难处理含铜废水处理技术研究
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摘要
综述了化学沉淀法、氧化还原法、吸附法、膜分离法在难处理含铜废水处理技术研究,结合各个技术特点,说明各个方法的优缺点,尤其强调了处理含络合铜废水各个技术的适用情况,并对含铜废水处理技术进行了展望,以期对含铜废水特别是络合铜废水的处理得到一定的借鉴。
This paper reviews study on treatment technologies of stubborn copper containing wastewater of the chemical precipitation,oxidation reduction method,adsorption,membrane separation,accroding various copper ion/complex treatment technologies and evaluate their application conditions and limitations.The application prospect and development of copper wastewater treatment technologies are also discussed in order to containing copper wastewater especially complexing copper wastewater treatment as a reference.
This paper reviews study on treatment technologies of stubborn copper containing wastewater of the chemical precipitation,oxidation reduction method,adsorption,membrane separation,accroding various copper ion/complex treatment technologies and evaluate their application conditions and limitations.The application prospect and development of copper wastewater treatment technologies are also discussed in order to containing copper wastewater especially complexing copper wastewater treatment as a reference.
引文
[1]马小隆,刘晓东,周广柱.电镀废水处理存在的问题及解决方案[J].山东科技大学学报:自然科学版,2005,24(1):107-111.
[2]蔡静.改性木屑的制备及其铜离子的吸附研究[D].北京:北京化工大学,2016.
[3]加福.化学镀技术1000问[M].北京:机械工业出版社,2015:452.
[4]葛丽颖,刘定富,曾祥钦,等.酸性含铜电镀废水处理[J].电镀与环保,2007,27(2):36-37.
[5]柴立元,尤翔宇,舒余德,等.印刷电路板含铜配离子复杂废水脱铜研究[J].中南大学学报:自然科学版,2010,41(1):27-33.
[6]张新,张进锋.污水处理机械设备的环保状况研究[J].中国科技纵横,2012(19):50-51.
[7]王绍楠,袁东,黄新薇,等.硫化钡对含铜镍电镀废水的处理研究[J].广东化工,2012,39(11):142-143.
[8]钟烘军.线路板废水处理工艺研究[C].中国环境科学学会学术年会论文集.北京:中国环境出版社,2012:1795-1797.
[9]刘文伟.浅探印制线路板生产中含Cu废水的处理技术[J].海峡科学,2010(6):83-84.
[10]黄万抚,王淑君.硫化沉淀法处理矿山酸性废水研究[J].环境工程学报,2004,5(8):60-62.
[11]陈明,倪文,黄万抚.反渗透处理金铜矿山酸性废水[J].膜科学与技术,2008,28(3):95-99.
[12]李福勤,赵慧,任志宏,等.络合-超滤技术深度处理矿山重金属废水[J].工业用水与废水,2013,44(5):14-17.
[13]甄豪波.重金属捕集剂研究进展[J].广东化工,2013,40(16):84,75.
[14] Fu H,Lv X S,Yang Y P,et al. Removal of micro complex copper in aqueous solution with a dithiocarbamate compound[J]. Desalination and Water Treatment,2012,39:103-111.
[15]常鹏利,王亚娥,方晓航.重金属废水处理的研究[J].绿色科技,2012,24(10):169-171.
[16]叶兴刚,祁恩成. TMT-15在PCB络合铜废水处理中的应用研究[J].湖北工业职业技术学院学报,2015,28(4):104-106.
[17] Wang Junjie,Wang Fenghe,Lei Wu,et al. Treatment of wastewater containing Cu~(2+)and Hg~(2+)with new heavy metal capturing agent NBMIPA[J]. Chinese Journal of Environmental Engineering,2012,6(11):3933-3936.
[18]汤兵.铁氧体法在重金属污染物解毒处理中的应用[J].环境导报,2001(2):26-29.
[19]段睿,王立和,杨翠英,等.常温中和铁氧体法处理高浓度含铜废水的研究[J].工业水处理,2013,33(5):53-56.
[20]余雅旋,宁寻安,李仕文,等.硫酸亚铁法与硫化钠法处理络合铜废水的对比研究[J].四川环境,2009,28(4):23-27.
