Mesoporous silica (KIT-6) derivatized with hydroxyquinoline functionalities as a selective adsorbent of uranium(VI)

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• 作者：Lu Zhu ; Xiangchen Shi ; Lijuan Song…
• 关键词：Mesoporous silica ; Surface modification ; Sorption ; Uranium(VI)
• 刊名：Journal of Radioanalytical and Nuclear Chemistry
• 出版年：2016
• 出版时间：May 2016
• 年：2016
• 卷：308
• 期：2
• 页码：381-392
• 全文大小：2,139 KB
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• 作者单位：Lu Zhu (1)
  Xiangchen Shi (1)
  Lijuan Song (1)
  Yalou Sun (1)
  Suwen Chen (1)
  Wangsuo Wu (1)
  
  1. School of Nuclear Science and Technology, Lanzhou University, Lanzhou, 730000, People’s Republic of China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Nuclear Chemistry
  Physical Chemistry
  Nuclear Physics, Heavy Ions and Hadrons
  Diagnostic Radiology
  Inorganic Chemistry
  
• 出版者：Akad茅miai Kiad贸, co-published with Springer Science+Business Media B.V., Formerly Kluwer Academic
• ISSN：1588-2780

文摘

Two modified mesoporous silica (KIT-6) materials for absorbing uranium(VI) were prepared respectively via post-grafting of 8-hydroxyquinoline and 8-hydroxyquinoline onto surface of KIT-6, which were characterized by FT-IR, NMR, TEM, and sorption/desorption analysis. Effect of pH values, contact time, ionic strength, solid–liquid ratio, temperature, and coexisting ions on sorption behavior of the modified KIT-6 were also investigated. Typical sorption isotherms (Langmuir and Freundlich) were used to determine the sorption process and the maximum U(VI) sorption capacity. The results indicate that the two modified KIT-6 exhibit better selective sorption of U(VI) as compared to the original KIT-6.