Transformation and fragmentation behavior of molten metal drop in sodium pool

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• 作者：Satoshi Nishimura ; Zhi-Gang Zhang ; Ken-Ichiro Sugiyama ; Izumi Kinoshita
• 关键词：Copper ; Recycling ; Leaching ; Oxidation ; Chlorine
• 刊名：Nuclear Engineering and Design
• 出版年：2007
• 期刊代码：132_00295493
• 类别：et
• 出版时间：December 2007
• 卷：237
• 期：23
• 页码：2201-2209
• 文件大小：992 K

摘要

In order to clarify the fragmentation mechanism of a metallic alloy (U–Pu–Zr) fuel on liquid phase formed by metallurgical reactions (liquefaction temperature = 650 °C), which is important in evaluating the sequence of core disruptive accidents for metallic fuel fast reactors, a series of experiments was carried out using molten aluminum (melting point = 660 °C) and sodium mainly under the condition that the boiling of sodium does not occur. When the instantaneous contact interface temperature (T_i) between molten aluminum drop and sodium is lower than the boiling point of sodium (T_c,bp), the molten aluminum drop can be fragmented and the mass median diameter (D_m) of aluminum fragments becomes small with increasing T_i. When T_i is roughly equivalent to or higher than T_c,bp, the fragmentation of aluminum drop is promoted by thermal interaction caused by the boiling of sodium on the surface of the drop. Furthermore, even under the condition that the boiling of sodium does not occur and the solid crust is formed on the surface of the drop, it is confirmed from an analytical evaluation that the thermal fragmentation of molten aluminum drop with solid crust has a potential to be caused by the transient pressurization within the melt confined by the crust. These results indicate the possibility that the metallic alloy fuel on liquid phase formed by the metallurgical reactions can be fragmented without occurring the boiling of sodium on the surface of the melt.