Lignite-derived mesoporous N- and O-enriched carbon sheet: a low-cost promising electrode for high-performance electrochemical capacitors
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- 作者：Siqi Zhu ; Qiuli Chen ; Yaoyao Shi ; Zhiyi Chen…
- 关键词：N ; and O ; enriched carbon sheet ; Hierarchical porosity ; Faradaic contribution ; Electrochemical capacitors
- 刊名：Journal of Solid State Electrochemistry
- 出版年：2016
- 出版时间：March 2016
- 年：2016
- 卷：20
- 期：3
- 页码：713-723
- 全文大小：1,718 KB
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Qiuli Chen (1)
Yaoyao Shi (1)
Zhiyi Chen (1)
Ruiqi Bao (1)
Lu Zhou (1)
Linrui Hou (1)
Kwun Nam Hui (2)
Changzhou Yuan (1) (2)
1. School of Materials Science & Engineering, Anhui University of Technology, Ma’anshan, 243002, Peoples Republic of China
2. Institute of Applied Physics and Materials Engineering, Faculty of Science and Technology, University of Macau, Macau, Peoples Republic of China - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Physical Chemistry
Analytical Chemistry
Industrial Chemistry and Chemical Engineering
Characterization and Evaluation Materials
Condensed Matter
Electronic and Computer Engineering - 出版者：Springer Berlin / Heidelberg
- ISSN：1433-0768
文摘
In the work, we successfully fabricate mesoporous N- and O-enriched carbon (NOC) with adjustable porosity and specific surface area (SSA) by using low-cost lignite as a precursor coupled with general KOH or ZnCl2 activation for electrochemical capacitors (ECs). Physicochemical and electrochemical characterizations reveal that chemical activating agents influence significantly upon the specific morphology, pore structure, and electrochemical performance of the resultant products. Strikingly, KOH-activated NOC (NOC-K) sheets are endowed with high SSA of ∼1257 m2 g−1, large pore volume of 1.3 cm3 g−1, and optimized pore size of ∼3 nm, rendering its electrochemical capacitance superior to those of NOC and ZnCl2-activated NOC (NOC-Z) in 6 M KOH. Thanks to its rich mesoporosity coupled with large electroactive SSA and heteroatom doping (N of ∼4.8 at.% and O of ∼23.3 at.%) effect, the NOC-K electrode yields even better electrochemical behaviors in 1 M H2SO4 than those in 6 M KOH.