Wet-process preparation of nickel-based photoanode for TCO-less fiber-shaped dye-sensitized solar cells

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• 作者：Zuohua Liu (1)
  Haijian Feng (1)
  Xing Fan (1)
  Xiaoying Zhang (1)
  Jun Du (1)
  Guixin Cai (2)
  Changyuan Tao (1)
  
• 关键词：Wet ; process ; Nickel ; Fiber ; shaped DSSC ; Transparent conductive oxide
• 刊名：Journal of Solid State Electrochemistry
• 出版年：2014
• 出版时间：March 2014
• 年：2014
• 卷：18
• 期：3
• 页码：763-769
• 全文大小：815 KB
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• 作者单位：Zuohua Liu (1)
  Haijian Feng (1)
  Xing Fan (1)
  Xiaoying Zhang (1)
  Jun Du (1)
  Guixin Cai (2)
  Changyuan Tao (1)
  
  1. College of Chemistry and Chemical Engineering, Chongqing University, Chonqing, 400030, People鈥檚 Republic of China
  2. School of Chemistry and Chemical Engineering, Southwest University, Chongqing, 400715, People鈥檚 Republic of China
  
• ISSN：1433-0768

文摘

Low-cost ZnO-type fiber-shaped dye-sensitized solar cells (DSSC) without transparent conductive oxide (TCO) were for the first time assembled through a low-temperature all-wet process, using a series of Ni-based composite fiber. Both Ni layer morphology and ZnO nano-array structure evidently influenced the performance of the corresponding DSSC. For applications in both liquid type and all-solid CuI type fiber-shaped DSSCs, the Ni-based photoanode is comparable with the Ti- or Fe-based photoanode. Our all-solid CuI type fiber-shaped DSSCs was even better than that of the reported all-solid Ti- or Fe-based devices with the same oxide thickness. Electrochemical analysis further indicated that side reactions on the electrode/electrolyte interface could be effectively suppressed after a layer of Ni plated. Even for Cu wire, of which its interfacial side reactions are too complicated for application in DSSC, the Cu/Ni composite fiber still works well. Similar technology can be used to fabricate many other low-cost and light-weight conductive fibers, which are potential photoanode materials for highly efficient TCO-less DSSCs.