CO催化氧化催化剂改性研究进展
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摘要
通过添加助剂(稀土金属和过渡金属)、选择合适载体(金属氧化物、分子筛及其他载体)及改进材料制备方法(采用微波替代传统加热方式等)三方面,综述了近年来对CO催化氧化催化剂进行改性的研究进展。非贵金属催化剂是催化领域的主流方向,采用不同的方法对非贵金属催化剂进行改性,提高CO催化氧化催化剂的催化活性、稳定性和实际应用是今后需要研究的主要内容。
The research progress is reviewed on modi?cation of CO catalytic oxidation catalysts by adding auxiliaries(rare earth and transition metals),selecting suitable carriers(metal oxides,molecular sieves and other carriers) and improving the material preparation methods(using microwave instead of traditional heating methods,etc.) in recent years. Non-noble metal catalyst is the mainstream direction of catalysis research. Modi?cation of non-noble metal catalysts by different methods to improve their catalytic activity,stability and practical application is the main research contents next.
The research progress is reviewed on modi?cation of CO catalytic oxidation catalysts by adding auxiliaries(rare earth and transition metals),selecting suitable carriers(metal oxides,molecular sieves and other carriers) and improving the material preparation methods(using microwave instead of traditional heating methods,etc.) in recent years. Non-noble metal catalyst is the mainstream direction of catalysis research. Modi?cation of non-noble metal catalysts by different methods to improve their catalytic activity,stability and practical application is the main research contents next.
引文
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[8]Kuncham K,Putla S,Benjaram M,et al.Nanocrystalline Ce1-xSmxO2-δ(x=0.4)solid solutions:Structural characterization versus CO oxidation[J].RSC Adv,2014,21(3):7953-7962.
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[10]Han Weiliang,Tang Zhicheng,Zhang Peng,et al.Study of one step synthesis of rare earth zeolite(Ln/ZSM-5)and application for low temperature CO catalytic oxidation[J].Catal Surveys Asia,2013,17(3/4):147-155.
[11]Li Hailong,Yu Ke,Chao Wan,et al.Comparison of the nickel addition patterns on the catalytic performances of LaCoO3,for low-temperature CO oxidation[J].Catal Today,2016,281:534-541.
[12]Liu Ruihui,Gao Nansha,Zhen Feng,et al.Doping effect of Al2O3 and CeO2 on Fe2O3 support for gold catalyst in COoxidation at low-temperature[J].Chem Eng J,2013,225:245-253.
[13]Guo Xiaolin,Li Jing,Zhou Renxian.Catalytic performance of manganese doped CuO-CeO2,catalysts for selective oxidation of CO in hydrogen-rich gas[J].Fuel,2016,163:56-64.
[14]Ma Shimei,Lu Guanzhong,Shen Yuexin,et al.Effect of Fe doping on the catalytic performance of CuO-CeO2 for low temperature CO oxidation[J].Catal Sci Technol,2011,1(4):669-674.
[15]Li Gengnan,Li Liang,Li Yongsheng,et al.A highly moisture-resistant Fe-doped mesoporous Co3O4 catalyst for efficient low-temperature CO oxidation[J].New J Chem,2015,39(3):1742-1748.
[16]Yu Sungju,Yun H J,Lee D M,et al.Preparation and characterization of Fe-doped TiO2 nanoparticles as a support for a high performance CO oxidation catalyst[J].J Mater Chem,2012,22(25):12629-12635.
[17]Cai L,Hu Zhenhao,Branton P,et al.The effect of doping transition metal oxides on copper manganese oxides for the catalytic oxidation of CO[J].Chin J Catal,2014,35(2):159-167.
[18]Guo Xiaolin,Qiu Zhihuan,Mao Jianxin,et al.Doping effect of transition metals(Zr,Mn,Ti and Ni)on well-shaped CuO/CeO2(rods):Nano/micro structure and catalytic performance for selective oxidation of CO in excess H2[J].J Dispersion Sci Technol,2018,20(40):25983-25994.
