Occurrence, sources, and ecological risks of PBDEs, PCBs, OCPs, and PAHs in surface sediments of the Yangtze River Delta city cluster, China

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• 作者：Ting Zhang (1) (2)
  Wen-Long Yang (3)
  She-Jun Chen (1)
  Dian-Long Shi (3)
  Hu Zhao (3)
  Yi Ding (4)
  Ye-Ru Huang (3)
  Nan Li (3)
  Yue Ren (3)
  Bi-Xian Mai (1)
  
• 关键词：PBDEs ; PCBs ; OCPs ; PAHs ; Sources ; Ecological risk
• 刊名：Environmental Monitoring and Assessment
• 出版年：2014
• 出版时间：August 2014
• 年：2014
• 卷：186
• 期：8
• 页码：5285-5295
• 全文大小：
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• 作者单位：Ting Zhang (1) (2)
  Wen-Long Yang (3)
  She-Jun Chen (1)
  Dian-Long Shi (3)
  Hu Zhao (3)
  Yi Ding (4)
  Ye-Ru Huang (3)
  Nan Li (3)
  Yue Ren (3)
  Bi-Xian Mai (1)
  
  1. State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou, 510640, China
  2. University of Chinese Academy of Sciences, Beijing, 100049, China
  3. State Environmental Protection Key Laboratory for Dioxin Pollution Control, National Research Center for Environmental Analysis and Measurement, Beijing, 100029, China
  4. College of Geosciences and Surveying Engineering, China University of Mining and Technology (Beijing), Beijing, 100083, China
  
• ISSN：1573-2959

文摘

Polybrominated diphenyl ethers (PBDEs), organochlorine pesticides (OCPs), polychlorinated biphenyls (PCBs), and polycyclic aromatic hydrocarbons (PAHs) in 25 surface sediments in three cities (Nantong, Wuxi, and Suzhou) in the Yangtze River Delta, eastern China were measured. The mean concentrations were 378, 45.8, 1.98, 4,002?ng/g for PBDEs, OCPs, PCBs, and PAHs, respectively. Their levels in the sediments in the three cities were generally consistent with the city industrialization. PBDEs and OCPs were markedly dominated by deca-BDE (>90?%) and DDTs (>70?%). A principle component analysis of the analytes identified three major factors suggesting different sources of the contaminants in the sediments. PBDEs and the organic carbon in the sediments have common sources from industrial activities; whereas OCPs and PCBs, correlated with the second factor, were mainly from historical sources. The third factor with loadings of PAHs is indicative of various combustion sources. Ecological risk assessment indicated that the potential highest risk is from DDTs, for which 22 sites exceed the effects range low (ERL) values and three sites exceed the effects range median (ERM) value.