexes with D-em class="EmphasisTypeItalic">π–A structure that use 4-(octyloxymethyl)-N,N-diphenylbenzenamine as donor group (D), C =N bond as a π-conjugation linkage (π), and transition metal complexes as an acceptor (A), were functionally designed and synthesized. All the four polymeric metal complexes exhibited some photovoltaic performance, the highest photoelectric conversion efficiency of compound P4 reached 1.09% (J _sc = 2.55 mA cm?, V _oc = 0.61 V and FF = 70.14%) under simulate AM 1.5 G solar irradiation. A new path for the synthesis and study of the dye sensitizer was provided.