Deposition of silver nanoparticles into silicon/carbon composite as a high-performance anode material for Li-ion batteries

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• 作者：Xianhua Hou ; Miao Zhang ; Jiyun Wang ; Shejun Hu…
• 关键词：Lithium ; ion batteries ; Anode ; Silicon ; Silver ; Amorphous carbon
• 刊名：Journal of Solid State Electrochemistry
• 出版年：2015
• 出版时间：December 2015
• 年：2015
• 卷：19
• 期：12
• 页码：3595-3604
• 全文大小：2,255 KB
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• 作者单位：Xianhua Hou (1) (2)
  Miao Zhang (1)
  Jiyun Wang (1)
  Shejun Hu (1) (2)
  Xiang Liu (3)
  
  1. Laboratory of Quantum Engineering and Quantum Materials, School of Physics and Telecommunication Engineering, South China Normal University, Guangzhou, 510006, China
  2. Engineering Research Center of Materials & Technology for Electrochemical Energy Storage (Ministry of Education), Guangzhou, 510006, China
  3. Institute of Advanced Materials, Nanjing University of Technology, Nanjing, 210009, China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Physical Chemistry
  Analytical Chemistry
  Industrial Chemistry and Chemical Engineering
  Characterization and Evaluation Materials
  Condensed Matter
  Electronic and Computer Engineering
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1433-0768

文摘

A silicon/silver/carbon (Si/Ag/C) composite with a core-core-shell structure has been synthesized via a simple method based on pyrolysis of an organic carbon source and silver mirror reaction. The Si and Ag nanoparticles are served as cores, while the porous amorphous carbon layer formed from pyrolysis of citric acid is served as shell. The porous amorphous carbon layer and highly conductive Ag nanoparticles can effectively alleviate the volume change of Si nanoparticles during lithiation/delithiation process and provide sufficient electrical conductivity for Si nanoparticles. As an anode material, the obtained Si/Ag/C composite exhibits excellent electrochemical performances, including high initial coulombic efficiency (85.6 % at 200 mA g?), stable cycling performance (a discharge capacity of 2006.3 mA g? at 200 mA g? after 100 cycles), and excellent rate performance (a discharge capacity of 826.4 mA h g? at 3 A g?). This simple method may open up an effective way to make other anode and cathode materials for commercial lithium-ion battery. Keywords Lithium-ion batteries Anode Silicon Silver Amorphous carbon