[19]Han S W,Kim D H,Jeong M G,et al.CO oxidation catalyzed by NiO supported on mesoporous Al2O3 at room temperature[J].Chem Eng J,2016,283:992-998.
[20]Estifaee P,Haghighi M,Mohammadi N,et al.CO oxidation over sonochemically synthesized Pd-Cu/Al2O3 nanocatalyst used in hydrogen purification:Effect of Pd loading and ultrasound irradiation time[J].Ultrason Sonochem,2014,21(3):1155-1165.
[21]Wang Fagen,Zhao Kunfeng,Zhang Haojie,et al.Low temperature CO catalytic oxidation over supported Pd-Cu catalysts calcined at different temperatures[J].Chem Eng J,2014,242:10-18.
[22]Bansmann J,Ku?erováG,Abdel-Mageed A M,et al.Influence of re-activation and ongoing CO oxidation reaction on the chemical and electronic properties of Au on a Au/CeO2catalyst:A XANES study at the Au LⅢedge[J].J Electron Spectrosc Relat Phenom,2017,220:86-90.
[23]Kast P,Friedrich M,Girgsdies F,et al.Strong metalsupport interaction and alloying in Pd/ZnO catalysts for COoxidation[J].Catal Today,2016,260:21-31.
[24]Leung E,Shimizu A,Barmak K,et al.Copper oxide catalyst supported on niobium oxide for CO oxidation at low temperatures[J].Catal Commun,2017,97:42-46.
[25]Ayastuy J L,Gurbani A,Gutierrez-Ortiz M A.Effect of calcination temperature on catalytic properties of Au/Fe2O3catalysts in CO-PROX[J].Int J Hydrogen Energy,2016,41(43):19546-19555.
[26]Liu Yuxi,Dai Hongxing,Deng Jiguang,et al.Mesoporous Co3O4-supported gold nanocatalysts:Highly active for the oxidation of carbon monoxide,benzene,toluene,and o-xylene[J].J Catal,2014,309:408-418.
[27]Sandoval A,Zanella R,Klimova T E.Titania nanotubes decorated with anatase nanocrystals as support for active and stable gold catalysts for CO oxidation[J].Catal Today,2017,282:140-150.
[28]Ye Qing,Zhao Jiansheng,Huo Feifei,et al.Nanosized Au supported on three-dimensionally ordered mesoporousβ-MnO2:Highly active catalysts for the low-temperature oxidation of carbon monoxide,benzene,and toluene[J].Microporous Mesoporous Mater,2013,172:20-29.
[29]Satsuma A,Osaki K,Yanagihara M,et al.Activity controlling factors for low-temperature oxidation of CO over supported Pd catalysts[J].Appl Catal,B,2013,132/133:511-518.
[30]Zhang Hongpeng,Liu Haichao.Insights into support effects on Ce-Zr-O mixed oxide-supported gold catalysts in CO oxidation[J].J Energy Chem,2013,22(1):106-109.
[31]Zhao Zhongkui,Yung M M,Ozkan U S.Effect of support on the preferential oxidation of CO over cobalt catalysts[J].Catal Commun,2008,9(6):1465-1471.
[32]Gatla S,Aubert D,Agostini G,et al.Room-temperature COoxidation catalyst:Low-temperature metal-support interaction between platinum nanoparticles and nanosized ceria[J].ACSCatal,2016,6(9):6151-6155.
[33]Cui Huizhen,Guo Yu,Wang Xu,et al.Gold-iron oxide catalyst for CO oxidation:Effect of support structure[J].Catalysts,2016,6(3):1-13.
[34]Li Kairong,Wang Yaojie,Wang Shurong,et al.A comparative study of CuO/TiO2-SnO2,CuO/TiO2 and CuO/SnO2 catalysts for low-temperature CO oxidation[J].J Nat Gas Chem,2009,18(4):449-452.
