介质阻挡等离子体制备臭氧研究进展
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摘要
从电极布置与形式、原料气体、电介质及填料3个方面阐述了国内外介质阻挡放电(DBD)等离子体产生臭氧的研究进展,分析了各因素对臭氧产生的影响,指出合理布置电极,同时充分利用催化剂填料与等离子体的协同作用,可提高氧气的转化率、臭氧浓度和能量效率。
The research progresses on production of ozone by dielectric barrier discharge(DBD) plasma at home and abroad are introduced from three aspects such as forms and arrangements of electrodes,feed gases,and dielectric barriers and packed materials.The effects of various factors on the generation of ozone are analyzed. It is indicated that arranging electrodes reasonably and making full use of the synergistic effects of catalysts and packing materials with plasma can increase the conversion rate of oxygen,the ozone concentration and the energy efficiency.
The research progresses on production of ozone by dielectric barrier discharge(DBD) plasma at home and abroad are introduced from three aspects such as forms and arrangements of electrodes,feed gases,and dielectric barriers and packed materials.The effects of various factors on the generation of ozone are analyzed. It is indicated that arranging electrodes reasonably and making full use of the synergistic effects of catalysts and packing materials with plasma can increase the conversion rate of oxygen,the ozone concentration and the energy efficiency.
引文
[1]杨春,胡兆吉,魏林生.放电等离子体臭氧发生技术研究现状与进展[J].高压电器,2010,46(9):78-85.
[2]商克峰,曹晓萌,王肖静,等.高压电极构型对DBD装置放电特性及臭氧生成的影响[J].高电压技术,2016,42(5):1394-1400.
[3]Andreev V V,Pichugin Y P,Telegin V G,et al.Combined barrier discharge in atmospheric-pressure air[J].Plasma Physics Reports,2012,38(13):1046-1049.
[4]Chebbah A,Hadjeri S,Nemmich S,et al.Development and experimental analysis of a new“serpentine-shape”surface-DBD ozone generator-comparison with a cylindrical volume-DBD ozone generator[J].Ozone Science&Engineering,2017,39(3):209-216.
[5]Pekrek S.Asymmetric properties and ozone production of surface dielectric barrier discharge with different electrode configurations[J].The European Physical Journal D,2013,67(5):1-7.
[6]Malik A M,Schoenbach K H,Heller R.Coupled surface dielectric barrier discharge reactor-ozone synthesis and nitric oxide conversion from air[J].Chemical Engineering Journal,2014,256(256):222-229.
[7]Nassour K,Brahami M,Nemmich S,et al.New hybrid surfacevolume dielectric barrier discharge reactor for ozone generation[J].IEEE Transactions on Industry Applications,2017,53(13):2477-2484.
[8]Jodpimai S,Boonduang S,Limsuwan P.Dielectric barrier discharge ozone generator using aluminum granules electrodes[J].Journal of Electrostatics,2015,74:108-114.
[9]Gnapowski S,Yamabe C,Ihara S.Ozone generation characteristics of ozonizer with the rotating type electrode[J].IEEJ Transactions on Fundamentals&Materials,2008,128(10):619-623.
[10]Fujishima T,Kawaguchii T,Amano T,et al.Ozone generation properties of screw-type electrode ozonizer by divided outer electrodes[C]//3rd International Conference on Electric and Electronics,2013:311-314.
[11]Chen H L,Lee H M,Chen S H,et al.Influence of Ar addition on ozone generation in nonthermal plasmas[J].Plasma Sources Science&Technology,2010,19(6):692-701.
[12]魏林生.等离子体臭氧产生的实验与理论研究[D].杭州:浙江大学,2008.
[13]Wei L S,Yuan D K,Zhang Y F,et al.The effect of inert gases on ozone generation using dielectric barrier discharge in dry air[J].Ozone Science&Engineering,2013,35(6):448-455.
[14]Zhang X M,Lee B J,Hong G I,et al.Ozone production with dielectric barrier discharge:Effects of power source and humidity[J].IEEE Transactions on Plasma Science,2016,44(10):2288-2296.
