呼和浩特市城区大气污染物浓度变化特征分析
详细信息    查看全文 | 推荐本文 |
  • 英文篇名:Variation characteristics of atmospheric pollutants in the urban area of Hohhot
  • 作者:邢雅婷 ; 王帅 ; 赵玲
  • 英文作者:XING Yating;WANG Shuai;ZHAO Ling;School of Ecology and Environment,Inner Mongolia University;
  • 关键词:大气污染物 ; 聚类分析 ; 气象因素 ; 呼和浩特市
  • 英文关键词:atmospheric pollutants;;cluster analysis;;meteorological factors;;Hohhot
  • 中文刊名:HJHX
  • 英文刊名:Environmental Chemistry
  • 机构:内蒙古大学生态与环境学院;
  • 出版日期:2019-04-23 16:14
  • 出版单位:环境化学
  • 年:2019
  • 期:v.38
  • 基金:内蒙古大学校级大学生创新创业训练计划项目(201817402);; 国家自然科学基金(21866022,21567018);; 内蒙古自然科学基金(2017MS0214)资助~~
  • 语种:中文;
  • 页:HJHX201905022
  • 页数:11
  • CN:05
  • ISSN:11-1844/X
  • 分类号:173-183
摘要
本文利用呼和浩特市8个国控监测点中CO、NO_2、SO_2、O_3、PM_(10)和PM_(2.5)逐时地面观测数据资料,采用聚类分析、相关性分析等方法,综合研究呼和浩特市城区大气污染物浓度时空变化特征.结果表明,2017年呼市PM_(10)、PM_(2.5)和O_3的污染较为严重,超标天数分别为49 d、52 d和41 d;CO和SO_2整体污染较轻.CO、NO_2、SO_2以及PM_(2.5)浓度表现出冬高夏低变化,O_3表现出夏高冬低变化,PM_(10)则表现为春冬高而夏秋低.O_3和NO_2均呈现单峰型日变化特征,且变化趋势相反;CO、SO_2和PM_(2.5)都呈现出相似的双峰型日变化.小召和工大金川校区监测点污染整体较为严重,小召监测点主要污染物为PM_(2.5)和PM_(10),工大金川校区主要污染物为SO_2.相关性分析表明,O_3浓度与气温呈显著正相关;PM_(2.5)与湿度呈显著正相关;CO、NO_2和SO_2均与风速呈显著负相关;PM_(10)与各气象要素在不同的季节相关性不同.
        Based on the data of CO, NO_2, SO_2, O_3, PM_(10) and PM_(2.5), the temporal and spatial variation of atmospheric pollutant concentration was studied in the urban area of Hohhot using cluster analysis and correlation analysis. The results showed that the pollution of PM_(10), PM_(2.5) and O_3 were much more serious in 2017, and the days of exceeding allowable limit were 49 d, 52 d and 41 d, respectively. Carbon monoxide and sulphur dioxide pollution were generally light. The concentrations of CO, NO_2, SO_2 and PM_(2.5) showed lower in winter and higher in summer. O_3 corcentration showed lower in summer and higher in winter. PM_(10) showed higher in spring and winter, and lower in summer and autumn. Both O_3 and NO_2 showed the single-peak daily change characteristics, and the trend was opposite. CO, SO_2 and PM_(2.5) all showed similar bipolar daily changes. Correlation analysis showed that O_3 concentration was positively correlated with temperature. PM_(2.5) was significantly positive correlation with humidity. CO, NO_2 and SO_2 all showed significantly negative correlation with wind speed. PM_(10) had different correlations with various meteorological factors in different seasons.
引文
[1] SONG C,WU L,XIE Y,et al.Air pollution in China:Status and spatiotemporal variations[J].Environmental Pollution,2017,227(1):334-347.
    [2] TAN Z F,LU K D,JIANG M Q,et al.Exploring ozone pollution in Chengdu,southwestern China:A case study from radical chemistry to O3-VOC-NOx sensitivity[J].Science of the T otal Environment,2018,636(15):775-786.
    [3] 严茹莎,李莉,安静宇,等.上海市夏季臭氧生成与其前体物控制模拟研究[J].环境污染与防治,2016,38(1):30-35.YAN R S,LI L,AN J Y,et al.Simulation study of ozone generation and its precursors control in Shanghai during summer time[J].Environmental Pollution & Control,2016,38(1):30-35(in Chinese).