[35]Dong Lihui,Tang Yanxia,Li Bin,et al.Influence of molar ratio and calcination temperature on the properties of TixSn1-xO2supporting copper oxide for CO oxidation[J].Appl Catal,B,2016,180:451-462.
[36]赵海霞,叶青,张玉,等.氧化锰八面体分子筛负载Cu催化剂催化氧化性能研究[J].环境污染与防治,2014(4):33-37.
[37]Fu Zhidan,Liu Lisha,Song Yong,et al.Catalytic oxidation of carbon monoxide,toluene,and ethyl acetate over the x Pd/OMS-2 catalysts:Effect of Pd loading[J].Front Chem Sci Eng,2017,11(2):185-196.
[38]Vargas O A G,De Los Reyes Heredia J A,Castellanos A M,et al.Cerium incorporating into MCM-41 mesoporous materials for CO oxidation[J].Mater Chem Phys,2013,139(1):125-133.
[39]Hassan H M A,Betiha M A,Elshaarawy R F M,et al.Promotion effect of palladium on Co3O4 incorporated within mesoporous MCM-41 silica for CO oxidation[J].Appl Surf Sci,2017,402:99-107.
[40]GuoYafei,Lin Jin,Li Changhai,et al.Copper manganese oxides supported on multi-walled carbon nanotubes as an efficient catalyst for low temperature CO oxidation[J].Catal Lett,2016,146(11):2364-2375.
[41]Li Xiaona,Yuan Zhen,Meng Jingheng,et al.Catalytic COoxidation on single Pt-atom doped aluminum oxide clusters:Electronegativity-ladder effect[J].J Phys Chem C,2015,119(27):15414-15420.
[42]Dhahri M,Mu?oz M A,Yeste M P,et al.Preparation of manganese-impregnated alumina-pillared bentonite,characterization and catalytic oxidation of CO[J].React Kinet Mech Catal,2016,118(2):655-668.
[43]Cao Jianliang,Wang Yi,Li Gaojie,et al.Mesoporous modified red mud supported CuO nanocatalysts for carbon monoxide oxidation[J].Curr Nanosci,2015,11(4):413-418.
[44]Sun Jingfang,Zhang Lei,Ge Chengyan,et al.Comparative study on the catalytic CO oxidation properties of CuO/CeO2,catalysts prepared by solid state and wet impregnation[J].Chin J Catal,2014,35(8):1347-1358.
[45]Li Shuna,Zhu Huaqing,Qin Zhangfeng,et al.Morphologic effects of nano CeO2-Ti O2,on the performance of Au/CeO2-Ti O2,catalysts in low-temperature CO oxidation[J].Appl Catal,B,2014,144(2):498-506.
[46]Amini E,Rezaei M,Sadeghinia M.Low temperature COoxidation over mesoporous CuFe2O4,nanopowders synthesized by a novel sol-gel method[J].Chin J Catal,2013,34(9):1762-1767.
[47]Polychronopoulou1 K,Zedan A F,Katsiotis M S,et al.Rapid microwave assisted sol-gel synthesis of CeO2 and CexSm1-xO2 nanoparticle catalysts for CO oxidation[J].J Mol Catal A:Chem,2016,428:41-55.
[48]Gu Chunlei,Lu Suhong,Miao Jie,et al.Meso-macroporous monolithic CuO/CeO2/γ/α-Al2O3 catalysts for CO preferential oxidation in hydrogen-rich gas:Effect of loading methods[J].Int J Hydrogen Energy,2010,35(12):6113-6122.
[49]陈豪,黄诗琳,郭长青,等.甘氨酸燃烧法制备Co/CeO2催化剂用于CO选择性氧化脱除[J].暨南大学学报,2014,35(5):445-448.
[50]Kudo S,Maki T,Yamada M,et al.A new preparation method of Au/ferric oxide catalyst for low temperature CO oxidation[J].Chem Eng Sci,2010,65(1):214-219.
[2]胡玲,张海东,王小菡,等.CO催化氧化催化剂活性成分研究进展[J].材料导报,2016,30(21):46-53.
