纳滤膜天然有机物污染及去除PPCPs的研究进展
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摘要
天然有机物(NOM)是造成纳滤膜污染的重要物质之一.从NOM对纳滤膜的污染和去除药物及个人护理品(PPCPs)两方面综述了纳滤膜的污染和截留机理.通过分析得出,微观作用力的解析将是揭示纳滤膜污染机理的关键.同时,纳滤对PPCPs去除效果预测模型的构建将是未来研究工作的重点.
Natural organic matter is one of the important substances for nanofiltration membrane fouling. The fouling and retention mechanism of nanofiltration membranes were reviewed from the aspects of the NOM fouling and the removal of pharmaceuticals and personal care products(PPCPs) by nanofiltration membrane. It was concluded that the analysis of microcosmic force will be the key to reveal the mechanism of nanofiltration membrane fouling. At the same time, the construction of the prediction model for the removal effect of PPCPs by nanofiltration will be the focus of future research work.
Natural organic matter is one of the important substances for nanofiltration membrane fouling. The fouling and retention mechanism of nanofiltration membranes were reviewed from the aspects of the NOM fouling and the removal of pharmaceuticals and personal care products(PPCPs) by nanofiltration membrane. It was concluded that the analysis of microcosmic force will be the key to reveal the mechanism of nanofiltration membrane fouling. At the same time, the construction of the prediction model for the removal effect of PPCPs by nanofiltration will be the focus of future research work.
引文
[1] Shan L,Fan H,Guo H,et al.Natural organic matter fouling behaviors on superwettingnanofiltration membranes[J].Water Res,2016,93:121-132.
[2] 董秉直.饮用水膜法处理新技术[M]//上海:同济大学出版社,2015.
[3] Zhang Y,Zhang N,Zhao P,et al.Characteristics of molecular weight distribution of dissolved organic matter in bromide-containing water and disinfection by-product formation properties during treatment processes[J].J Environ Sci,2018,65(3):179-189.
[4] 丰桂珍,董秉直.DOM纳滤膜污染及对膜截留卡马西平性能的影响[J].环境科学,2013,34(11):4295-4303.
[5] 郭驭,王小亻毛.纳滤膜污染机理、表征及控制[J].给水排水,2017,53(9):120-131.
[6] 李昆,王健行,魏源送.纳滤在水处理与回用中的应用现状与展望[J].环境科学学报,2016,36(8):2714-2729.
[7] Mohammad A W,Teow Y H,Ang W L,et al.Nanofiltration membranes review:Recent advances and future prospects[J].Desalination,2015,356:226-254.
[8] Park M,Anumol T,Simon J,et al.Pre-ozonation for high recovery of nanofiltration (NF) membrane system:Membrane fouling reduction and trace organic compound attenuation[J].J Membr Sci,2017,523:255-263.
[9] Yu W,Liu T,Crawshaw J,et al.Ultrafiltration and nanofiltration membrane fouling by natural organic matter:Mechanisms and mitigation by pre-ozonation and pH[J].Water Res,2018,139:353-362.
[10] Mahlangu T O,Thwala J M,Mamba B B,et al.Factors governing combined fouling by organic and colloidal foulants in cross-flow nanofiltration[J].J Membr Sci,2015,491:53-62.
[11] 寇朝卫,张干伟,沈舒苏,等.基于XDLVO理论解析膜法水处理过程中膜污染问题的研究[J].膜科学与技术,2017,37(1):8-15.
[12] Heffernan R,Habimana O,Semi?o A J C,et al.A physical impact of organic fouling layers on bacterial adhesion during nanofiltration[J].Water Res,2014,67(12):118-128.
[13] Feng G Z,Chu H Q,Dong B Z.Characterizing dissolved organic matter fouling of nanofiltration membranes and evaluating effects of naproxen retention[J].Desalin Water Treat,2015,56(11):2835-2847.
[14] Sari M A,Chellam S.Relative contributions of organic and inorganic fouling during nanofiltration of inland brackish surface water[J].J Membr Sci,2017,523:68-76.
[15] Lin Y L,Lee C H.Elucidating the rejection mechanisms of PPCPs by nanofiltration and reverse osmosis membranes[J].Ind Eng Chem Res,2014,53(16):6798-6806.
[16] Lin Y L.Effects of organic,biological and colloidal fouling on the removal of pharmaceuticals and personal care products by nanofiltration and reverse osmosis membranes[J].J Membr Sci,2017,542:342-351.