    [4] SUN L,XUE L,WANG T,et al.Significant increase of summertime ozone at Mount Tai in Central Eastern China[J].Atmospheric Chemistry and Physics,2016,16(16):10637-10650.
    [5] 程麟钧,王帅,宫正宇,等.京津冀区域臭氧污染趋势及时空分布特征[J].中国环境监测,2017,33(1):14-21.CHENG L J,WANG S,GONG Z Y,et al.Pollution trends of ozone and its characteristics of temporal and spatial distribution in Beijing-Tianjin-Hebei region[J].Environmental Monitoring in China,2017,33(1):14-21(in Chinese).
    [6] TAO W,LI K X,BRIMBLECOMBE P,et al.Ozone pollution in China:A review of concentrations,meteorological influences,chemical precursors,and effects[J].Science of the Total Environment,2017,575(1):1582-1596.
    [7] XING Y F,XU Y H,SHI M H,et al.The impact of PM2.5 on the human respiratory system[J].Journal of Thoracic Disease,2016,8(1):69-74.
    [8] BROOK R D,RAJAGOPALAN S,POPE C A.Particulate matter air pollution and cardiovascular disease an update to the scientific statement from the american heart association[J].Circulation,2010,121(21):2331-2378.
    [9] 宋宇,唐孝炎,方晨,等.北京市能见度下降与颗粒物污染的关系[J].环境科学学报,2003,23(4):468-471.SONG Y,TANG X Y,FANG C,et all.Relationship between the visibility degradation and particle pollution in Beijing[J].Acta Scientiae Circumstantiae,2003,23(4):468-471(in Chinese).
    [10] 刀谞,张霖琳,王超,等.京津冀冬季与夏季PM2.5/PM10及其水溶性离子组分区域性污染特征分析[J].环境化学,2015,34(1):60-69.DAO X,ZHANG L L,WANG C,et all.Characteristics of mass and ionic compounds of atmospheric particles in winter and summer of Beijing-Tianjin-Hebei area,China[J].Environmental Chemistry,2015,34(1):60-69(in Chinese).
    [11] 赵阳,林晓辉,胡恭任,等.南昌市秋季PM2.5中多环芳烃的污染特征、风险评价及来源分析[J].环境化学,2016,35(3):500-507.ZHAO Y,LIN X H,HU G R,et all.Pollution characteristics,risk assessment and source analysis of polycyclic aromatic hydrocarbons in PM2.5 collected in autumn in Nanchang City[J].Environmental Chemistry,2016,35(3):500-507(in Chinese).
    [12] 徐鹏,郝庆菊,吉东生,等.重庆市北碚城区大气污染物浓度变化特征观测研究[J].环境科学,2014,35(3):820-829.Xu P,Hao Q J,Ji D S,et al.Observation of atmospheric pollutants in the urban area of Beibei District,Chongqing[J].Environmental Science,2014,35(3):820-829(in Chinese).
    [13] 耿红,宣莹莹,蔡夏童,等.太原市2014年春节期间常规大气污染物浓度变化及聚类分析[J].环境科学学报,2015,35(4):965-974.GENG H,XUAN Y Y,CAI X T,et al.Mass concentration variation and cluster analysis of urban air pollutants in Taiyuan,Shanxi Province during Chinese New Year of 2014[J].Acta Scientiae Circumstantiae,2015,35(4):965-974(in Chinese).
    [14] 谢雨竹,潘月鹏,倪长健,等.成都市区夏季大气污染物浓度时空变化特征分析[J].环境科学学报,2015,35(4):975-983.XIE Y Z,PAN Y P,NI C J,et al.Temporal and spatial variations of atmospheric pollutants in urban Chengdu during summer[J].Acta Scientiae Circumstantiae,2015,35(4):975-983(in Chinese).
    [15] 智颖,李婧.呼和浩特市空气颗粒物影响因素研究[J].中国环境监测,2014,30(3):26-30.ZHI Y,LI J.The influence factors research of Hohhot air particulate matter[J].Environmental Monitoring in China,2014,30(3):26-30(in Chinese).
