钼酸铋基光催化材料的研究进展
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摘要
近年来,钼酸铋基光催化剂以其优良的特性拓宽了光催化领域的研究,催化剂的制备与应用一直是研究者的关注热点。重点介绍了Bi_2MoO_6的晶体结构、制备方法、形貌及其光催化性能,对比了常见制备方法的优缺点,综述了国内外研究者在改性钼酸铋基光催化材料方面所做的工作,得出在可见光响应下具有高催化活性和高稳定性的钼酸铋基光催化材料将是下一步研究的主要方向。
In recent years,bismuth molybdate-based photocatalysts have broadened the research in the field of photocatalysis with its excellent properties. The preparation and application of catalysts have always been the focus of researchers. The preparation method and photocatalytic performance of Bi_2MoO_6 were introduced. The advantages and disadvantages of common preparation methods were compared. The work done by domestic and foreign researchers on modified bismuth molybdate-based photocatalytic materials is reviewed. It is concluded that the bismuth molybdate-based photocatalytic material with high catalytic activity and high stability under visible light response will be the main direction of the next step.
In recent years,bismuth molybdate-based photocatalysts have broadened the research in the field of photocatalysis with its excellent properties. The preparation and application of catalysts have always been the focus of researchers. The preparation method and photocatalytic performance of Bi_2MoO_6 were introduced. The advantages and disadvantages of common preparation methods were compared. The work done by domestic and foreign researchers on modified bismuth molybdate-based photocatalytic materials is reviewed. It is concluded that the bismuth molybdate-based photocatalytic material with high catalytic activity and high stability under visible light response will be the main direction of the next step.
引文
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[20]陈智琴,曾卫军,周泽华,等.微波水热法制备纳米Ti O2的研究进展[C].全国高技术陶瓷学术年会,2008.
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[24]王智宏.退火法修复Zn O缺陷及回流法制备钼酸铋的光催化性能研究[D].天津:河北工业大学,2015.
[25] Xu Y S,Zhang W D. Monodispersed Ag3PO4nanocrystals loaded on the surface of spherical Bi2Mo O6with enhanced photocatalytic performance[J]. Dalton Transactions,2013,42(4):1094-1101.
[26] Chen L,He J,Liu Y,et al. Recent advances in bismuth-containing photocatalysts with heterojunctions[J]. Chinese Journal of Catalysis,2016,37(6):780-791.
[27]王丹军,申会东,郭莉,等. BiOBr/Bi2Mo O6异质结的构筑及对甲基橙的吸附/光催化性能的协同作用机制[J].环境科学学报,2017,37(5):1751-1762.
[28]林雪,郭晓宇,王庆伟,等. Bi2Mo O6/BiVO4异质结的水热合成和可见光催化活性[J].物理化学学报,2014,30(11).
[29]徐梦秋,柴波,闫俊涛,等. Bi2Mo O6/Ag3PO4复合光催化剂的制备及其光催化性能[J].硅酸盐学报,2018,46(1).
[30] Meng X,Zhang Z. Pd-doped Bi2Mo O6,Plasmonic Photocatalysts with Enhanced Visible Light Photocatalytic Performance[J]. Applied Surface Science,2017,392:169-180.
[31]张俊磊,张丽莎,鞠小逖,等. Bi2Mo O6-Pt异质结的制备及其光催化性能研究[J].环境科学学报,2016,36(6):2050-2058.
[32]宫荟竹,宋小龙,王长华,等. Ag修饰Bi2Mo O6纳米材料的合成表征及光催化性能研究[J].北华大学学报(自然科学版),2014,15(1):39-42.
[33]陈世界,王鹏,翟明翚,等. C/Fe-Bi2Mo O6的制备及其光催化降解诺氟沙星的性能研究[J].高师理科学刊,2016,36(1):48-51.