[17] Acero J L,Benítez F J,Real F J,et al.Influence of membrane,pH and water matrix properties on the retention of emerging contaminants by ultrafiltration and nanofiltration[J].Desalin Water Treat,2016,57(25):11685-11698.
[18] Koyuncu I,Topacik D,Wiesner M R.Factors influencing flux decline during nanofiltration of solutions containing dyes and salts[J].Water Res,2004,38(2):432-440.
[19] Wang J,Wang L,Miao R,et al.Enhanced gypsum scaling by organic fouling layer on nanofiltration membrane:Characteristics and mechanisms[J].Water Res,2016,91:203-213.
[20] Mo Y,Tiraferri A,Yip N Y,et al.Improved antifouling properties of polyamide nanofiltration membranes by reducing the density of surface carboxyl groups[J].Environ Sci Technol,2012,46(24):13253-13261.
[21] Wang T H,Yen Y J,Hsieh Y K,et al.Size effect of calcium-humic acid non-rigid complexes on the fouling behaviors in nanofiltration:An LA-ICP-MS study[J].Colloids Surf A Physicochem Eng Aspects,2017,513:335-347.
[22] Zhao C W,Zhang J,He G Z,et al.Perfluorooctane sulfonate removal by nanofiltration membrane the role of calcium ions[J].Chem Eng J,2013,233:224-232.
[23] Zhao C W,Tang C Y,Li P ,et al.Perfluorooctane sulfonate removal by nanofiltration membrane - The effect and interaction of magnesium ion/humic acid[J].J Membr Sci,2016,503:31-41.
[24] Braeken L ,Boussu K ,Bruggen B V D ,et al.Modeling of the adsorption of organic compounds on polymeric nanofiltration membranes in solutions containing two compounds[J].Chemphyschem,2005,6(8):1606-1612.
[25] Hermia J.Constant pressure blocking filtration law application to powder-law non-Newtonian fluid[J].Trans Inst Chem Eng,1982,60 (3) :183-187.
[26] Chang E E,Chang Y C,Liang C H,et al.Identifying the rejection mechanism for nanofiltration membranes fouled by humic acid and calcium ions exemplified by acetaminophen,sulfamethoxazole,and triclosan[J].J Hazard Mater,2012,221/222(4):19-27.
[27] Vogel D,Simon A,Alturki A A,et al.Effects of fouling and scaling on the retention of trace organic contaminants by a nanofiltration membrane:The role of cake-enhanced concentration polarisation[J].Sep Purif Technol,2010,73(2):256-263.
[28] Schippers J C,Verdouw J.The modified fouling index,a method of determining the fouling characteristics of water[J].Desalination,1980,32(1/3):137-148.
[29] Nghiem L D N,Coleman P J,Espendiller C.Mechanisms underlying the effects of membrane fouling on the nanofiltration of trace organic contaminants[J].Desalination,2010,250(2):682-687.
[30] 魏源送,王健行,岳增刚,等.纳滤膜技术在废水深度处理中的膜污染及控制研究进展[J].环境科学学报,2017,37(1):1-10.
[31] Picioreanu C,Vrouwenvelder J S,Loosdrecht M C M.Three-dimensional modeling of biofouling and fluid dynamics in feed spacer channels of membrane devices[J].J Membr Sci,2009,345(1):340-354.
[32] Shetty G R ,Chellam S.Predicting membrane fouling during municipal drinking water nanofiltration using artificial neural networks[J].J Membr Sci,2003,217(1):69-86.
[33] Yu W,Campos L C,Graham N.Application of pulsed UV-irradiation and pre-coagulation to control ultrafiltration membrane fouling in the treatment of micro-polluted surface water[J].Water Res,2016,107:83-92.
[34] Miao R,Wang L,Zhu M,et al.Effect of hydration forces on protein fouling of ultrafiltration membranes:The role of protein charge,hydrated ion species,and membrane hydrophilicity[J].Environ Sci Technol,2016,51(1):167-174.
[35] Wang Y N,Tang C Y.Nanofiltration membrane fouling by oppositely charged macromolecules:Investigation on flux behavior,foulant mass deposition,and solute rejection[J].Environ Sci Technol,2011,45(20):8941-8947.
[36] Zazouli M A,Nasseri S,Ulbricht M.Fouling effects of humic and alginic acids in nanofiltration and influence of solution composition[J].Desalination,2010,250(2):688-692.
