超支化有机硅功能高分子的研究进展
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摘要
超支化有机硅一般具有三维结构,分子与分子之间基本不出现链缠结,使其宏观上表现出低粘度、高反应活性、高溶解性等特性。超支化有机硅因制备方法较简单、成本较低、可规模化生产、易于功能化等优点,在功能高分子材料领域有广阔的应用前景。本文综述了超支化有机硅功能高分子的制备,包括超支化聚硅氧烷、聚碳硅烷、聚硅烷以及含杂原子的超支化有机硅的制备,重点总结了超支化有机硅功能高分子在催化剂载体、生物医药材料、耐热材料、陶瓷前驱体以及光电材料方面的应用,并对超支化有机硅功能高分子未来的发展作出了展望。
Hyperbranched organic silicon usually have three dimensional structure and no chain entanglement between molecules and molecules, making them exhibit low viscosity, high reactivity, high solubility and so on. Hyperbranched organic silicon has wide-range prospect in the field of functional polymers due to its simple procedures, lower cost as well as scale production and functionalization. The paper reviews the preparation of the functional polymer of hyperbranched organic silicon including the hyperbranched polysiloxane, polycarbosilane, polysilane as well as the organic silicon of hyperbranched with heteroatom. It concludes the implementation of the functional polymer of hyperbranched organic silicon in areas, such as the catalyst carrier, biomedical materials, heat-resistant material, ceramic precursor and photoelectric material, and provides an outlook of the future of the functional polymer of hyperbranched organic silicon.
Hyperbranched organic silicon usually have three dimensional structure and no chain entanglement between molecules and molecules, making them exhibit low viscosity, high reactivity, high solubility and so on. Hyperbranched organic silicon has wide-range prospect in the field of functional polymers due to its simple procedures, lower cost as well as scale production and functionalization. The paper reviews the preparation of the functional polymer of hyperbranched organic silicon including the hyperbranched polysiloxane, polycarbosilane, polysilane as well as the organic silicon of hyperbranched with heteroatom. It concludes the implementation of the functional polymer of hyperbranched organic silicon in areas, such as the catalyst carrier, biomedical materials, heat-resistant material, ceramic precursor and photoelectric material, and provides an outlook of the future of the functional polymer of hyperbranched organic silicon.
引文
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[2] Gao C,Yan D.Prog Polym Sci,2004,29(3):183～275.
[3] Si Q F,Wang X,Fan X D,Wang S J.J Polym Sci Pol Chem,2005,43(9):1883～1894.
[4] 张国彬,范晓东,孔杰,刘郁杨,解云川.化学进展,2008,(Z1):326～338.
[5] 薛磊,刘莹,黄艳华,苏正涛.有机硅材料,2016,30(01):58～69.
[6] 李光亮.有机硅高分子化学.北京:科学出版社,1998:1～5.
[7] Agrawal G,Zhu X,Moeller M,Choudhary V.Polymer,2017,133:40～49.
[8] Chen S,Zhuo D,Hu J.Ind Eng Chen Res,2018,57(31),10372～10378.
[9] Zhang H,Yuan L,Liang G,Gu A J.Appl Surf Sci,2014,320:883～894.
[10] Liu Z,Yuan L,Liang G Z,Gu A J.Polym Advan Technol,2015,26(12):1608～1618.
[11] Liu H,Gao X,Deng B,Huang G.J Appl Polym Sci,2018,135(23):46340.
[12] Yan H X,Jia Y,Ma L,Wang Y L.Nano,2014,9(03):1450040.
[13] 葛娟,卢丹,周权,宋宁,倪礼忠.功能高分子学报,2018,31(04):374～380.
[14] Zhong X Q,Pei X L,Miao Y L,He L,Huang Q.J Eur Ceram Soc,2017,37(10):3263～3270.
[15] Li X,Pei X,Zhong X,Mo G,He L,Huang Z,Huang Q.J Am Ceram Soc.(doi:10.1111/jace.15966)
[16] Liu X X,Rathore J S,Dubois G,Interrante L V.J Polym Sci Pol Chem,2017,55(9):1547～1557.
[17] Ponomarenko S A,Kirchmeyer S.Conjugated organosilicon materials for organic electronics and photonics.Berlin:Springer Group,2010:33～110.
[18] 张梦萌,颜红侠,唐玉生,叶帅.材料导报,2011,25(15):86～91.
[19] 王灯旭,孙文艳,冯圣玉.化学进展,2008,20(11):1651～1658.