[34]李跃军,曹铁平,梅泽民,等. Pr掺杂Bi2Mo O6/Ti O2复合纳米纤维的制备及可见光催化性能[J].高等学校化学学报,2017,38(12):2313-2319.
[35]王丹军,申会东,岳林林,等. Eu3+掺杂γ-Bi2Mo O6的合成及其光催化活性研究[J].稀土,2016(3):13-20.
[36]强小丹,高春燕,王丹军,等. Fe3+掺杂Bi2Mo O6光催化剂的合成及其活性研究[J].应用化工,2012,41(9):1553-1556.
[37]宋继梅,胡海琴,周亚运,等. F掺杂可见光催化剂Bi2Mo O6的制备及其增强的光催化性能[J].中国钼业,2013,37(5):36-40.
[2]李红花,李坤威,汪浩,等.α-Bi2Mo3O12和γ-Bi2Mo O6的水热合成及可见光催化性能[J].无机化学学报,2009,25(3):512-516.
[3]缪应纯,潘改芳,霍宇凝,等.原位稀土修饰Bi2Mo O6高效可见光催化剂[J].无机化学学报,2014,30(7):1587-1592.
[4]张家靓,张立峰. Mo(VI)-V(V)-H2O系的热力学平衡与钼酸盐深度除钒工艺的理论分析[J].稀有金属,2016,40(7):701-707.
[5]于建强,张俊武,张妍,et al. Synthesis method of surface hydrophobicity bismuth orthovanadate with performance of catalyzing and degrading pollutant by visible light:,CN 101811040 A[P]. 2010.
[6]杨佳,牛晓君,陈伟仡,等. BiOBr@Bi2Mo O6复合光催化剂制备及其对RhB和BPA降解[J].中国环境科学,2017,37(6):2130-2138.
[7] Teng Z,Liu C,Peng T,et al. Synthesis Conditions and Visible Light Photocatalytic Activity of Perovskite Catalyst Lao,9Sro,1Ni03[J].Materials Review,2016,30(6):19.
[8] Wang X,Gu F,LI L,et al. A facile mixed-solvothermal route to y-Bi2Mo O6nanoflakes and their visible-light-responsive photocatalytic activity[J]. Materials Research Bulletin,2013,48:3761.
[9]孙明志,郭鹏瑶,丁航行,等.煅烧温度对溶胶-凝胶法制备钼酸铋光催化性能的影响[J].材料热处理学报,2017,38(3):21-28.
[10] Liu J,Yu J,Xu G. METHOD FOR PREPARING NI-MG/AL2O3CATALYST,WO/2013/166653[P]. 2013.
[11]王敏,杨长秀,郑浩岩,等.反应温度对钼酸铋粉体形貌和可见光催化性能的影响[J].硅酸盐学报,2015,43(11):1643-1649.
[12]高俊杰,郭鹏瑶,高文皓,等.反应时间对Bi2Mo O6晶体形貌和可见光催化性能的影响[J].材料热处理学报,2016,37(9):11-16.
[13]张雄斌,贺辛亥,程稼稷,等.纳米氧化锌的制备及改性研究进展[J].人工晶体学报,2017,46(10):2054-2057.
[14] Umapathy V,Manikandan A,Antony S A,et al. Structure,morphology and opto-magnetic properties of Bi2Mo O6,nano-photocatalyst synthesized by sol-gel method[J]. Transactions of Nonferrous Metals Society of China,2015,25(10):3271-3278.
[15]缪应纯,王刚,陈广,等.醇热制备微球Bi2Mo O6及其光催化活性[J].化学试剂,2014,36(2):160-164.
[16]朱礼.钼酸铋复合氧化物的制备、修饰及其可见光催化性能的研究[D].广州:华南理工大学硕士学位论文,2011.
[17]杨浩,郑华艳,常瑜,等.以共沉淀法为基础的铜基催化剂制备新技术的研究进展[J].化工进展,2014,33(2):379-386.