[37] Lamsal R,Montreuil K R,Kent F C,et al.Characterization and removal of natural organic matter by an integrated membrane system[J].Desalination,2012,303(10):12-16.
[38] Mustafa G,Wyns K,Buekenhoudt A,et al.New insights into the fouling mechanism of dissolved organic matter applying nanofiltration membranes with a variety of surface chemistries[J].Water Res,2016,93:195-204.
[39] Feng G Z,Chu H Q,Dong B Z.Fouling effects of algogenic organic matters during nanofiltration of naproxen[J].Desalination,2014,350:69-78.
[40] Nilson J A,Digiano F A.Influence of NOM composition on nanofiltration[J].J Awwa,1996,88(5):53-66.
[41] Amy G,Cho J.Interactions between natural organic matter (NOM) and membranes:Rejection and fouling[J].Water Sci Technol,2015,40(9):131-139.
[42] Salgado C,Palacio L,Carmona F J,et al.Influence of low and high molecular weight compounds on the permeate flux decline in nanofiltration of red grape must[J].Desalination,2013,315(9):124-134.
[43] 丰桂珍,董秉直.藻类有机物对纳滤膜去除萘普生效果影响研究[J].中国环境科学,2013,33(3):423-429.
[44] Roudman A R,Digiano F A.Surface energy of experimental and commercial nanofiltration membranes:Effects of wetting and natural organic matter fouling[J].J Membr Sci,2000,175(1):61-73.
[45] Contreras A E,Kim A,Li Q.Combined fouling of nanofiltration membranes:Mechanisms and effect of organic matter[J].J Membr Sci,2009,327(1):87-95.
[46] Liikanen R,Ylikuivila J,Laukkanen R.Efficiency of various chemical cleanings for nanofiltration membrane fouled by conventionally-treated surface water[J].J Membr Sci,2002,195(2):265-276.
[47] Simon A,Mcdonald J A,Khan S J,et al.Effects of caustic cleaning on pore size of nanofiltration membranes and their rejection of trace organic chemicals[J].J Membr Sci,2013,447:153-162.
[48] Al-Amoudi A,Williams P,Mandale S,et al.Cleaning results of new and fouled nanofiltration membrane characterized by Zeta potential and permeability[J].Sep Purif Technol,2007,54(2):234-240.
[49] Yoon Y,Westerhoff P,Snyder S A,et al.Removal of endocrine disrupting compounds and pharmaceuticals by nanofiltration and ultrafiltration membranes[J].Desalination,2007,202(1):16-23.
[50] 黄丹,郑甜甜,刘蕊,等.纳滤去除水中布洛芬的研究[J].膜科学与技术,2014,34(2):72-76.
[51] Bruggen B V D,Schaep J,Wilms D,et al.Influence of molecular size,polarity and charge on the retention of organic molecules by nanofiltration[J].J Membr Sci,1999,156(1):29-41.
[52] Ogutverici A,Yilmaz L,Yetis U,et al.Triclosan removal by NF from a real drinking water source - Effect of natural organic matter[J].Chem Eng J,2016,283:330-337.
[2] 董秉直.饮用水膜法处理新技术[M]//上海:同济大学出版社,2015.
[3] Zhang Y,Zhang N,Zhao P,et al.Characteristics of molecular weight distribution of dissolved organic matter in bromide-containing water and disinfection by-product formation properties during treatment processes[J].J Environ Sci,2018,65(3):179-189.
[4] 丰桂珍,董秉直.DOM纳滤膜污染及对膜截留卡马西平性能的影响[J].环境科学,2013,34(11):4295-4303.
[5] 郭驭,王小亻毛.纳滤膜污染机理、表征及控制[J].给水排水,2017,53(9):120-131.
[6] 李昆,王健行,魏源送.纳滤在水处理与回用中的应用现状与展望[J].环境科学学报,2016,36(8):2714-2729.
[7] Mohammad A W,Teow Y H,Ang W L,et al.Nanofiltration membranes review:Recent advances and future prospects[J].Desalination,2015,356:226-254.
[8] Park M,Anumol T,Simon J,et al.Pre-ozonation for high recovery of nanofiltration (NF) membrane system:Membrane fouling reduction and trace organic compound attenuation[J].J Membr Sci,2017,523:255-263.
[9] Yu W,Liu T,Crawshaw J,et al.Ultrafiltration and nanofiltration membrane fouling by natural organic matter:Mechanisms and mitigation by pre-ozonation and pH[J].Water Res,2018,139:353-362.
