Chemical compositions of snow from Mt. Yulong, southeastern Tibetan Plateau

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• 作者：Hewen Niu ; Yuanqing He ; Shichang Kang ; Xixi Lu…
• 关键词：Atmospheric circulations ; major ions ; seasonal variations ; physical stratigraphy
• 刊名：Journal of Earth System Science
• 出版年：2016
• 出版时间：March 2016
• 年：2016
• 卷：125
• 期：2
• 页码：403-416
• 全文大小：2,165 KB
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• 作者单位：Hewen Niu (1) (2)
  Yuanqing He (1) (2)
  Shichang Kang (1) (3)
  Xixi Lu (4)
  Xiaoyi Shi (2)
  Shijin Wang (1)
  
  1. State Key Laboratory of Cryospheric Science, Cold and Arid Regions Environment and Engineering Research Institute, Chinese Academy of Sciences, Lanzhou, 730000, China
  2. Key Laboratory of Western China’s Environmental Systems (Ministry of Education), College of Earth and Environmental Sciences, Lanzhou University, Lanzhou, 730000, China
  3. CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing, 100101, China
  4. Department of Geography, National University of Singapore, 1 Arts Link, Singapore, 117570, Singapore
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：Earth sciences
  Geosciences
  Extraterrestrial Physics and Space Sciences
  
• 出版者：Springer India
• ISSN：0973-774X

文摘

The snow and ice in Mt. Yulong offer a unique opportunity to investigate changes in climate and large scale atmospheric circulations over Asia. During February and April 2012, surface snow samples were collected from the Baishui Glacier No. 1 at different altitudes along the eastern slope of Mt. Yulong. Two snowpits were also excavated from Mt. Yulong at altitudes of 4780 and 4730 m a.s.l. in February 2012. The concentrations of inorganic ions were higher at an elevation of 4506 m a.s.l. in the glacier with significant contribution of anthropogenic (mainly NH\(_{4}^{\mathrm {+}}\), SO\(_{4}^{\mathrm {2-}}\), NO\(_{3}^{\mathrm {-}})\) and crustal (mainly Ca 2+) constituents. Concentration of HCOO − in surface snow exhibited large variability, ranging from 0.04 to 6.8 μeq L −1, attributed to dominant contribution from biomass burning emissions. Ion balance (ΔC) and Na +/Cl − calculations indicated an excess of cations (particularly higher Ca 2+ concentrations) and Cl − in snow, considering the sea-salt ratio, respectively. Monsoon season (June–September) ion concentrations in snowpit samples were generally two-fold lower than in other seasons. Principal component analysis was used to identify different sources of ions. Three main factors, accounting for more than 80% of the total variance, were related to different sources, including agricultural activities, biomass burning, and crustal aerosols.