Compositional segregation, structural transformation and property-temperature relationship of high-Curie temperature Pb(In1/2Nb1/2)O3–Pb(Mg
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- 作者：Jianwei Chen ; Xiaobing Li ; Xiangyong Zhao…
- 刊名：Journal of Materials Science: Materials in Electronics
- 出版年：2015
- 出版时间：December 2015
- 年：2015
- 卷：26
- 期：12
- 页码：9316-9328
- 全文大小：5,076 KB
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47.B. Jaffe, R.S. Roth, S. Marzullo, J. Res - 作者单位：Jianwei Chen (1) (2)
Xiaobing Li (1)
Xiangyong Zhao (1)
Xi’an Wang (1)
Chao Chen (1) (2)
Hao Deng (1) (2)
Bo Ren (1)
Jie Jiao (1)
Haosu Luo (1)
1. Key Laboratory of Inorganic Functional Material and Device, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 201800, China
2. University of Chinese Academy of Sciences, Beijing, 100049, China - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Optical and Electronic Materials
Characterization and Evaluation Materials - 出版者：Springer New York
- ISSN：1573-482X
文摘
Ternary ferroelectric single crystal Pb(In1/2Nb1/2)O3–Pb(Mg1/3Nb2/3)O3–PbTiO3 (PIN–PMN–PT) was grown by the modified Bridgman method. The compositional variation of different regions of the crystals was measured, and the segregation regularity of the crystals was proposed. Variations in the dielectric properties and domain structures of the PIN–PMN–PT single crystals were investigated as a function of temperature and composition, and the phase transformation behavior of the crystals was observed. The PIN–PMN–PT crystals showed high Curie temperatures (T C = 160-10 °C), ferroelectric phase transition temperatures (T R-em class="EmphasisTypeItalic ">T up to 132 °C) and coercive fields (E C = 6- kV/cm) as well as excellent piezoelectric properties (d 33 up to 2,800 pC/N) and electromechanical coefficients (k 33 > 0.90). As the temperature increased, k 33 values remained relatively constant and d 33 increased gradually prior to ferroelectric phase transformation, and these results reflect the wide temperature usage range of PIN–PMN–PT single crystals. The polarization (P r ) and E C of the crystals showed unique trends during the phase transformation process; high P r and E C values can be maintained prior to depolarization, which indicates that the PIN–PMN–PT single crystals are candidate materials for high-power applications. In summary, PIN–PMN–PT single crystals with ultrahigh electric properties, large coercive fields and excellent thermal stability may potentially be applied in harsh environments.