    [16] 周海军,杜远江,都达古拉,等.呼和浩特市冬季PM10中多环芳烃的污染特征及来源解析[J].环境化学,2016,35(8):1707-1714.ZHOU H J,DU Y J,DU D G L,et al.Characterization and source apportionment of polycyclic aromatic hydrocarbons bound to PM10 during winter in Hohhot[J].Environmental Chemistry,2016,35(8):1707-1714(in Chinese).
    [17] 张存厚,李福胜,朝鲁门,等.呼和浩特市空气质量状况及与气象因子的相关性分析[J].干旱区资源与环境,2018,32(2):87-93.ZHANG C H,LI F S,ZHAO L M,et all.Correlations between air quality status and meteorological factors in Hohhot City[J].Journal of Arid Land Resources and Environment,2018,32(2):87-93(in Chinese).
    [18] 薛敏,王跃思,孙扬,等.北京市大气中CO的浓度变化监测分析[J].环境科学,2006,27(2):200-206.XUE M,WANG S Y,SUN Y,et al.Measurement on the atmospheric CO Concentration in Beijing[J].Environmental Science,2006,27(2):200-206(in Chinese).
    [19] 凌宏,王迎红,胡波,等.2007年夏季北京大气CO检测分析[J].环境化学,2009,28(4):567-570.LING H,WANG Y H,HU B,et al.Observation and research on carbon monoxide in the atmosphere of Beijing during the summer time of 2007[J].Environmental Chemistry,2009,28(4):567-570(in Chinese).
    [20] 周春艳,王桥,厉青,等.近10年长江三角洲对流层NO2柱浓度时空变化及影响因素[J].中国环境科学,2016,36(7):1921-1930.ZHOU C Y,WANG Q,LI Q,et al.Spatio-temporal change and influencing factors of tropospheric NO2 column density of Yangtze River Delta in the decade[J].China Environmental Science,2016,36(7):1921-1930(in Chinese).
    [21] 赵辉,郑有飞,徐静馨,等.乌鲁木齐市大气污染物浓度的变化特征[J].环境化学,2015,34(11):2118-2126.ZHAO H,ZHENG Y F,XU J Q,et al.Variation characteristics of air pollutant concentrations in Urumqi[J].Environmental Chemistry,2015,34(11):2118-2126(in Chinese).
    [22] 郑晓霞,李令军,赵文吉,等.京津冀地区大气NO2污染特征研究[J].生态环境学报,2014,23(12):1938-1945.ZHENG X X,LI L J,ZHAO W J,et al.Spatial and temporal characteristics of atmospheric NO2 in the Beijing-Tianjin-Hebei Region[J].Ecology and Environmental Sciences,2014,23(12):1938-1945(in Chinese).
    [23] 贺鹏,张先明.中国燃煤发电厂烟气脱硫技术及应用[J].电力科技与环保,2014,30(1):8-11.Flue gas desulphurization technology and its application in coal-fired power generation of China[J].Electric Power Technology and Environmental Protection,2014,30(1):8-11(in Chinese).
    [24] 王占山,李云婷,陈添,等.北京城区臭氧日变化特征及与前体物的相关性分析[J].中国环境科学,2014,34(12):3001-3008.WANG Z S,LI X T,CHEN T,et al.Analysis on diurnal variation characteristics of ozone and correlations with its precursors in urban atmosphere of Beijing[J].China Environmental Science,2014,34(12):3001-3008(in Chinese).
    [25] 司瑶冰,宫春宁,郑有飞.呼和浩特市大气污染与天气气候的关系[J].气象科技,2005,33(2):173-177.SI Y B,GONG C N,ZHENG Y F.Correlation between air pollution density and climate in Hohhot[J].Meteorological Science and Technology,2005,33(2):173-177(in Chinese).
    [26] Pui D Y H,Chen S C,Zuo Z L.PM2.5 in China:Measurements,sources,visibility and health effects,and mitigation[J].Particuology,2014,13(2):1-26.
    [27] 姜新华,薛河儒,张存厚,等.基于主成分分析的呼和浩特市空气质量影响因素研究[J].安全与环境工程,2016,23(1):75-79.JIANG X H,XUE H R,ZHANG C H,et al.Research on the influencing factors of air quality in Hohhot City based on principal component analysis[J].Safety and Environmental Engineering,2016,23(1):75-79(in Chinese).
