Effect of triethylamine treatment of titanium silicalite-1 on cyclohexanone ammoximation in a continuous system

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• 作者：Teng Zhang (1)
  Yaquan Wang (1)
  Shuhai Wang (1)
  Xiaoxue Wu (1)
  Pengxu Yao (1)
  Wenping Feng (1)
  Yi Lin (1)
  Juan Xu (1)
  
  1. Key Laboratory for Green Chemical Technology of the Ministry of Education ; School of Chemical Engineering & Technology ; Tianjin University ; Tianjin ; 300072 ; People鈥檚 Republic of China
  
• 关键词：TS ; 1 ; Hydrothermal treatment ; Triethylamine ; Hollow cavity ; Cyclohexanone ammoximation
• 刊名：Reaction Kinetics, Mechanisms and Catalysis
• 出版年：2015
• 出版时间：April 2015
• 年：2015
• 卷：114
• 期：2
• 页码：735-752
• 全文大小：564 KB
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• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Catalysis
  Industrial Chemistry and Chemical Engineering
  Physical Chemistry
  
• 出版者：Akad茅miai Kiad贸, co-published with Springer Science+Business Media B.V., Formerly Kluwer Academic
• ISSN：1878-5204

文摘

TS-1 has been hydrothermally treated by aqueous solutions of triethylamine, characterized by a number of techniques and studied in the ammoximation of cyclohexanone with NH3 and H2O2 in a continuous system. Some irregular hollow cavities are created after the treatment by desilication. The catalytic activities of TS-1 are not affected, but the catalyst stabilities significantly increase after the treatment, which can be attributed to the generation of the cavities. The treatment conditions are optimized, with the catalyst stability being extended to ten times of the conventional TS-1. After the treatment, triethylamine can be separated simply through distillation and recycled. The causes of deactivation are elucidated to be the deposition of higher weight byproducts formed on the surface of the catalysts and the deactivated TS-1 can be effectively regenerated through calcination in air.