[3]姚小江,贡营涛,李红丽.铈基催化剂用于NH3选择性催化还原NOx的研究进展[J].物理化学学报,2015,31(5):817-828.
[4]Reddy B M,Thrimurthulu G,Katta L,et al.Structural characteristics and catalytic activity of nanocrystalline ceria-praseodymia solid solutions[J].J Phys Chem C,2009,113(36):15882-15890.
[5]Benjaram M R,Katta L,Thrimurthulu G.Novel nanocrystalline Ce1-xLaxO2-δ(x=0.2)solid solutions:Structural characteristics and catalytic performance[J].Cheminform,2010,22(2):467-475.
[6]Reddy L H,Reddy G K,Devaiah D,et al.A rapid microwave-assisted solution combustion synthesis of CuO promoted Ce O2-MxOy(M=Zr,La,Pr and Sm)catalysts for CO oxidation[J].Appl Catal,A,2012,445/446:297-305.
[7]Said Alod-EI-Aziz A,El-Wahab M M M A,Goda M N.Synthesis and characterization of pure and(Ce,Zr,Ag)doped mesoporous CuO-Fe2O3 as highly efficient and stable nanocatalysts for COoxidation at low temperature[J].Appl Surf Sci,2016,390:649-665.
[8]Kuncham K,Putla S,Benjaram M,et al.Nanocrystalline Ce1-xSmxO2-δ(x=0.4)solid solutions:Structural characterization versus CO oxidation[J].RSC Adv,2014,21(3):7953-7962.
[9]Damma D,Takuya T,Thirupathi B,et al.Ce0.80M0.12Sn0.08O2-δ(M=Hf,Zr,Pr,and La)ternary oxide solid solutions with superior properties for CO oxidation[J].RSC Advances,2015,38(5):30275-30285.
[10]Han Weiliang,Tang Zhicheng,Zhang Peng,et al.Study of one step synthesis of rare earth zeolite(Ln/ZSM-5)and application for low temperature CO catalytic oxidation[J].Catal Surveys Asia,2013,17(3/4):147-155.
[11]Li Hailong,Yu Ke,Chao Wan,et al.Comparison of the nickel addition patterns on the catalytic performances of LaCoO3,for low-temperature CO oxidation[J].Catal Today,2016,281:534-541.
[12]Liu Ruihui,Gao Nansha,Zhen Feng,et al.Doping effect of Al2O3 and CeO2 on Fe2O3 support for gold catalyst in COoxidation at low-temperature[J].Chem Eng J,2013,225:245-253.
[13]Guo Xiaolin,Li Jing,Zhou Renxian.Catalytic performance of manganese doped CuO-CeO2,catalysts for selective oxidation of CO in hydrogen-rich gas[J].Fuel,2016,163:56-64.
[14]Ma Shimei,Lu Guanzhong,Shen Yuexin,et al.Effect of Fe doping on the catalytic performance of CuO-CeO2 for low temperature CO oxidation[J].Catal Sci Technol,2011,1(4):669-674.
[15]Li Gengnan,Li Liang,Li Yongsheng,et al.A highly moisture-resistant Fe-doped mesoporous Co3O4 catalyst for efficient low-temperature CO oxidation[J].New J Chem,2015,39(3):1742-1748.
[16]Yu Sungju,Yun H J,Lee D M,et al.Preparation and characterization of Fe-doped TiO2 nanoparticles as a support for a high performance CO oxidation catalyst[J].J Mater Chem,2012,22(25):12629-12635.
[17]Cai L,Hu Zhenhao,Branton P,et al.The effect of doping transition metal oxides on copper manganese oxides for the catalytic oxidation of CO[J].Chin J Catal,2014,35(2):159-167.
[18]Guo Xiaolin,Qiu Zhihuan,Mao Jianxin,et al.Doping effect of transition metals(Zr,Mn,Ti and Ni)on well-shaped CuO/CeO2(rods):Nano/micro structure and catalytic performance for selective oxidation of CO in excess H2[J].J Dispersion Sci Technol,2018,20(40):25983-25994.
