New insights into trace element wet deposition in the Himalayas: amounts, seasonal patterns, and implications
详细信息    查看全文
  • 作者:Zhiyuan Cong (1)
    Shichang Kang (1) (2)
    Yulan Zhang (1)
    Shaopeng Gao (1)
    Zhongyan Wang (1)
    Bin Liu (1) (3)
    Xin Wan (1) (3)

    1. Key Laboratory of Tibetan Environment Changes and Land Surface Processes
    ; Institute of Tibetan Plateau Research ; Chinese Academy of Sciences ; Building 3 ; Courtyard 16 ; Lincui Road ; Chaoyang District ; 100101 ; Beijing ; China
    2. State Key Laboratory of Cryospheric Sciences
    ; Cold and Arid Regions Environmental and Engineering Research Institute ; CAS ; 730000 ; Lanzhou ; China
    3. University of Chinese Academy of Sciences
    ; 100049 ; Beijing ; China
  • 关键词:Himalayas ; Trace elements ; Wet deposition ; Ice core ; Long ; range transport
  • 刊名:Environmental Science and Pollution Research
  • 出版年:2015
  • 出版时间:February 2015
  • 年:2015
  • 卷:22
  • 期:4
  • 页码:2735-2744
  • 全文大小:912 KB
  • 参考文献:1. Bacardit M, Camarero L (2010a) Atmospherically deposited major and trace elements in the winter snowpack along a gradient of altitude in the Central Pyrenees: the seasonal record of long-range fluxes over SW Europe. Atmos Environ 44:582鈥?95 CrossRef
    2. Bacardit M, Camarero L (2010b) Major and trace elements in soils in the Central Pyrenees: high altitude soils as a cumulative record of background atmospheric contamination over SW Europe. Environ Sci Pollut Res 17:1606鈥?621 CrossRef
    3. Barbante C, Boutron C, Morel C, Ferrari C, Jaffrezo JL, Cozzi G, Gaspari V, Cescon P (2003) Seasonal variations of heavy metals in central Greenland snow deposited from 1991 to 1995. J Environ Monit 5:328鈥?35 CrossRef
    4. Barbante C, Schwikowski M, D枚ring T, G盲ggeler HW, Schotterer U, Tobler L, Van de Velde K, Ferrari C, Cozzi G, Turetta A, Rosman K, Bolshov M, Capodaglio G, Cescon P, Boutron C (2004) Historical record of European emissions of heavy metals to the atmosphere since the 1650s from alpine snow/ice cores drilled near Monte Rosa. Environ Sci Technol 38:4085鈥?090 CrossRef
    5. Bonasoni P et al (2010) Atmospheric brown clouds in the Himalayas: first two years of continuous observations at the Nepal Climate Observatory-Pyramid (5079聽m). Atmos Chem Phys 10:7515鈥?531 CrossRef
    6. Canepari S, Astolfi M, Farao C, Maretto M, Frasca D, Marcoccia M, Perrino C (2013) Seasonal variations in the chemical composition of particulate matter: a case study in the Po Valley. Part II: concentration and solubility of micro-and trace-elements. Environmental Science and Pollution Research, 1鈥?3
    7. Cao J, Xu B, He J, Liu X, Han Y, Wang G, Zhu C (2009) Concentrations, seasonal variations, and transport of carbonaceous aerosols at a remote mountainous region in western China. Atmos Environ 43:4444鈥?452 CrossRef
    8. Cong Z, Kang S, Liu X, Wang G (2007) Elemental composition of aerosol in the Nam Co region, Tibetan Plateau, during summer monsoon season. Atmos Environ 41:1180鈥?187 CrossRef
    9. Cong Z, Kang S, Dong S, Liu X, Qin D (2010a) Elemental and individual particle analysis of atmospheric aerosols from high Himalayas. Environ Monit Assess 160:323鈥?35 CrossRef
    10. Cong Z, Kang S, Zhang Y, Li X (2010b) Atmospheric wet deposition of trace elements to central Tibetan Plateau. Appl Geochem 25:1415鈥?421 CrossRef
