Study of the histamine copper(II) chloride complex catalytic activity

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• 作者：I. Belfilali (1)
  S. Louhibi (1)
  R. Mahboub (2)
  R. Touzani (3)
  S. El Kadiri (3)
  T. Roisnel (4)
  
  1. Laboratory of Inorganic and Environment Chemistry ; University of Tlemcen ; B.P. 119 ; 13000 ; Tlemcen ; Algeria
  2. Department of Chemistry ; Faculty of Sciences ; University of Tlemcen ; B.P. 119 ; Tlemcen ; 13000 ; Algeria
  3. Laboratory of Applied Chemistry and Environment ; URAC18 ; University Mohamed 1st ; B.P. 524 ; 60000 ; Oujda ; Morocco
  4. Chemistry Sciences Laboratory of Rennes ; UMR 6226 CNRS ; University of Rennes 1 ; 35042 ; Rennes ; France
  
• 关键词：Histamine ; Copper(II) complex ; RX data ; Catecholase activity
• 刊名：Research on Chemical Intermediates
• 出版年：2015
• 出版时间：March 2015
• 年：2015
• 卷：41
• 期：3
• 页码：1819-1831
• 全文大小：798 KB
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• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Catalysis
  Physical Chemistry
  Inorganic Chemistry
  
• 出版者：Springer Netherlands
• ISSN：1568-5675

文摘

The histamine (His) copper(II) chloride complex Cu(His)Cl2 was synthesized. Its octahedral geometry was confirmed by spectroscopic and X-rays methods. The catalytic activities of the Cu(His)Cl2 complex and the in situ generated copper(II) complexes were evaluated in the oxidation of catechol to o-quinone under atmospheric oxygen. The oxidation rates depend on the nature of the ion salts. A kinetic study revealed that the Cu(His)Cl2 complex has the highest oxidation rate compared to the in situ-formed one.