[21]杨文清,关念云.线路板生产络合铜废水的处理研究[J].工业用水与废水,2017,48(2):51-53.
[22]黄思聪.铁碳微电解-重金属捕集-沉淀-BOC吸附工艺处理PCB废水的工艺应用[D].广州:华南理工大学,2012.
[23]陈润华,柴立元,王云燕,等.含Cu-EDTA络合配离子废水的铁碳微电解[J].中国有色金属学报,2012(4):983-990.
[24]张彦,徐祺辉,孙尧,等. Fenton-铁氧体法处理含铜模拟废水的研究[J].电镀与环保,2017,37(3):51-55.
[25]杨凯,黄庆,刘政,等.四川省汽车行业有机废气治理现状及展望[J].绿色科技,2014(8):237-240.
[26]吴小华,徐龙君,刘科,等.煤基活性炭制备工艺对吸附铜离子性能的影响[J].煤炭转化,2013,36(3):76-79.
[27] Ismaiel Ahmed Abu,Aroua Mohamed Kheireddine,Yusoff,et al. Palm shell activated carbon impregnated with task-specific ionic-liquids as a novel adsorbent for the removal of mercury from contaminated water[J]. Chemical Engineering Journal,2013,225:306-314.
[28]刘海.湿地植物及活性炭制备和改性及其对重金属离子的吸附机理研究[D].济南:山东大学,2017.
[29] Chen J Paul,Chong Kai-Hau. Surface modification of a granular activated carbon by citric acid for enhancement of copper adsorption[J]. Carbon,2003,41(10):1979-1986.
[30]林本兰,吴兰兰,崔升,等.新型重金属离子吸附剂的研究进展[J].材料导报,2015,29(10):18-23.
[31] Eren E,Afsin B. An investigation of Cu(II)adsorption by raw and acid-activated bentonite:A combined potentiometric,thermodynamic,XRD,IR,DTA study[J]. Journal of Hazardous Materials,2008,151(2/3):682-691.
[32] Syafalnir A,Nair P U. New approach of heavymetal(chromium,iron,copper and nickel)removal using surfactantmodified zeolite for tin mining wastewater[J]. World Applied Sciences Journal,2013,27(5):614-620.
[33] Belviso C,Cavalcante F,Ragone P,et al. Immobilization of Zn and Pb in polluted soil by in situ crystallization zeolites from fly ash[J]. Water Air Soil Poll,2012,223(8):5357-5364.
[34] Gorgievski Milan,Bo6ic Dragana,Stankovic',et al. Kinetics,equilibrium and mechanism of Cu2+,Ni2+and Zn2+ions biosorption using wheat straw[J]. Ecological Engineering,2013,58:113-122.
[35] Peng Shuai,Meng Hecheng,Ouyang,et al. Nanoporous magnetic cellulose-chitosan composite microspheres:preparation,characterization,and application for Cu(II)adsorption[J].Industrial and Engineering Chemistry Research,2014,53(6):2106-2113.
[36] Akar Tamer,Tunali Sibel1. Biosorption characteristics of Aspergillus flavus biomass for removal of Pb(II)and Cu(II)ions from an aqueous solution[J]. Bioresource Technology,2006,97(15):1780-1787.
[37]黄万抚,刘玉娇,李新冬,等.膜分离技术用于废水中金属的分离和回收[J].工业水处理,2016,36(7):5-10.
[38]王湛,周翀.膜分离技术基础[M].北京:化学工业出版社,2006:31-36.
[39]蒋树贤.络合铜废水深度处理新方法的研究[D].广州:中山大学,2009.
[40] Cséfalvay Edit,Pauer Viktor,Mizsey,et al. Recovery of copper from process waters by nanofiltration and reverse osmosis[J]. Desalination,2009,240(1/2/3):132-142.
[41] Tortora F,Innocenzi V,Prisciandaro M. Heavy metal removal from liquid wastes by using micellar-enhanced ultrafiltration[J]. Water Air Soil Pollut,2016,240:227-240.
[42] Rabindra Bade,Seung Hwan Lee. Micellar enhanced ultrafiltration and activated carbon fibre hybrid processes for copper removal from wastewater[J]. Korean Journal of Chemical Engineering,2007,24(2):239-245.