    [28] 赵晨曦,王云琦,王玉杰,等.北京地区冬春PM2.5和PM10污染水平时空分布及其与气象条件的关系[J].环境科学,2014,35(2):418-427.ZHAO C X,WANG Y Q,WANG Y J,et al.Temporal and spatial distribution of PM2.5 and PM10 pollution status and the correlation of particulate matters and meteorological factors during Winter and Spring in Beijing[J].Environmental Science,2014,35(2):418-427(in Chinese).
    [29] ATKINSON R.Atmospheric chemistry of VOCs and NOx[J].Atmospheric Environment,2000,34(12-14):2063-2101.
    [30] 王莉莉,王跃思,吉东生,等.天津滨海新区秋冬季大气污染特征分析[J].中国环境科学,2011,31(7):1077-1086.WANG L L,WANG Y S,JI D S,et al.Characteristics of atmospheric pollutants in Tianjin Binhai New Area during autumn and winter[J].China Environmental Science,2011,31(7):1077-1086(in Chinese).
    [31] 安俊琳,王跃思,李昕,等.北京大气中NO、NO2和O3浓度变化的相关性分析[J].环境科学,2007,28(4):4706-4711.AN J L,WANG Y S,LI X,et al.Analysis of the relationship between NO,NO2 and O3 concentrations in Beijing[J].Environmental Science,2007,28(4):4706-4711(in Chinese).
    [32] LOUIE P K K,WATSON J G,CHOW J C,et al.Seasonal characteristics and regional transport of PM2.5 in Hong Kong[J].Atmospheric Environment,2005,39(9):1695-1710.
    [33] LIU Z,HU B,WANG L L,et al.Seasonal and diurnal variation in particulate matter (PM10 and PM2.5) at an urban site of Beijing:analyses from a 9-year study [J].Environmental Science and Pollution Research,2015,22(1):627-642.
    [34] CABALLERO S,ESCLAPEZ R,GALINDO N,et al.Use of a passive sampling network for the determination of urban NO2 spatiotemporal variations [J].Atmospheric Environment,2012,63(1):148-155.
    [35] GOMISCEK B,HAUCK H,STOPPER S,et al.Spatial and temporal variations of PM1,PM2.5,PM10 and particle number concentration during the AUPHEP-project[J].Atmospheric Environment,2004,38(24):3917-3934.
    [36] 李军,孙春宝,刘咸德,等.气象因素对北京市大气颗粒物浓度影响的非参数分析[J].环境科学研究,2009,22(6):663-669.LI J,SUN C B,LIU X D,et al.Non-parameter statistical analysis of impacts of meteorological conditions on PM concentration in Beijing[J].Research of Environmental Sciences,2009,22(6):663-669(in Chinese).
    [37] 王闯,王帅,杨碧波,等.气象条件对沈阳市环境空气臭氧浓度影响研究[J].中国环境监测,2015,31(3):32-37.WANG C,WANG S,YANG B B,et al.Study of the effect of meteorological conditions on the ambient air ozone concentrations in Shenyang[J].Environmental Monitoring in China,2015,31(3):32-37(in Chinese).
    [38] ZHANG H L,WANG Y G,HU J L,et al.Relationships between meteorological parameters and criteria air pollutants in three megacities in China[J].Environmental Research,2015,140(1):242-254.
    [39] HE J J,GONG S L,YU Y,et al.Air pollution characteristics and their relation to meteorological conditions during 2014-2015 in major Chinese cities[J].Environmental Pollution,2017,223(1):484-496.
    [40] HERMAN J R,BHARTIA P K,TORRES O,et al.Global distribution of UV-absorbing aerosols from Nimbus 7/TOMS data[J].Journal of Geophysical Research:Atmospheres,1997,102(D14):16911-16922.
    [41] DICKERSON R R,KONDRAGUNTA S,STENCHIKOV G,et al.The impact of aerosols on solar ultraviolet radiation and photochemical smog[J].Science,1997,278(5339):827-830.

© 2004-2018 中国地质图书馆版权所有 京ICP备05064691号 京公网安备11010802017129号

地址:北京市海淀区学院路29号 邮编:100083

电话:办公室:(+86 10)66554848;文献借阅、咨询服务、科技查新:66554700