    11. Cong ZY, Kang SC, Qin DH (2009) Seasonal features of aerosol particles recorded in snow from Mt. Qomolangma (Everest) and their environmental implications. J Environ Sci-China 21:914鈥?19 CrossRef
    12. Davidson CI, Chu L, Grimm TC, Nasta MA, Qamoos MP (1981) Wet and dry deposition of trace elements onto the Greenland ice sheet. Atmos Environ 15:1429鈥?437 CrossRef
    13. Decesari S, Facchini MC, Carbone C, Giulianelli L, Rinaldi M, Finessi E, Fuzzi S, Marinoni A, Cristofanelli P, Duchi R, Bonasoni P, Vuillermoz E, Cozic J, Jaffrezo JL, Laj P (2010) Chemical composition of PM10 and PM1 at the high-altitude Himalayan station Nepal Climate Observatory-Pyramid (NCO-P) (5079聽m聽a.s.l.). Atmos Chem Phys 10:4583鈥?596 CrossRef
    14. Draxler RR, Rolph GD (2003) HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) model access via NOAA ARL READY website (http://www.arl.noaa.gov/ready/hysplit4.html). NOAA Air Resources Laboratory, Silver Spring, MD
    15. Engling G, Zhang Y-N, Chan C-Y, Sang X-F, Lin M, Ho K-F, Li Y-S, Lin C-Y, Lee JJ (2011) Characterization and sources of aerosol particles over the southeastern Tibetan Plateau during the Southeast Asia biomass-burning season. Tellus B 63:117鈥?28 CrossRef
    16. Fang G-C, Huang Y-L, Huang J-H (2010) Study of atmospheric metallic elements pollution in Asia during 2000鈥?007. J Hazard Mater 180:115鈥?21 CrossRef
    17. Gabrieli J, Carturan L, Gabrielli P, Kehrwald N, Turetta C, Cozzi G, Spolaor A, Dinale R, Staffler H, Seppi R (2011) Impact of Po Valley emissions on the highest glacier of the eastern European Alps. Atmos Chem Phys 11:8087鈥?102 CrossRef
    18. Gaspari V, Barbante C, Cozzi G, Cescon P, Boutron CF, Gabrielli P, Capodaglio G, Ferrari C, Petit JR, Delmonte B (2006) Atmospheric iron fluxes over the last deglaciation: climatic implications. Geophys Res Lett 33:L03704 CrossRef
    19. Hong SM, Lee K, Hou SG, Hur SD, Ren JW, Burn LJ, Rosman KJR, Barbante C, Boutron CF (2009) An 800-year record of atmospheric As, Mo, Sn, and Sb in Central Asia in high-altitude ice cores from Mt. Qomolangma (Everest), Himalayas. Environ Sci Technol 43:8060鈥?065 CrossRef
    20. Hur SD, Cunde X, Hong S, Barbante C, Gabrielli P, Lee K, Boutron CF, Ming Y (2007) Seasonal patterns of heavy metal deposition to the snow on Lambert Glacier basin, East Antarctica. Atmos Environ 41:8567鈥?578 CrossRef
    21. Kang S, Zhang Q, Kaspari S, Qin D, Cong Z, Ren J, Mayewski PA (2007) Spatial and seasonal variations of elemental composition in Mt. Everest (Qomolangma) snow/firn. Atmos Environ 41:7208鈥?218 CrossRef
    22. Kang SC, Mayewski PA, Qin DH, Sneed SA, Ren JW, Zhang DQ (2004) Seasonal differences in snow chemistry from the vicinity of Mt. Everest, central Himalayas. Atmos Environ 38:2819鈥?829 CrossRef
    23. Kaspari S, Mayewski PA, Handley M, Kang S, Hou S, Sneed S, Maasch K, Qin D (2009a) A high-resolution record of atmospheric dust composition and variability since AD 1650 from a Mount Everest ice core. J Clim 22:3910鈥?925 CrossRef
    24. Kaspari S, Mayewski PA, Handley M, Osterberg E, Kang SC, Sneed S, Hou SG, Qin DH (2009b) Recent increases in atmospheric concentrations of Bi, U, Cs, S and Ca from a 350-year Mount Everest ice core record. J Geophys Res-Atmos 114:14 CrossRef
    25. Kaspari S, Schwikowski M, Gysel M, Flanner M, Kang S, Hou S, Mayewski P (2011) Recent increase in black carbon concentrations from a Mt. Everest ice core spanning 1860鈥?000 AD. Geophys Res Lett 38:L04703. doi:10.1029/2010GL046096 CrossRef
