Multi-metals Measured at Sediment–Water Interface (SWI) by Diffusive Gradients in Thin Films (DGT) Technique for Geochemical Research

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• 作者：Zhihao Wu ; Lixin Jiao ; Shengrui Wang…
• 刊名：Archives of Environmental Contamination and Toxicology
• 出版年：2016
• 出版时间：February 2016
• 年：2016
• 卷：70
• 期：2
• 页码：429-437
• 全文大小：696 KB
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• 作者单位：Zhihao Wu (1) (2)
  Lixin Jiao (1)
  Shengrui Wang (1)
  Yuanzhi Xu (1)
  
  1. State Key Laboratory of Environmental Criteria and Risk Assessment, State Environmental Protection Key Laboratory for Lake Pollution Control, Research Center of Lake Eco-environment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, People’s Republic of China
  2. State Key Laboratory of Water Environment Simulation, School of Environment, Beijing Normal University, Beijing, 100875, People’s Republic of China
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：Environment
  Terrestrial Pollution
  Agriculture
  Ecology
  Forestry
  Environment
  Soil Science and Conservation
  
• 出版者：Springer New York
• ISSN：1432-0703

文摘

Diffusive gradients in thin films (DGT) technique was used to determine pore water profile and to assess remobilization character of metals at sediment/water interface. The remobilization of Mn was due to redox reaction in profile, which engendered two large peaks: one with DGT concentration of 1355 µg L−1 at depth of −4.75 cm in sediment and the other with DGT concentration of 1040 µg L−1 at depth of −3.25 cm in sediment pore water. Fe reduction zone had a large peak of Fe (3209 µg L−1) at depth of −4.75 cm in sediment. Fe DGT-profile also indicated the little peaks and low values of dissolved Fe concentration in Fe-reduction/S-reduction boundary zone in sediment. Detailed correspondence of trace metals with Fe or Mn features in DGT-profiles suggested that their release is related to the reductive dissolution of Fe- or Mn-oxide. Electronic supplementary materialThe online version of this article (doi:10.​1007/​s00244-015-0184-1) contains supplementary material, which is available to authorized users.