Chelant-Assisted Depollution of Metal-Contaminated Fe-Coated Sands and Subsequent Recovery of the Chemicals Using Solid-Phase Extraction Systems

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• 作者：Ismail M. M. Rahman (1) (2)
  Zinnat A. Begum (3)
  Hikaru Sawai (2)
  Masashi Ogino (2)
  Yoshiaki Furusho (4)
  Satoshi Mizutani (5)
  Hiroshi Hasegawa (6)
  
  1. Department of Applied and Environmental Chemistry ; Faculty of Science ; University of Chittagong ; Chittagong ; 4331 ; Bangladesh
  2. Graduate School of Natural Science and Technology ; Kanazawa University ; Kakuma ; Kanazawa ; 920-1192 ; Japan
  3. Department of Civil Engineering ; Southern University ; 739/A Mehedibag Road ; Chittagong ; 4000 ; Bangladesh
  4. GL Sciences Inc. ; Nishishinjuku 6-22-1 ; Shinjuku ; Tokyo ; 163-1130 ; Japan
  5. Graduate School of Engineering ; Osaka City University ; Sugimoto 3-3-138 ; Sumiyoshi-Ku ; Osaka ; 558-8585 ; Japan
  6. Institute of Science and Engineering ; Kanazawa University ; Kakuma ; Kanazawa ; 920-1192 ; Japan
  
• 关键词：Polymeric Fe ; modified sand ; Potentially toxic element (PTE) ; Wastewater treatment ; Sludge decontamination ; Chelant ; induced washing ; Solid ; Phase Extraction (SPE)
• 刊名：Water, Air, and Soil Pollution
• 出版年：2015
• 出版时间：March 2015
• 年：2015
• 卷：226
• 期：3
• 全文大小：797 KB
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• 刊物类别：Earth and Environmental Science
• 刊物主题：Environment
  Environment
  Atmospheric Protection, Air Quality Control and Air Pollution
  Waste Water Technology, Water Pollution Control, Water Management and Aquatic Pollution
  Terrestrial Pollution
  Hydrogeology
  
• 出版者：Springer Netherlands
• ISSN：1573-2932

文摘

The disposal of potentially toxic element (PTE)-loaded sludge that is produced during industrial or commercial wastewater treatments evoke concerns because of the probability of hazardous environmental consequences. In the current work, we proposed a chelant-assisted decontamination technique of the laboratory-produced PTE-loaded (As, Cd, Pb) polymeric-Fe-coated sludge and subsequent recovery of the chelants and PTEs. The chelant options include both biodegradable (EDDS, GLDA, and HIDS) and non-biodegradable (EDTA) alternatives. The washing performance was compared and discussed in terms of the solution pH and relative stabilities of the complexes of PTEs and chelants in solution. The changes in solution pH or chelants have no significant effect on the chelant-induced removal efficiency of Cd, and the same result was observed for Pb at extreme and moderate acidic pH. The As-extraction rate is also improved with chelant in the solution despite a limited interaction between the chelant and the arsenic species in the solution. The column-packed solid-phase extraction (SPE) system, which was equipped with macrocycle, chelating resin, or ion-exchange resin, was used to explore the corresponding separation performance of the PTEs and chelant. The macrocycle-equipped SPE system shows better selectivity than other SPEs in terms of extraction and recovery performance of the PTEs regardless of the chelants. Some unique points of the proposed process are minimum environmental burden due to the use of biodegradable materials in the washing solution and cost minimization by recycling the ingredients.