    26. Kawamura K, Izawa Y, Mochida M, Shiraiwa T (2012) Ice core records of biomass burning tracers (levoglucosan and dehydroabietic, vanillic and p-hydroxybenzoic acids) and total organic carbon for past 300聽years in the Kamchatka Peninsula, Northeast Asia. Geochim Cosmochim Acta 99:317鈥?29 CrossRef
    27. Koffman BG, Handley MJ, Osterberg EC, Wells ML, Kreutz KJ (2014) Dependence of ice-core relative trace-element concentration on acidification. J Glaciol 60:103 CrossRef
    28. Krachler M, Zheng J, Fisher D, Shotyk W (2009) Global atmospheric As and Bi contamination preserved in 3000聽year old Arctic ice. Glob Biogeochem Cycles 23:GB3011 CrossRef
    29. Lee K, Hur SD, Hou S, Hong S, Qin X, Ren J, Liu Y, Rosman KJR, Barbante C, Boutron CF (2008) Atmospheric pollution for trace elements in the remote high-altitude atmosphere in central Asia as recorded in snow from Mt. Qomolangma (Everest) of the Himalayas. Sci Total Environ 404:171鈥?81 CrossRef
    30. Li CL, Kang SC, Zhang QG (2009) Elemental composition of Tibetan Plateau top soils and its effect on evaluating atmospheric pollution transport. Environ Pollut 157:2261鈥?265 CrossRef
    31. Li M, Ma Y, Hirohiko I, Ma W, Sun F, Wang Y, Zhu Z (2007) Characteristics of micrometeorological elements near surface and soil on the northern slope of Mt. Qomolangma area. Plateau Meteorol 26:1263鈥?268 (In Chinese with English abstract)
    32. Liu Y, Hou S, Hong S, Do Hur S, Lee K, Wang Y (2011a) High-resolution trace element records of an ice core from the eastern Tien Shan, central Asia, since 1953聽AD. J Geophys Res 116:D12307. doi:10.1029/2010JD015191 CrossRef
    33. Liu Y, Hou S, Hong S, Hur SD, Lee K, Wang Y (2011b) Atmospheric pollution indicated by trace elements in snow from the northern slope of Cho Oyu range, Himalayas. Environ Earth Sci 63:311鈥?20 CrossRef
    34. Luck JM, Ben Othman D (2002) Trace element and Pb isotope variability during rainy events in the NW Mediterranean: constraints on anthropogenic and natural sources. Chem Geol 182:443鈥?60 CrossRef
    35. Ma Y, Wang Y, Zhong L, Wu R, Wang S, Li M (2011) The characteristics of atmospheric turbulence and radiation energy transfer and the structure of atmospheric boundary layer over the northern slope area of Himalaya. J Meteorol Soc Jpn 89A:345鈥?53 CrossRef
    36. Ming J, Cachier H, Xiao C, Qin D, Kang S, Hou S, Xu J (2008) Black carbon record based on a shallow Himalayan ice core and its climatic implications. Atmos Chem Phys 8:1343鈥?352 CrossRef
    37. Ningombam SS, Bagare S, Sinha N, Singh RB, Srivastava A, Larson E, Kanawade V (2014) Characterization of aerosol optical properties over the high-altitude station Hanle, in the trans-Himalayan region. Atmos Res 138:308鈥?23 CrossRef
    38. Ozsoy T, Ornektekin S (2009) Trace elements in urban and suburban rainfall, Mersin, northeastern Mediterranean. Atmos Res 94:203鈥?19 CrossRef
    39. Pacyna JM, Pacyna EG (2001) An assessment of global and regional emissions of trace metals to the atmosphere from anthropogenic sources worldwide. Environ Rev 9:269鈥?98 CrossRef
    40. Planchon FAM, Boutron CF, Barbante C, Cozzi G, Gaspari V, Wolff EW, Ferrari CP, Cescon P (2002) Changes in heavy metals in Antarctic snow from Coats Land since the mid-19th to the late-20th century. Earth Planet Sci Lett 200:207鈥?22 CrossRef
    41. Ramanathan V, Chung C, Kim D, Bettge T, Buja L, Kiehl JT, Washington WM, Fu Q, Sikka DR, Wild M (2005) Atmospheric brown clouds: impacts on South Asian climate and hydrological cycle. Proc Natl Acad Sci U S A 102:5326鈥?333 CrossRef
