Polyacrylic acid sodium salt film entrapped Ag-nanocubes as molecule traps for SERS detection
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- 作者：Zhulin Huang ; Guowen Meng ; Qing Huang ; Bin Chen ; Fei Zhou ; Xiaoye Hu…
- 关键词：SERS ; Ag ; nanocube ; polyacrylic acid sodium salt ; trace detection
- 刊名：Nano Research
- 出版年：2014
- 出版时间：August 2014
- 年：2014
- 卷：7
- 期：8
- 页码：1177-1187
- 全文大小：2,155 KB
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Guowen Meng (1) (2)
Qing Huang (3)
Bin Chen (1)
Fei Zhou (1)
Xiaoye Hu (1)
Yiwu Qian (1)
Haibin Tang (1)
Fangming Han (1)
Zhaoqin Chu (1)
1. Key Laboratory of Materials Physics and Anhui Key Laboratory of Nanomaterials and Nanostructures, Institute of Solid State Physics, Chinese Academy of Sciences, P. O. Box 1129, Hefei, 230031, China
2. University of Science and Technology of China, Hefei, 230026, China
3. Key Laboratory of Ion Beam Bioengineering, Hefei Institutes of Physical Science, Chinese Academy of Sciences, Hefei, 230031, China - ISSN：1998-0000
文摘
Surface-enhanced Raman spectroscopy (SERS) is a fast analytical technique for trace chemicals; however, it requires the active SERS-substrates to adsorb analytes, thus limiting target species to those with the desired affinity for substrates. Here we present networked polyacrylic acid sodium salt (PAAS) film entrapped Ag-nanocubes (denoted as Ag-nanocubes@PAAS) as an effective SERS-substrate for analytes with and without high affinity. Once the analyte aqueous solution is cast on the dry Ag-nanocubes@PAAS substrate, the bibulous PAAS becomes swollen forcing the Ag-nanocubes loose, while the analytes diffuse in the interstices among the Ag-nanocubes. When dried, the PAAS shrinks and pulls the Ag-nanocubes back to their previous aggregated state, while the PAAS network “detains-the analytes in the small gaps between the Ag-nanocubes for SERS detection. The strategy has been proven effective for not only singleanalytes but also multi-analytes without strong affinity for Ag, showing its potential in SERS-based simultaneous multi-analyte detection of both adsorbable and non-adsorbable pollutants in the environment.