臭氧氧化技术在水处理中的应用进展
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摘要
臭氧氧化技术在水处理领域逐渐得到了广泛应用。介绍了臭氧的物理化学性质、单独臭氧氧化技术、催化臭氧氧化技术及其组合工艺技术,总结了各类催化臭氧氧化技术的催化剂和反应机理的研究进展,并展望了臭氧氧化技术在水处理方向的发展前景。
Ozone oxidation technology has been widely applied in wastewater treatment field.The physiochemical properties of ozone,single ozone oxidation,catalytic ozone oxidation,and combined technology thereof were briefly introduced,the research progress of catalysts and reaction mechanism of various catalytic ozone oxidation technologies were summarized,and the application directions and prospects of ozone oxidation in water treatment field were forecasted.
Ozone oxidation technology has been widely applied in wastewater treatment field.The physiochemical properties of ozone,single ozone oxidation,catalytic ozone oxidation,and combined technology thereof were briefly introduced,the research progress of catalysts and reaction mechanism of various catalytic ozone oxidation technologies were summarized,and the application directions and prospects of ozone oxidation in water treatment field were forecasted.
引文
[1]黄磊,唐琪玮,黄思远,等.臭氧氧化技术及其在水处理领域的发展[J].净水技术,2018,37(s1):106-112.
[2]黄程兰,刘敏,陈滢.臭氧在污水处理中的应用[J].四川化工,2012,15(1):25-27.
[3]KASPRZYK-HORDERN B,ZI魷LEK M,NAWROCKI J.Catalytic ozonation and methods of enhancing molecular ozone reactions in water treatment[J].Applied Catalysis B:Environmental,2003,46(4):639-669.
[4]迟婷.臭氧氧化技术对各种染料处理效果及机理的研究[D]青岛:青岛科技大学,2015.
[5]PIERA E,CALPE J C,BRILLAS E,et al.2,4-Dichlorophenox yacetic acid degradation by catalyzed ozonation:TiO2/UVA/O3and Fe(Ⅱ)/UVA/O3systems[J].Applied Catalysis B:Environmental,2000,27(3):169-177.
[6]TANAKA K,ABE K,SHENG C Y,et al.Photocatalytic waste water treatment combined with ozone pretreatment[J].Environmen tal Science&Technology,1992,26(12):2534-2536.
[7]PINES D S,RECKHOW D A.Effect of dissolved cobalt(Ⅱ)on the ozonation of oxalic acid[J].Environmental Science&Technology,2002,36(19):4046-4051.
[8]黄深.城市污水厂二级处理出水臭氧深度处理研究[D].北京:清华大学,2008.
[9]LEGUBE B,KARPEL VEL LEITNER N.Catalytic ozonation:a promising advanced oxidation technology for water treatment[J].Catalysis Today,1999,53(1):61-72.
[10]GRACIA R,ARAG譈ES J L,OVELLEIRO J L.Study of the catalytic ozonation of humic substances in water and their ozonation byproducts[J].Ozone:Science&Engineering,1996,18(3):195-208.
[11]押玉荣,陈金杰,韩墨菲,等.Mn-Al2O3催化臭氧氧化处理工业废水试验研究[J].工业用水与废水,2018,49(5):27-30.
[12]洪浩峰,潘湛昌,徐阁,等.活性炭负载催化剂臭氧催化氧化处理印染废水研究[J].工业用水与废水,2010,41(3):29-33.
[13]GHUGE S P,SAROHA A K.Catalytic ozonation for the treatment of synthetic and industrial effluents-application of mesoporous materials:a review[J].Journal of Environmental Management,2018,211(1):83-102.
[14]KAPTIJN J P.The ecoclear誖process results from full-scale installations[J].Ozone:Science&Engineering,1997,19(4):297-305.
[15]S魣NCHEZ L,PERAL J,DOM魬NECH X.Aniline degradation by combined photocatalysis and ozonation[J].Applied Catalysis B:Environmental,1998,19(1):59-65.
[16]BELTR魣N F J,RIVAS F J,MONTERO-DE-ESPINOSA R.Catalytic ozonation of oxalic acid in an aqueous TiO2slurry reactor[J].Applied Catalysis B:Environmental,2002,39(3):221-231.
[17]CHANG C Y,CHEN J N.Ozonolysis of 2,4-dichlorophenol in a two-phase solvent/water system[J].Water Science and Technology,1994,29(9):343-346.
[18]KASPRZYK B,NAWROCKI J.Preliminary results on ozonation enhancement by a perfluorinated bonded alumina phase[J].Ozone:Science&Engineering,2002,24(1):63-68.
[19]KASPRZYK-HORDERN B,DABROWSKA A,NAWROCKI J.Proceedings of the International Conference on Ozone[C].Berlin,2003.
[20]杨霞霞,陈雪松,朱震杰,等.多相紫外臭氧联合氧化法处理亚甲基蓝的研究[J].浙江冶金,2015,(4):29-31.
[21]董德明,曹珍,闫征楚,等.臭氧-超声联用处理聚乙烯醇废水[J].吉林大学学报(地球科学版),2016,46(4):1191-1198.
[22]谭江月.超声波臭氧技术联用处理对硝基苯胺废水研究[J].水处理技术,2011,37(4):64-71.