[18]杜永芳,宋继梅,王红,等.共沉淀法制备α-Bi2Mo3O12和γ-Bi2Mo O6及可见光催化性能[J].合肥工业大学学报:自然科学版,2012(11):1500-1505.
[19]左广玲,叶红勇,李入林.超声辅助沉淀法制备γ-Bi2Mo O6及其光催化性能[J].化工环保,2015,35(1):89-93.
[20]陈智琴,曾卫军,周泽华,等.微波水热法制备纳米Ti O2的研究进展[C].全国高技术陶瓷学术年会,2008.
[21]张婷,黄剑锋,曹丽云,等.微波水热温度对合成Bi2Mo O6微晶形貌和光学性能的影响[J].人工晶体学报,2012,41(3):000616-620.
[22]张婷,黄剑锋,曹丽云,等.微波水热合成时间对Bi2Mo O6微晶形貌和可见光催化性能的影响[J].硅酸盐学报,2013,41(5):710-714.
[23]张琴,汪晓凤,段芳,等. Bi2Mo O6中空微球的制备及其光催化性能[J].无机化学学报,2015,31(11):2152-2158.
[24]王智宏.退火法修复Zn O缺陷及回流法制备钼酸铋的光催化性能研究[D].天津:河北工业大学,2015.
[25] Xu Y S,Zhang W D. Monodispersed Ag3PO4nanocrystals loaded on the surface of spherical Bi2Mo O6with enhanced photocatalytic performance[J]. Dalton Transactions,2013,42(4):1094-1101.
[26] Chen L,He J,Liu Y,et al. Recent advances in bismuth-containing photocatalysts with heterojunctions[J]. Chinese Journal of Catalysis,2016,37(6):780-791.
[27]王丹军,申会东,郭莉,等. BiOBr/Bi2Mo O6异质结的构筑及对甲基橙的吸附/光催化性能的协同作用机制[J].环境科学学报,2017,37(5):1751-1762.
[28]林雪,郭晓宇,王庆伟,等. Bi2Mo O6/BiVO4异质结的水热合成和可见光催化活性[J].物理化学学报,2014,30(11).
[29]徐梦秋,柴波,闫俊涛,等. Bi2Mo O6/Ag3PO4复合光催化剂的制备及其光催化性能[J].硅酸盐学报,2018,46(1).
[30] Meng X,Zhang Z. Pd-doped Bi2Mo O6,Plasmonic Photocatalysts with Enhanced Visible Light Photocatalytic Performance[J]. Applied Surface Science,2017,392:169-180.
[31]张俊磊,张丽莎,鞠小逖,等. Bi2Mo O6-Pt异质结的制备及其光催化性能研究[J].环境科学学报,2016,36(6):2050-2058.
[32]宫荟竹,宋小龙,王长华,等. Ag修饰Bi2Mo O6纳米材料的合成表征及光催化性能研究[J].北华大学学报(自然科学版),2014,15(1):39-42.
[33]陈世界,王鹏,翟明翚,等. C/Fe-Bi2Mo O6的制备及其光催化降解诺氟沙星的性能研究[J].高师理科学刊,2016,36(1):48-51.
[34]李跃军,曹铁平,梅泽民,等. Pr掺杂Bi2Mo O6/Ti O2复合纳米纤维的制备及可见光催化性能[J].高等学校化学学报,2017,38(12):2313-2319.
[35]王丹军,申会东,岳林林,等. Eu3+掺杂γ-Bi2Mo O6的合成及其光催化活性研究[J].稀土,2016(3):13-20.
[36]强小丹,高春燕,王丹军,等. Fe3+掺杂Bi2Mo O6光催化剂的合成及其活性研究[J].应用化工,2012,41(9):1553-1556.
[37]宋继梅,胡海琴,周亚运,等. F掺杂可见光催化剂Bi2Mo O6的制备及其增强的光催化性能[J].中国钼业,2013,37(5):36-40.