[15]Wei L S,Dong G P,Zhang Y F,et al.Effect of SF6on ozone generation using dielectric barrier discharge[J].High Voltage Engineering,2013,39(10):2520-2525.
[16]Osawa N,Tsuji T,Ogiso R,et al.Effect of nitrogen addition to ozone generation characteristics by diffuse and filamentary dielectric barrier discharges at atmospheric pressure[J].European Physical Journal Applied Physics,2017,78(2):20804.
[17]Zosimov A V,Lunin V V,Samoilovich V G,et al.Nonstationary effects in ozone generation by barrier discharges in N2/O2mixtures[J].Russian Journal of Physical Chemistry A,2016,90(8):1687-1692.
[18]Wei L S,Yuan D K,Zhang Y F,et al.An analysis of the effect of inert gases on ozone generation using dielectric barrier discharge in oxygen[J].The European Physical Journal D,2014,68(1):1-7.
[19]Naovaratpong S,Boonyaroonate I,Nathakaranakule A.Plasma density control in a dielectric barrier discharge(DBD)ozone generator using a laser engraved dielectric layer and alumina sand filled discharge channel[J].Lasers in Engineering,2014,28:189-200.
[20]周立福,杨学昌,陈波,等.臭氧发生器用高介电硅橡胶复合材料特性及试验分析[J].高电压技术,2010,36(5):1258-1263.
[21]陈波,杨学昌,陶顺忠.等离子喷涂介质层提升臭氧发生器性能的试验研究[J].高电压技术,2013,(7):1703-1709.
[22]Dwivedi C,Toley M A,Dey G R,et al.Ozone generation from argonoxygen mixtures in presence of different packing materials within dielectric barrier discharge gap[J].Ozone Science&Engineering,2013,35(2):134-145.
[23]Huang W D,Ren T T,Xia W D.Ozone generation by hybrid discharge combined with catalysis[J].Ozone Science&Engineering,2007,29(2):107-112.
[24]王健.催化剂耦合介质阻挡放电制取臭氧的试验和模型研究[D].合肥:中国科学技术大学,2009.
[25]Pekrek S.Experimental study of surface dielectric barrier discharge in air and its ozone production[J].Journal of Physics D Applied Physics,2012,45(7):075201.
[26]Pekrek S,Mike2 J,BeshajovPeliknov I,et al.Effect of Ti O2on various regions of active electrode on surface dielectric barrier discharge in air[J].Plasma Chemistry&Plasma Processing,2016,36(5):1187-1200.
[27]Pekrek S,Mike2 J,Krsa J.Comparative study of Ti O2and Zn O photocatalysts for the enhancement of ozone generation by surface dielectric barrier discharge in air[J].Applied Catalysis A General,2015,502:122-128.
[2]商克峰,曹晓萌,王肖静,等.高压电极构型对DBD装置放电特性及臭氧生成的影响[J].高电压技术,2016,42(5):1394-1400.
[3]Andreev V V,Pichugin Y P,Telegin V G,et al.Combined barrier discharge in atmospheric-pressure air[J].Plasma Physics Reports,2012,38(13):1046-1049.
[4]Chebbah A,Hadjeri S,Nemmich S,et al.Development and experimental analysis of a new“serpentine-shape”surface-DBD ozone generator-comparison with a cylindrical volume-DBD ozone generator[J].Ozone Science&Engineering,2017,39(3):209-216.
[5]Pekrek S.Asymmetric properties and ozone production of surface dielectric barrier discharge with different electrode configurations[J].The European Physical Journal D,2013,67(5):1-7.
[6]Malik A M,Schoenbach K H,Heller R.Coupled surface dielectric barrier discharge reactor-ozone synthesis and nitric oxide conversion from air[J].Chemical Engineering Journal,2014,256(256):222-229.
[7]Nassour K,Brahami M,Nemmich S,et al.New hybrid surfacevolume dielectric barrier discharge reactor for ozone generation[J].IEEE Transactions on Industry Applications,2017,53(13):2477-2484.