[10] Mahlangu T O,Thwala J M,Mamba B B,et al.Factors governing combined fouling by organic and colloidal foulants in cross-flow nanofiltration[J].J Membr Sci,2015,491:53-62.
[11] 寇朝卫,张干伟,沈舒苏,等.基于XDLVO理论解析膜法水处理过程中膜污染问题的研究[J].膜科学与技术,2017,37(1):8-15.
[12] Heffernan R,Habimana O,Semi?o A J C,et al.A physical impact of organic fouling layers on bacterial adhesion during nanofiltration[J].Water Res,2014,67(12):118-128.
[13] Feng G Z,Chu H Q,Dong B Z.Characterizing dissolved organic matter fouling of nanofiltration membranes and evaluating effects of naproxen retention[J].Desalin Water Treat,2015,56(11):2835-2847.
[14] Sari M A,Chellam S.Relative contributions of organic and inorganic fouling during nanofiltration of inland brackish surface water[J].J Membr Sci,2017,523:68-76.
[15] Lin Y L,Lee C H.Elucidating the rejection mechanisms of PPCPs by nanofiltration and reverse osmosis membranes[J].Ind Eng Chem Res,2014,53(16):6798-6806.
[16] Lin Y L.Effects of organic,biological and colloidal fouling on the removal of pharmaceuticals and personal care products by nanofiltration and reverse osmosis membranes[J].J Membr Sci,2017,542:342-351.
[17] Acero J L,Benítez F J,Real F J,et al.Influence of membrane,pH and water matrix properties on the retention of emerging contaminants by ultrafiltration and nanofiltration[J].Desalin Water Treat,2016,57(25):11685-11698.
[18] Koyuncu I,Topacik D,Wiesner M R.Factors influencing flux decline during nanofiltration of solutions containing dyes and salts[J].Water Res,2004,38(2):432-440.
[19] Wang J,Wang L,Miao R,et al.Enhanced gypsum scaling by organic fouling layer on nanofiltration membrane:Characteristics and mechanisms[J].Water Res,2016,91:203-213.
[20] Mo Y,Tiraferri A,Yip N Y,et al.Improved antifouling properties of polyamide nanofiltration membranes by reducing the density of surface carboxyl groups[J].Environ Sci Technol,2012,46(24):13253-13261.
[21] Wang T H,Yen Y J,Hsieh Y K,et al.Size effect of calcium-humic acid non-rigid complexes on the fouling behaviors in nanofiltration:An LA-ICP-MS study[J].Colloids Surf A Physicochem Eng Aspects,2017,513:335-347.
[22] Zhao C W,Zhang J,He G Z,et al.Perfluorooctane sulfonate removal by nanofiltration membrane the role of calcium ions[J].Chem Eng J,2013,233:224-232.
[23] Zhao C W,Tang C Y,Li P ,et al.Perfluorooctane sulfonate removal by nanofiltration membrane - The effect and interaction of magnesium ion/humic acid[J].J Membr Sci,2016,503:31-41.
[24] Braeken L ,Boussu K ,Bruggen B V D ,et al.Modeling of the adsorption of organic compounds on polymeric nanofiltration membranes in solutions containing two compounds[J].Chemphyschem,2005,6(8):1606-1612.
[25] Hermia J.Constant pressure blocking filtration law application to powder-law non-Newtonian fluid[J].Trans Inst Chem Eng,1982,60 (3) :183-187.
[26] Chang E E,Chang Y C,Liang C H,et al.Identifying the rejection mechanism for nanofiltration membranes fouled by humic acid and calcium ions exemplified by acetaminophen,sulfamethoxazole,and triclosan[J].J Hazard Mater,2012,221/222(4):19-27.
[27] Vogel D,Simon A,Alturki A A,et al.Effects of fouling and scaling on the retention of trace organic contaminants by a nanofiltration membrane:The role of cake-enhanced concentration polarisation[J].Sep Purif Technol,2010,73(2):256-263.
[28] Schippers J C,Verdouw J.The modified fouling index,a method of determining the fouling characteristics of water[J].Desalination,1980,32(1/3):137-148.
[29] Nghiem L D N,Coleman P J,Espendiller C.Mechanisms underlying the effects of membrane fouling on the nanofiltration of trace organic contaminants[J].Desalination,2010,250(2):682-687.
[30] 魏源送,王健行,岳增刚,等.纳滤膜技术在废水深度处理中的膜污染及控制研究进展[J].环境科学学报,2017,37(1):1-10.