[43] Xiarchos Ioannis,Jaworska Agnieszka,ZakrzewskaTrznadel,et al. Response surface methodology for the modelling of copper removal from aqueous solutions using micellar-enhanced ultrafiltration[J]. Journal of Membrane Science,2008,321(2):222-231.
[44] Schwarze Michael,Chiappisi Leonardo,Prévost,et al. Oleylethoxycarboxylate——An efficient surfactant for copper extraction and surfactant recycling via micellar enhanced ultrafiltration[J]. Journal of Colloid and Interface Science,2014,421:184-190.
[2]蔡静.改性木屑的制备及其铜离子的吸附研究[D].北京:北京化工大学,2016.
[3]加福.化学镀技术1000问[M].北京:机械工业出版社,2015:452.
[4]葛丽颖,刘定富,曾祥钦,等.酸性含铜电镀废水处理[J].电镀与环保,2007,27(2):36-37.
[5]柴立元,尤翔宇,舒余德,等.印刷电路板含铜配离子复杂废水脱铜研究[J].中南大学学报:自然科学版,2010,41(1):27-33.
[6]张新,张进锋.污水处理机械设备的环保状况研究[J].中国科技纵横,2012(19):50-51.
[7]王绍楠,袁东,黄新薇,等.硫化钡对含铜镍电镀废水的处理研究[J].广东化工,2012,39(11):142-143.
[8]钟烘军.线路板废水处理工艺研究[C].中国环境科学学会学术年会论文集.北京:中国环境出版社,2012:1795-1797.
[9]刘文伟.浅探印制线路板生产中含Cu废水的处理技术[J].海峡科学,2010(6):83-84.
[10]黄万抚,王淑君.硫化沉淀法处理矿山酸性废水研究[J].环境工程学报,2004,5(8):60-62.
[11]陈明,倪文,黄万抚.反渗透处理金铜矿山酸性废水[J].膜科学与技术,2008,28(3):95-99.
[12]李福勤,赵慧,任志宏,等.络合-超滤技术深度处理矿山重金属废水[J].工业用水与废水,2013,44(5):14-17.
[13]甄豪波.重金属捕集剂研究进展[J].广东化工,2013,40(16):84,75.
[14] Fu H,Lv X S,Yang Y P,et al. Removal of micro complex copper in aqueous solution with a dithiocarbamate compound[J]. Desalination and Water Treatment,2012,39:103-111.
[15]常鹏利,王亚娥,方晓航.重金属废水处理的研究[J].绿色科技,2012,24(10):169-171.
[16]叶兴刚,祁恩成. TMT-15在PCB络合铜废水处理中的应用研究[J].湖北工业职业技术学院学报,2015,28(4):104-106.
[17] Wang Junjie,Wang Fenghe,Lei Wu,et al. Treatment of wastewater containing Cu~(2+)and Hg~(2+)with new heavy metal capturing agent NBMIPA[J]. Chinese Journal of Environmental Engineering,2012,6(11):3933-3936.
[18]汤兵.铁氧体法在重金属污染物解毒处理中的应用[J].环境导报,2001(2):26-29.
[19]段睿,王立和,杨翠英,等.常温中和铁氧体法处理高浓度含铜废水的研究[J].工业水处理,2013,33(5):53-56.
[20]余雅旋,宁寻安,李仕文,等.硫酸亚铁法与硫化钠法处理络合铜废水的对比研究[J].四川环境,2009,28(4):23-27.
[21]杨文清,关念云.线路板生产络合铜废水的处理研究[J].工业用水与废水,2017,48(2):51-53.
[22]黄思聪.铁碳微电解-重金属捕集-沉淀-BOC吸附工艺处理PCB废水的工艺应用[D].广州:华南理工大学,2012.
[23]陈润华,柴立元,王云燕,等.含Cu-EDTA络合配离子废水的铁碳微电解[J].中国有色金属学报,2012(4):983-990.
[24]张彦,徐祺辉,孙尧,等. Fenton-铁氧体法处理含铜模拟废水的研究[J].电镀与环保,2017,37(3):51-55.