[20] 王桂荣,解菊,董玉慧,薛运生.分子科学学报,2014,30(02):94～101.
[21] 熊英,梁秋鸿,王晓玲,武青青,杨建静.中国科学:化学,2016,46(05):517～524.
[22] Kong J,Schmalz T,Motz G,Muller A.Macromolecules,2011,44(6):1280～1291.
[23] Gu J W,Xu S,Zhuang Q,Tang Y S,Kong J.IEEE T Dielect El In,2017,24(2):784～790.
[24] 刘婷婷,田威,白阳,范晓东.高分子通报,2013,5:9～16.
[25] 沈利亚.低表面能复合改性有机硅树脂的制备及表征.上海:华东理工大学,2012.
[26] Mangala K,Sreekumar K.J Appl Polym Sci,2015,132(10):41593.
[27] Zhang Y H,Yuan L,Guan Q B,Liang G Z,Gu A J.J Mater Chem A,2017,5(32):16889～16897.
[28] Jiang B,Zhang K Y,Zhang T,Xu Z M,Huang Y D.Compos Part B-Eng,2017,121:1～8.
[29] Jiang Z J,Yuan L,Liang G Z,Gu A J.Polym Degrad Stabil,2015,121:30～41.
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[31] Jia P,Liu H C,Wang Y C,Cai X F.RSC Adv,2015,5(118):97413～97421.
[32] 周新贵.航空制造技术,2014,450(6):30～34.
[33] 苗玉龙,裴学良,莫高明,杨建行,黄庆,何流.陶瓷学报,2016,37(02):109～114.
[34] Yu Z J,Yang L,Min H,Zhang P,Liu A H,Riedel R.J Eur Ceram Soc,2015,35(2):851～858.
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[36] Liu F,Kong J,Luo C,Ye F,Luan L,Tian N,Liu Y,Zhang H,Gu J,Tang Y.Adv Compos Lett,2018,1(3):506～517.
[37] Xue Y Y,Qiu X Q,Wu Y,Qian Y,Zhou M S,Deng Y H,Li Y.Polym Chem,2016,7(21):3502～3508.;
[38] Li D,Hu R R,Guo D,Zang Q G,Li J H,Wang Y K,Zheng Y S,Tang B Z,Zhang H.J Phys Chem C,2017,121(38):20947～20954.
[39] Mei J,Leung N L C,Kwok R T K,Lam J W Y,Tang B Z.Chem Rev,2015,115(21):11718～11940.
[40] Yuan Y Y,Zhang C J,Gao M,Zhang R Y,Tang B Z,Liu B.Angew Chem Int Ed,2015,54(6):1780～1786.
[41] Li W Z,Wu X Y,Zhao Z J,Qin A J,Hu R R,Tang B Z.Macromolecules,2015,48(21):7747～7754.
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[43] Miao X P,Liu T,Zhang C,Geng X X,Meng Y,Li X X.Phys Chem Chem Phys,2016,18(6):4295～4299.
[44] Lee W I,Bae Y,Bard A J.J Am Chem Soc,2004,126(27):8358～8359.
[45] Sun M,Hong C Y,Pan C Y.J Am Chem Soc,2012,134(51):20581～20584.
[46] Zhou Q,Cao B,Zhu C,Xu S,Gong Y,Yuan W Z,Zhang Y.Small,2016,12(47):6586～6592.
[47] Zuo Y J,Wang D X,Zhang J,Feng S Y.RSC Adv,2014,4(108):62827～62834.
[48] Niu S,Yan H X,Li S,Xu P L,Zhi X L,Li T T.Macromol Chem Phys,2016,217(10):1185～1190.
[49] Davletbaeva I M,Nurgaliyeva G R,Akhmetshina A I,Davletbaev R S,Atlaskin A A,Sazanova T S,Efimov S V,Klochkov V V,Vorotyntsev I V.RSC Adv,2016,6(112):111109～111119.
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[51] Wang D J,Imae T.J Am Chem Soc,2004,126(41):13204～13205.
[52] Chen J,Guo J,Chang B S,Yang W L.Colloid Polym Sci,2012,290(6):517～524.
[53] Li W Y,Qu J L,Du J W,Ren K F,Wang Y X,Sun J Z,Hu Q L.Chem Commun,2014,50(67):9584～9587.
[54] Lu H,Zhang J,Feng S.Phys Chem Chem Phys,2015,17(40):26783～26789.
[55] Yao R Q,Fu C P,Mao Y,Zhang S F,Feng Z D,Chen L F,Zhang Y.Synth Met,2015,207:79～86.