[31] Picioreanu C,Vrouwenvelder J S,Loosdrecht M C M.Three-dimensional modeling of biofouling and fluid dynamics in feed spacer channels of membrane devices[J].J Membr Sci,2009,345(1):340-354.
[32] Shetty G R ,Chellam S.Predicting membrane fouling during municipal drinking water nanofiltration using artificial neural networks[J].J Membr Sci,2003,217(1):69-86.
[33] Yu W,Campos L C,Graham N.Application of pulsed UV-irradiation and pre-coagulation to control ultrafiltration membrane fouling in the treatment of micro-polluted surface water[J].Water Res,2016,107:83-92.
[34] Miao R,Wang L,Zhu M,et al.Effect of hydration forces on protein fouling of ultrafiltration membranes:The role of protein charge,hydrated ion species,and membrane hydrophilicity[J].Environ Sci Technol,2016,51(1):167-174.
[35] Wang Y N,Tang C Y.Nanofiltration membrane fouling by oppositely charged macromolecules:Investigation on flux behavior,foulant mass deposition,and solute rejection[J].Environ Sci Technol,2011,45(20):8941-8947.
[36] Zazouli M A,Nasseri S,Ulbricht M.Fouling effects of humic and alginic acids in nanofiltration and influence of solution composition[J].Desalination,2010,250(2):688-692.
[37] Lamsal R,Montreuil K R,Kent F C,et al.Characterization and removal of natural organic matter by an integrated membrane system[J].Desalination,2012,303(10):12-16.
[38] Mustafa G,Wyns K,Buekenhoudt A,et al.New insights into the fouling mechanism of dissolved organic matter applying nanofiltration membranes with a variety of surface chemistries[J].Water Res,2016,93:195-204.
[39] Feng G Z,Chu H Q,Dong B Z.Fouling effects of algogenic organic matters during nanofiltration of naproxen[J].Desalination,2014,350:69-78.
[40] Nilson J A,Digiano F A.Influence of NOM composition on nanofiltration[J].J Awwa,1996,88(5):53-66.
[41] Amy G,Cho J.Interactions between natural organic matter (NOM) and membranes:Rejection and fouling[J].Water Sci Technol,2015,40(9):131-139.
[42] Salgado C,Palacio L,Carmona F J,et al.Influence of low and high molecular weight compounds on the permeate flux decline in nanofiltration of red grape must[J].Desalination,2013,315(9):124-134.
[43] 丰桂珍,董秉直.藻类有机物对纳滤膜去除萘普生效果影响研究[J].中国环境科学,2013,33(3):423-429.
[44] Roudman A R,Digiano F A.Surface energy of experimental and commercial nanofiltration membranes:Effects of wetting and natural organic matter fouling[J].J Membr Sci,2000,175(1):61-73.
[45] Contreras A E,Kim A,Li Q.Combined fouling of nanofiltration membranes:Mechanisms and effect of organic matter[J].J Membr Sci,2009,327(1):87-95.
[46] Liikanen R,Ylikuivila J,Laukkanen R.Efficiency of various chemical cleanings for nanofiltration membrane fouled by conventionally-treated surface water[J].J Membr Sci,2002,195(2):265-276.
[47] Simon A,Mcdonald J A,Khan S J,et al.Effects of caustic cleaning on pore size of nanofiltration membranes and their rejection of trace organic chemicals[J].J Membr Sci,2013,447:153-162.
[48] Al-Amoudi A,Williams P,Mandale S,et al.Cleaning results of new and fouled nanofiltration membrane characterized by Zeta potential and permeability[J].Sep Purif Technol,2007,54(2):234-240.
[49] Yoon Y,Westerhoff P,Snyder S A,et al.Removal of endocrine disrupting compounds and pharmaceuticals by nanofiltration and ultrafiltration membranes[J].Desalination,2007,202(1):16-23.
[50] 黄丹,郑甜甜,刘蕊,等.纳滤去除水中布洛芬的研究[J].膜科学与技术,2014,34(2):72-76.
[51] Bruggen B V D,Schaep J,Wilms D,et al.Influence of molecular size,polarity and charge on the retention of organic molecules by nanofiltration[J].J Membr Sci,1999,156(1):29-41.
[52] Ogutverici A,Yilmaz L,Yetis U,et al.Triclosan removal by NF from a real drinking water source - Effect of natural organic matter[J].Chem Eng J,2016,283:330-337.