[25]杨凯,黄庆,刘政,等.四川省汽车行业有机废气治理现状及展望[J].绿色科技,2014(8):237-240.
[26]吴小华,徐龙君,刘科,等.煤基活性炭制备工艺对吸附铜离子性能的影响[J].煤炭转化,2013,36(3):76-79.
[27] Ismaiel Ahmed Abu,Aroua Mohamed Kheireddine,Yusoff,et al. Palm shell activated carbon impregnated with task-specific ionic-liquids as a novel adsorbent for the removal of mercury from contaminated water[J]. Chemical Engineering Journal,2013,225:306-314.
[28]刘海.湿地植物及活性炭制备和改性及其对重金属离子的吸附机理研究[D].济南:山东大学,2017.
[29] Chen J Paul,Chong Kai-Hau. Surface modification of a granular activated carbon by citric acid for enhancement of copper adsorption[J]. Carbon,2003,41(10):1979-1986.
[30]林本兰,吴兰兰,崔升,等.新型重金属离子吸附剂的研究进展[J].材料导报,2015,29(10):18-23.
[31] Eren E,Afsin B. An investigation of Cu(II)adsorption by raw and acid-activated bentonite:A combined potentiometric,thermodynamic,XRD,IR,DTA study[J]. Journal of Hazardous Materials,2008,151(2/3):682-691.
[32] Syafalnir A,Nair P U. New approach of heavymetal(chromium,iron,copper and nickel)removal using surfactantmodified zeolite for tin mining wastewater[J]. World Applied Sciences Journal,2013,27(5):614-620.
[33] Belviso C,Cavalcante F,Ragone P,et al. Immobilization of Zn and Pb in polluted soil by in situ crystallization zeolites from fly ash[J]. Water Air Soil Poll,2012,223(8):5357-5364.
[34] Gorgievski Milan,Bo6ic Dragana,Stankovic',et al. Kinetics,equilibrium and mechanism of Cu2+,Ni2+and Zn2+ions biosorption using wheat straw[J]. Ecological Engineering,2013,58:113-122.
[35] Peng Shuai,Meng Hecheng,Ouyang,et al. Nanoporous magnetic cellulose-chitosan composite microspheres:preparation,characterization,and application for Cu(II)adsorption[J].Industrial and Engineering Chemistry Research,2014,53(6):2106-2113.
[36] Akar Tamer,Tunali Sibel1. Biosorption characteristics of Aspergillus flavus biomass for removal of Pb(II)and Cu(II)ions from an aqueous solution[J]. Bioresource Technology,2006,97(15):1780-1787.
[37]黄万抚,刘玉娇,李新冬,等.膜分离技术用于废水中金属的分离和回收[J].工业水处理,2016,36(7):5-10.
[38]王湛,周翀.膜分离技术基础[M].北京:化学工业出版社,2006:31-36.
[39]蒋树贤.络合铜废水深度处理新方法的研究[D].广州:中山大学,2009.
[40] Cséfalvay Edit,Pauer Viktor,Mizsey,et al. Recovery of copper from process waters by nanofiltration and reverse osmosis[J]. Desalination,2009,240(1/2/3):132-142.
[41] Tortora F,Innocenzi V,Prisciandaro M. Heavy metal removal from liquid wastes by using micellar-enhanced ultrafiltration[J]. Water Air Soil Pollut,2016,240:227-240.
[42] Rabindra Bade,Seung Hwan Lee. Micellar enhanced ultrafiltration and activated carbon fibre hybrid processes for copper removal from wastewater[J]. Korean Journal of Chemical Engineering,2007,24(2):239-245.
[43] Xiarchos Ioannis,Jaworska Agnieszka,ZakrzewskaTrznadel,et al. Response surface methodology for the modelling of copper removal from aqueous solutions using micellar-enhanced ultrafiltration[J]. Journal of Membrane Science,2008,321(2):222-231.
[44] Schwarze Michael,Chiappisi Leonardo,Prévost,et al. Oleylethoxycarboxylate——An efficient surfactant for copper extraction and surfactant recycling via micellar enhanced ultrafiltration[J]. Journal of Colloid and Interface Science,2014,421:184-190.