    42. Ruth U, Barbante C, Bigler M, Delmonte B, Fischer H, Gabrielli P, Gaspari V, Kaufmann P, Lambert F, Maggi V (2008) Proxies and measurement techniques for mineral dust in Antarctic ice cores. Environ Sci Technol 42:5675鈥?681 CrossRef
    43. Sakata M, Asakura K (2009) Factors contributing to seasonal variations in wet deposition fluxes of trace elements at sites along Japan Sea coast. Atmos Environ 43:3867鈥?875 CrossRef
    44. Stohl A (1998) Computation, accuracy and applications of trajectories鈥攁 review and bibliography. Atmos Environ 32:947鈥?66 CrossRef
    45. Wang XP, Xu BQ, Kang SC, Cong ZY, Yao TD (2008) The historical residue trends of DDT, hexachlorocyclohexanes and polycyclic aromatic hydrocarbons in an ice core from Mt. Everest, central Himalayas, China. Atmos Environ 42:6699鈥?709 CrossRef
    46. Weller R, W枚ltjen J, Piel C, Resenberg R, Wagenbach D, K枚Nig-Langlo G, Kriews M (2008) Seasonal variability of crustal and marine trace elements in the aerosol at Neumayer station, Antarctica. Tellus B 60:742鈥?52 CrossRef
    47. Wolff E, Hall J, Mulvaney R, Pasteur E, Wagenbach D, Legrand M (1998) Relationship between chemistry of air, fresh snow and firn cores for aerosol species in coastal Antarctica. J Geophys Res: Atmos (1984鈥?012) 103:11057鈥?1070 CrossRef
    48. Zhang N, Cao J, Liu S, Zhao Z, Xu H, Xiao S (2014) Chemical composition and sources of PM2.5 and TSP collected at Qinghai Lake during summertime. Atmos Res 138:213鈥?22 CrossRef
    49. Zhou J, Wang Y, Yue T, Li Y, Wai K-M, Wang W (2012) Origin and distribution of trace elements in high-elevation precipitation in southern China. Environ Sci Pollut Res 19:3389鈥?399 CrossRef
  • 刊物类别:Earth and Environmental Science
  • 刊物主题:Environment
    Environment
    Atmospheric Protection, Air Quality Control and Air Pollution
    Waste Water Technology, Water Pollution Control, Water Management and Aquatic Pollution
    Industrial Pollution Prevention
  • 出版者:Springer Berlin / Heidelberg
  • ISSN:1614-7499
文摘
Our research provides the first complete year-long dataset of wet deposition of trace elements in the high Himalayas based on a total of 42 wet deposition events on the northern slope of Mt. Qomolangma (Everest). Except for typical crustal elements (Al, Fe, and Mn), the concentration level of most trace elements (Sc, V, Cr, Co, Ni, Cu, Zn, As, Mo, Cd, Sn, Cs, Pb, Bi, and U) are generally comparable to those preserved in snow pits and ice cores from the nearby East Rongbuk Glacier. Cadmium was the element most affected by anthropogenic emissions. No pronounced seasonal variations are observed for most trace elements despite different transport pathways. In our study, the composition of wet precipitation reflects a regional background condition and is not clearly related to specific source regions. For the trace element record from ice cores and snow pits in the Himalayas, it could be deduced that the pronounced seasonal patterns were caused by the dry deposition of trace elements (aerosols) during their long exposure to the atmosphere after precipitation events. Our findings are of value for the understanding of the trace element deposition mechanisms in the Himalayas.

© 2004-2018 中国地质图书馆版权所有 京ICP备05064691号 京公网安备11010802017129号

地址:北京市海淀区学院路29号 邮编:100083

电话:办公室:(+86 10)66554848;文献借阅、咨询服务、科技查新:66554700