Non-aqueous phase liquid-contaminated soil remediation by ex situ dielectric barrier discharge plasma
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- 作者：C. A. Aggelopoulos (1) (2)
C. D. Tsakiroglou (1)
S. Ognier (2)
S. Cavadias (2)
1. Institute of Chemical Engineering Sciences ; Foundation for Research and Technology Hellas ; Stadiou Str. ; Platani ; 26504 ; Patras-Rio ; Greece
2. Laboratoire de G茅nie des Proc茅d茅s Plasmas et Traitements de Surfaces - EA 3492 ; Universit茅 Pierre et Marie Curie 鈥?Ecole Nationale Sup茅rieure de Chimie de Paris ; Pierre & Marie Curie Str. ; 75231 ; Paris Cedex ; France - 关键词：Dielectric barrier discharge ; Non ; aqueous phase liquid removal efficiency ; Plasma oxidation ; Soil heterogeneity ; Soil remediation
- 刊名：International Journal of Environmental Science and Technology
- 出版年：2015
- 出版时间：March 2015
- 年：2015
- 卷：12
- 期：3
- 页码：1011-1020
- 全文大小：613 KB
- 参考文献：1. Adams JA, Reddy KR, Tekola L (2011) Remediation of chlorinated solvents plumes using in situ air sparging-A 2-D laboratory study. Int J Environ Res Public Health 8:2226鈥?239 CrossRef
2. Bai HY, Chen JR, Li XY, Zhang CH (2009) Non-thermal plasmas chemistry as a tool for environmental pollutants abatement. Rev Environ Contam Toxicol 201:117鈥?36
3. Barcelona MJ, Xie G (2001) In situ lifetimes and kinetics of a reductive whey barrier and an oxidative ORC barrier in the subsurface. Environ Sci Technol 35:3378鈥?385 CrossRef
4. Brusseau ML, Rohay V, Truex MJ (2010) Analysis of soil vapor extraction data to evaluate mass-transfer constraints and estimate source-zone mass flux. Ground Water Monit Remediat 30:57鈥?4 CrossRef
5. Cai XD, Du WT, Wu JY, Li RF, Guo Y, Yang ZJ (2012) Effective treatment of trichloroethylene-contaminated soil by hydrogen peroxide in soil slurries. Pedosphere 22:572鈥?79 CrossRef
6. Carroll KC, Oostrom M, Truex MJ, Rohay VJ, Brusseau ML (2012) Assessing performance and closure for soil vapor extraction: integrating vapor discharge and impact to groundwater quality. J Contam Hydrol 128:71鈥?2 CrossRef
7. Chang CL, Lin TS (2005) Decomposition of toluene and acetone in packed dielectric barrier discharge reactors. Plasma Chem Plasma Process 25:641鈥?57 CrossRef
8. Coates J (2000) Interpretation of infrared spectra, a practical approach. In: Meyers RA (ed) Encyclopedia of analytical chemistry. Wiley, Chichester, pp 10815鈥?0837
9. Devlin JF, Barker JF (1994) A semipassive nutrient injection scheme for enhanced in situ bioremediation. Ground Water 32:374鈥?80 CrossRef
10. Devlin JF, Katic D, Barker JF (2004) In situ sequenced bioremediation of mixed contaminants in groundwater. J Contam Hydrol 69:233鈥?61 CrossRef
11. Gierczak RFD, Devlin JF, Rudolph DL (2006) Combined use of field and laboratory testing to predict preferred flow paths in an heterogeneous aquifer. J Contam Hydrol 82:75鈥?8 CrossRef
12. Hao XL, Zhou MH, Lei LC (2007) Non-thermal plasma-induced photocatalytic degradation of 4-chlorophenol in water. J Hazard Mater 141:475鈥?82 CrossRef
13. Istok JD, Amonette JE, Coe CR, Fruchter JS, Humphrey MD, Szcsody JE, Teel SS, Vermeul VR, Williams MD, Yabusaki SB (1999) In situ redox manipulation by dithionite injection: intermediate-scale laboratory experiments. Ground Water 37:884鈥?89 CrossRef
14. Khan FI, Husain T, Hejazi R (2004) An overview and analysis of site remediation technologies. J Environ Manag 71:95鈥?22 CrossRef
15. Kim HH (2003) Plasma-driven catalyst processing packed with photocatalyst for gas-phase benzene decomposition. Catal Commun 4:347鈥?51 CrossRef
16. Kim HH, Ogata A, Futamura S (2005) Atmospheric plasma-driven catalysis for the low temperature decomposition of dilute aromatic compounds. J Phys D Appl Phys 38:1292鈥?299 CrossRef
17. Ko S, Crimi M, Marvin BK, Holmes V, Huling SG (2012) Comparative study on oxidative treatments of NAPL containing chlorinated ethanes and ethenes using hydrogen peroxide and persulfate in soils. J Environ Manag 108:42鈥?8 CrossRef
18. Lee BY, Park SH, Lee SC, Kang M, Choung SJ (2004) Decomposition of benzene by using a discharge plasma-photocatalyst hybrid system. Catal Today 93鈥?5:769鈥?76 CrossRef
19. Locke BR, Sato M, Sunka P, Hoffman MR (2006) Electrohydraulic discharge and nonthermal plasma for water treatment. Ind Eng Chem Res 45:882鈥?05 CrossRef
20. Lou J, Lu N, Li J, Wang T, Wu Y (2012) Remediation of chloramphenicol-contaminated soil by atmospheric pressure dielectric barrier discharge. Chem Eng J 180:99鈥?05 CrossRef
21. Masuda S (1988) Pulsed corona induced plasma chemical process: a horizon of new plasma chemical technologies. Pure Appl Chem 60:727鈥?31 CrossRef