[8]Jodpimai S,Boonduang S,Limsuwan P.Dielectric barrier discharge ozone generator using aluminum granules electrodes[J].Journal of Electrostatics,2015,74:108-114.
[9]Gnapowski S,Yamabe C,Ihara S.Ozone generation characteristics of ozonizer with the rotating type electrode[J].IEEJ Transactions on Fundamentals&Materials,2008,128(10):619-623.
[10]Fujishima T,Kawaguchii T,Amano T,et al.Ozone generation properties of screw-type electrode ozonizer by divided outer electrodes[C]//3rd International Conference on Electric and Electronics,2013:311-314.
[11]Chen H L,Lee H M,Chen S H,et al.Influence of Ar addition on ozone generation in nonthermal plasmas[J].Plasma Sources Science&Technology,2010,19(6):692-701.
[12]魏林生.等离子体臭氧产生的实验与理论研究[D].杭州:浙江大学,2008.
[13]Wei L S,Yuan D K,Zhang Y F,et al.The effect of inert gases on ozone generation using dielectric barrier discharge in dry air[J].Ozone Science&Engineering,2013,35(6):448-455.
[14]Zhang X M,Lee B J,Hong G I,et al.Ozone production with dielectric barrier discharge:Effects of power source and humidity[J].IEEE Transactions on Plasma Science,2016,44(10):2288-2296.
[15]Wei L S,Dong G P,Zhang Y F,et al.Effect of SF6on ozone generation using dielectric barrier discharge[J].High Voltage Engineering,2013,39(10):2520-2525.
[16]Osawa N,Tsuji T,Ogiso R,et al.Effect of nitrogen addition to ozone generation characteristics by diffuse and filamentary dielectric barrier discharges at atmospheric pressure[J].European Physical Journal Applied Physics,2017,78(2):20804.
[17]Zosimov A V,Lunin V V,Samoilovich V G,et al.Nonstationary effects in ozone generation by barrier discharges in N2/O2mixtures[J].Russian Journal of Physical Chemistry A,2016,90(8):1687-1692.
[18]Wei L S,Yuan D K,Zhang Y F,et al.An analysis of the effect of inert gases on ozone generation using dielectric barrier discharge in oxygen[J].The European Physical Journal D,2014,68(1):1-7.
[19]Naovaratpong S,Boonyaroonate I,Nathakaranakule A.Plasma density control in a dielectric barrier discharge(DBD)ozone generator using a laser engraved dielectric layer and alumina sand filled discharge channel[J].Lasers in Engineering,2014,28:189-200.
[20]周立福,杨学昌,陈波,等.臭氧发生器用高介电硅橡胶复合材料特性及试验分析[J].高电压技术,2010,36(5):1258-1263.
[21]陈波,杨学昌,陶顺忠.等离子喷涂介质层提升臭氧发生器性能的试验研究[J].高电压技术,2013,(7):1703-1709.
[22]Dwivedi C,Toley M A,Dey G R,et al.Ozone generation from argonoxygen mixtures in presence of different packing materials within dielectric barrier discharge gap[J].Ozone Science&Engineering,2013,35(2):134-145.
[23]Huang W D,Ren T T,Xia W D.Ozone generation by hybrid discharge combined with catalysis[J].Ozone Science&Engineering,2007,29(2):107-112.
[24]王健.催化剂耦合介质阻挡放电制取臭氧的试验和模型研究[D].合肥:中国科学技术大学,2009.
[25]Pekrek S.Experimental study of surface dielectric barrier discharge in air and its ozone production[J].Journal of Physics D Applied Physics,2012,45(7):075201.
[26]Pekrek S,Mike2 J,BeshajovPeliknov I,et al.Effect of Ti O2on various regions of active electrode on surface dielectric barrier discharge in air[J].Plasma Chemistry&Plasma Processing,2016,36(5):1187-1200.
[27]Pekrek S,Mike2 J,Krsa J.Comparative study of Ti O2and Zn O photocatalysts for the enhancement of ozone generation by surface dielectric barrier discharge in air[J].Applied Catalysis A General,2015,502:122-128.