[19]Han S W,Kim D H,Jeong M G,et al.CO oxidation catalyzed by NiO supported on mesoporous Al2O3 at room temperature[J].Chem Eng J,2016,283:992-998.
[20]Estifaee P,Haghighi M,Mohammadi N,et al.CO oxidation over sonochemically synthesized Pd-Cu/Al2O3 nanocatalyst used in hydrogen purification:Effect of Pd loading and ultrasound irradiation time[J].Ultrason Sonochem,2014,21(3):1155-1165.
[21]Wang Fagen,Zhao Kunfeng,Zhang Haojie,et al.Low temperature CO catalytic oxidation over supported Pd-Cu catalysts calcined at different temperatures[J].Chem Eng J,2014,242:10-18.
[22]Bansmann J,Ku?erováG,Abdel-Mageed A M,et al.Influence of re-activation and ongoing CO oxidation reaction on the chemical and electronic properties of Au on a Au/CeO2catalyst:A XANES study at the Au LⅢedge[J].J Electron Spectrosc Relat Phenom,2017,220:86-90.
[23]Kast P,Friedrich M,Girgsdies F,et al.Strong metalsupport interaction and alloying in Pd/ZnO catalysts for COoxidation[J].Catal Today,2016,260:21-31.
[24]Leung E,Shimizu A,Barmak K,et al.Copper oxide catalyst supported on niobium oxide for CO oxidation at low temperatures[J].Catal Commun,2017,97:42-46.
[25]Ayastuy J L,Gurbani A,Gutierrez-Ortiz M A.Effect of calcination temperature on catalytic properties of Au/Fe2O3catalysts in CO-PROX[J].Int J Hydrogen Energy,2016,41(43):19546-19555.
[26]Liu Yuxi,Dai Hongxing,Deng Jiguang,et al.Mesoporous Co3O4-supported gold nanocatalysts:Highly active for the oxidation of carbon monoxide,benzene,toluene,and o-xylene[J].J Catal,2014,309:408-418.
[27]Sandoval A,Zanella R,Klimova T E.Titania nanotubes decorated with anatase nanocrystals as support for active and stable gold catalysts for CO oxidation[J].Catal Today,2017,282:140-150.
[28]Ye Qing,Zhao Jiansheng,Huo Feifei,et al.Nanosized Au supported on three-dimensionally ordered mesoporousβ-MnO2:Highly active catalysts for the low-temperature oxidation of carbon monoxide,benzene,and toluene[J].Microporous Mesoporous Mater,2013,172:20-29.
[29]Satsuma A,Osaki K,Yanagihara M,et al.Activity controlling factors for low-temperature oxidation of CO over supported Pd catalysts[J].Appl Catal,B,2013,132/133:511-518.
[30]Zhang Hongpeng,Liu Haichao.Insights into support effects on Ce-Zr-O mixed oxide-supported gold catalysts in CO oxidation[J].J Energy Chem,2013,22(1):106-109.
[31]Zhao Zhongkui,Yung M M,Ozkan U S.Effect of support on the preferential oxidation of CO over cobalt catalysts[J].Catal Commun,2008,9(6):1465-1471.
[32]Gatla S,Aubert D,Agostini G,et al.Room-temperature COoxidation catalyst:Low-temperature metal-support interaction between platinum nanoparticles and nanosized ceria[J].ACSCatal,2016,6(9):6151-6155.
[33]Cui Huizhen,Guo Yu,Wang Xu,et al.Gold-iron oxide catalyst for CO oxidation:Effect of support structure[J].Catalysts,2016,6(3):1-13.
[34]Li Kairong,Wang Yaojie,Wang Shurong,et al.A comparative study of CuO/TiO2-SnO2,CuO/TiO2 and CuO/SnO2 catalysts for low-temperature CO oxidation[J].J Nat Gas Chem,2009,18(4):449-452.
