Enhanced thermal and mechanical properties of epoxy composites by addition of hyperbranched polyglycerol grown on cellulose fibers

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• 作者：Xiane Xiao ; Shaorong Lu ; Lulu Pan ; Cen Zeng ; Zihai He…
• 关键词：Cellulose ; Hyperbranched polyglycerol ; Epoxy composites ; Thermal properties ; Mechanical properties
• 刊名：Journal of Polymer Research
• 出版年：2016
• 出版时间：April 2016
• 年：2016
• 卷：23
• 期：4
• 全文大小：997 KB
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• 作者单位：Xiane Xiao (1)
  Shaorong Lu (1)
  Lulu Pan (1)
  Cen Zeng (1)
  Zihai He (1)
  Jian Gao (1)
  Jinhong Yu (1) (2)
  
  1. Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, Ministry of Education, School of Material Science and Engineering, Guilin University of Technology, Guilin, 541004, China
  2. Key Laboratory of Marine Materials and Related Technologies, Zhejiang Key Laboratory of Marine Materials and Protective Technologies, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, 315201, China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Polymer Sciences
  Industrial Chemistry and Chemical Engineering
  Characterization and Evaluation Materials
  
• 出版者：Springer Netherlands
• ISSN：1572-8935

文摘

We reported a novel approach for epoxy composites by incorporation of hyperbranched polyglycerol (HPG) grafted sisal cellulose fibers (SCF). In this work, we have synthesized SCF wrapped HPG shell (SCF-g-HPG) by a “grafting from” strategy for the strong interfacial interaction between fillers and matrix. It was found that the thermal and mechanical properties of epoxy composites were greatly improved by incorporating SCF-g-HPG. For example, the impact strength, flexural strength, tensile strength, Young’s modulus and toughness of the composites with 3.0 wt% SCF-g-HPG loading were 38.35 KJ/m2, 123.40 MPa, 86.62 MPa, 151.7 MPa, and 417.84 MJ/m3, significantly increased by 119.1 %, 55.2 %, 45.6 %, 43.1 %, and 166.1 % respectively, as compared with neat epoxy. In addition, thermal stability of SCF-g-HPG/epoxy composites also showed an obvious enhancement compared with neat epoxy.