[23]胡晓.臭氧高级氧化技术在水处理领域的研究进展[J].安徽农学通报,2017,23(16):104.
[24]李绍峰,黄君礼,伦中财,等.臭氧-生物活性炭-膜法处理自来水[J].中国给水排水,2002,18(3):69-72.
[25]孙珊珊,刘邦海,张科亭,等.臭氧-生物处理联用工艺深度处理苯胺黑染料废水[J].中国海洋大学学报,2018,48(8):125-130.
[26]鲁秀国,黄林长,张耀,等.臭氧氧化-生物接触氧化处理黑臭水[J].水处理技术,2018,44(4):89-91.
[2]黄程兰,刘敏,陈滢.臭氧在污水处理中的应用[J].四川化工,2012,15(1):25-27.
[3]KASPRZYK-HORDERN B,ZI魷LEK M,NAWROCKI J.Catalytic ozonation and methods of enhancing molecular ozone reactions in water treatment[J].Applied Catalysis B:Environmental,2003,46(4):639-669.
[4]迟婷.臭氧氧化技术对各种染料处理效果及机理的研究[D]青岛:青岛科技大学,2015.
[5]PIERA E,CALPE J C,BRILLAS E,et al.2,4-Dichlorophenox yacetic acid degradation by catalyzed ozonation:TiO2/UVA/O3and Fe(Ⅱ)/UVA/O3systems[J].Applied Catalysis B:Environmental,2000,27(3):169-177.
[6]TANAKA K,ABE K,SHENG C Y,et al.Photocatalytic waste water treatment combined with ozone pretreatment[J].Environmen tal Science&Technology,1992,26(12):2534-2536.
[7]PINES D S,RECKHOW D A.Effect of dissolved cobalt(Ⅱ)on the ozonation of oxalic acid[J].Environmental Science&Technology,2002,36(19):4046-4051.
[8]黄深.城市污水厂二级处理出水臭氧深度处理研究[D].北京:清华大学,2008.
[9]LEGUBE B,KARPEL VEL LEITNER N.Catalytic ozonation:a promising advanced oxidation technology for water treatment[J].Catalysis Today,1999,53(1):61-72.
[10]GRACIA R,ARAG譈ES J L,OVELLEIRO J L.Study of the catalytic ozonation of humic substances in water and their ozonation byproducts[J].Ozone:Science&Engineering,1996,18(3):195-208.
[11]押玉荣,陈金杰,韩墨菲,等.Mn-Al2O3催化臭氧氧化处理工业废水试验研究[J].工业用水与废水,2018,49(5):27-30.
[12]洪浩峰,潘湛昌,徐阁,等.活性炭负载催化剂臭氧催化氧化处理印染废水研究[J].工业用水与废水,2010,41(3):29-33.
[13]GHUGE S P,SAROHA A K.Catalytic ozonation for the treatment of synthetic and industrial effluents-application of mesoporous materials:a review[J].Journal of Environmental Management,2018,211(1):83-102.
[14]KAPTIJN J P.The ecoclear誖process results from full-scale installations[J].Ozone:Science&Engineering,1997,19(4):297-305.
[15]S魣NCHEZ L,PERAL J,DOM魬NECH X.Aniline degradation by combined photocatalysis and ozonation[J].Applied Catalysis B:Environmental,1998,19(1):59-65.
[16]BELTR魣N F J,RIVAS F J,MONTERO-DE-ESPINOSA R.Catalytic ozonation of oxalic acid in an aqueous TiO2slurry reactor[J].Applied Catalysis B:Environmental,2002,39(3):221-231.
[17]CHANG C Y,CHEN J N.Ozonolysis of 2,4-dichlorophenol in a two-phase solvent/water system[J].Water Science and Technology,1994,29(9):343-346.
[18]KASPRZYK B,NAWROCKI J.Preliminary results on ozonation enhancement by a perfluorinated bonded alumina phase[J].Ozone:Science&Engineering,2002,24(1):63-68.
[19]KASPRZYK-HORDERN B,DABROWSKA A,NAWROCKI J.Proceedings of the International Conference on Ozone[C].Berlin,2003.
[20]杨霞霞,陈雪松,朱震杰,等.多相紫外臭氧联合氧化法处理亚甲基蓝的研究[J].浙江冶金,2015,(4):29-31.
[21]董德明,曹珍,闫征楚,等.臭氧-超声联用处理聚乙烯醇废水[J].吉林大学学报(地球科学版),2016,46(4):1191-1198.
[22]谭江月.超声波臭氧技术联用处理对硝基苯胺废水研究[J].水处理技术,2011,37(4):64-71.
[23]胡晓.臭氧高级氧化技术在水处理领域的研究进展[J].安徽农学通报,2017,23(16):104.
[24]李绍峰,黄君礼,伦中财,等.臭氧-生物活性炭-膜法处理自来水[J].中国给水排水,2002,18(3):69-72.
[25]孙珊珊,刘邦海,张科亭,等.臭氧-生物处理联用工艺深度处理苯胺黑染料废水[J].中国海洋大学学报,2018,48(8):125-130.
[26]鲁秀国,黄林长,张耀,等.臭氧氧化-生物接触氧化处理黑臭水[J].水处理技术,2018,44(4):89-91.