22. Mok YS, Nam CM, Cho MH, Nam IS (2002) Decomposition of volatile organic compounds and nitric oxide by nonthermal plasma discharge processes. IEEE Trans Plasma Sci 30:408鈥?16 CrossRef
23. Nelson L, Barker J, Li T, Thomson N, Ioannidis M, Chatzis J (2009) A field trial to assess the performance of CO2-supersaturated water injection for residual volatile LNAPL recovery. J Contam Hydrol 109:82鈥?0 CrossRef
24. Ognier S, Iya-Sou D, Fourmond C, Cavadias S (2009) Analysis of mechanisms at the plasma-liquid interface in a gas-liquid discharge reactor used for treatment of polluted water. Plasma Chem Plasma Process 29:261鈥?73 CrossRef
25. Qu GZ, Lu N, Li J, Wu Y, Li GF, Li D (2009) Simultaneous pentachlorophenol decomposition and granular activated carbon regeneration assisted by dielectric barrier discharge plasma. J Hazard Mater 172:472鈥?78 CrossRef
26. Redolfi M, Aggadi N, Duten X, Touchard S, Pasquiers S, Hassouni K (2009) Oxidation of acetylene in atmospheric pressure pulsed corona discharge cell working in the nanosecond regime. Plasma Chem Plasma Process 29:173鈥?95 CrossRef
27. Redolfi M, Makhloufi C, Ognier S, Cavadias S (2010) Oxidation of kerosene components in a soil matrix by a dielectric barrier discharge reactor. Process Saf Environ Prot 88:207鈥?12 CrossRef
28. Schnarr M, Truax C, Farquhar G, Hood E, Gonullu T, Stickney B (1998) Laboratory and controlled field experiments using potassium permanganate to remediate trichloroethylene and perchloroethylene DNAPLs in porous media. J Contam Hydrol 29:205鈥?24 CrossRef
29. Sivachandiran L, Thevenet F, Gravejat P, Rousseau A (2013) Isopropanol saturated TiO2 surface regeneration by non-thermal plasma: influence of air relative humidity. Chem Eng J 214:17鈥?6 CrossRef
30. Switzer C, Pironi P, Gerhard JI, Rein G, Torero JL (2009) Self-sustaining smoldering combustion: a novel remediation process for non-aqueous-phase liquids in porous media. Environ Sci Technol 43:5871鈥?877 CrossRef
31. Triplett Kingston JL, Dahlen PR, Johnson PC (2010) State-of-the-practice review of in situ thermal technologies. Ground Water Monit Remediat 30:64鈥?2 CrossRef
32. Wang TC, Lu N, Li J, Wu Y (2010) Degradation of pentachlorophenol in soil by pulsed corona discharge plasma. J Hazard Mater 180:436鈥?41 CrossRef
33. Wang TC, Lu N, Li J, Wu Y (2011) Plasma-TiO2 catalytic method for high-efficiency remediation of p-Nitrophenol contaminated soil in pulsed corona. Environ Sci Technol 45:9301鈥?307 CrossRef
34. Zhang Y, Zheng J, Qu X, Yu W, Chen H (2008) Catalytic effect of activated carbon and activated carbon fiber in non-equilibrium plasma-based water treatment. Plasma Sci Technol 10:358鈥?62 CrossRef - 刊物主题：Environment, general; Environmental Science and Engineering; Environmental Chemistry; Waste Water Technology / Water Pollution Control / Water Management / Aquatic Pollution; Soil Science & Conservation; Ecotoxicology;
- 出版者：Springer Berlin Heidelberg
- ISSN：1735-2630
文摘
Non-thermal dielectric barrier discharge plasma is examined as a method for the ex situ remediation of non-aqueous phase liquid (NAPL)-contaminated soils. A mixture of equal mass concentrations (w/w) of n-decane, n-dodecane and n-hexadecane was used as model NAPL. Two soil types differing with respect to the degree of micro-heterogeneity were artificially polluted by NAPL: a homogeneous silicate sand and a moderately heterogeneous loamy sand. The effect of soil heterogeneity, NAPL concentration and energy density on soil remediation efficiency was investigated by treating NAPL-polluted samples for various treatment times and three NAPL concentrations. The concentration and composition of the residual NAPL in soil were determined with NAPL extraction in dichloromethane and GC-FID analysis, while new oxidized products were identified with attenuated total reflection Fourier transform infrared spectroscopy (ATR-FTIR). The experimental results indicated that the overall NAPL removal efficiency increases rapidly in early times reaching a plateau at late times, where NAPL is removed almost completely. The overall NAPL removal efficiency decreases with its concentration increasing and soil heterogeneity strengthening. The removal efficiency of each NAPL compound is inversely proportional to the number of carbon atoms and consistent with alkane volatility. A potential NAPL degradation mechanism is suggested by accounting for intermediates and final products as quantified by GC-FID and identified by ATR-FTIR.