[35]Dong Lihui,Tang Yanxia,Li Bin,et al.Influence of molar ratio and calcination temperature on the properties of TixSn1-xO2supporting copper oxide for CO oxidation[J].Appl Catal,B,2016,180:451-462.
[36]赵海霞,叶青,张玉,等.氧化锰八面体分子筛负载Cu催化剂催化氧化性能研究[J].环境污染与防治,2014(4):33-37.
[37]Fu Zhidan,Liu Lisha,Song Yong,et al.Catalytic oxidation of carbon monoxide,toluene,and ethyl acetate over the x Pd/OMS-2 catalysts:Effect of Pd loading[J].Front Chem Sci Eng,2017,11(2):185-196.
[38]Vargas O A G,De Los Reyes Heredia J A,Castellanos A M,et al.Cerium incorporating into MCM-41 mesoporous materials for CO oxidation[J].Mater Chem Phys,2013,139(1):125-133.
[39]Hassan H M A,Betiha M A,Elshaarawy R F M,et al.Promotion effect of palladium on Co3O4 incorporated within mesoporous MCM-41 silica for CO oxidation[J].Appl Surf Sci,2017,402:99-107.
[40]GuoYafei,Lin Jin,Li Changhai,et al.Copper manganese oxides supported on multi-walled carbon nanotubes as an efficient catalyst for low temperature CO oxidation[J].Catal Lett,2016,146(11):2364-2375.
[41]Li Xiaona,Yuan Zhen,Meng Jingheng,et al.Catalytic COoxidation on single Pt-atom doped aluminum oxide clusters:Electronegativity-ladder effect[J].J Phys Chem C,2015,119(27):15414-15420.
[42]Dhahri M,Mu?oz M A,Yeste M P,et al.Preparation of manganese-impregnated alumina-pillared bentonite,characterization and catalytic oxidation of CO[J].React Kinet Mech Catal,2016,118(2):655-668.
[43]Cao Jianliang,Wang Yi,Li Gaojie,et al.Mesoporous modified red mud supported CuO nanocatalysts for carbon monoxide oxidation[J].Curr Nanosci,2015,11(4):413-418.
[44]Sun Jingfang,Zhang Lei,Ge Chengyan,et al.Comparative study on the catalytic CO oxidation properties of CuO/CeO2,catalysts prepared by solid state and wet impregnation[J].Chin J Catal,2014,35(8):1347-1358.
[45]Li Shuna,Zhu Huaqing,Qin Zhangfeng,et al.Morphologic effects of nano CeO2-Ti O2,on the performance of Au/CeO2-Ti O2,catalysts in low-temperature CO oxidation[J].Appl Catal,B,2014,144(2):498-506.
[46]Amini E,Rezaei M,Sadeghinia M.Low temperature COoxidation over mesoporous CuFe2O4,nanopowders synthesized by a novel sol-gel method[J].Chin J Catal,2013,34(9):1762-1767.
[47]Polychronopoulou1 K,Zedan A F,Katsiotis M S,et al.Rapid microwave assisted sol-gel synthesis of CeO2 and CexSm1-xO2 nanoparticle catalysts for CO oxidation[J].J Mol Catal A:Chem,2016,428:41-55.
[48]Gu Chunlei,Lu Suhong,Miao Jie,et al.Meso-macroporous monolithic CuO/CeO2/γ/α-Al2O3 catalysts for CO preferential oxidation in hydrogen-rich gas:Effect of loading methods[J].Int J Hydrogen Energy,2010,35(12):6113-6122.
[49]陈豪,黄诗琳,郭长青,等.甘氨酸燃烧法制备Co/CeO2催化剂用于CO选择性氧化脱除[J].暨南大学学报,2014,35(5):445-448.
[50]Kudo S,Maki T,Yamada M,et al.A new preparation method of Au/ferric oxide catalyst for low temperature CO oxidation[J].Chem Eng Sci,2010,65(1):214-219.