中国古代制釉技术的锶同位素比值方法初探
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摘要
为了揭示制釉原料种类以及不同加入比例对中国古代釉料锶同位素比值的影响规律,以浙江杭州老虎洞窑、河南汝窑以及江西景德镇的制釉原料为研究对象,采用科学分析与工艺模拟实验相结合的研究方法,科学揭示了制釉原料种类以及不同加入比例对釉料锶同位素比值影响规律。结果初步表明只有充分掌握各地瓷石或者长石类原料及配比关系对锶同位素比值的影响规律,才能对古代不同窑口的制釉技术进行科学的对比研究。
In order to reveal the influence of raw material and formulation on Sr isotope ratio of ancient glaze, the raw materials of making glaze from Laohudong kiln site in Hangzhou city, Ru kiln site in Baofeng city and Jingdezhen in Jiangxi province. were analyzed by EDXRF and Strontium isotope analysis.The results show that it is difficult to accurately distinguish whether wood ash or limestone was the source of calcium in glaze according to the Sr isotope ratio data alone. The strontium isotope ratio data of ancient Chinese glaze are comprehensive information of calcareous raw materials and porcelain stone or feldspar raw materials together. The preliminary results of this work indicate that Strontium isotope analysis method is need further studied before applying it to research the Chinese glaze.
In order to reveal the influence of raw material and formulation on Sr isotope ratio of ancient glaze, the raw materials of making glaze from Laohudong kiln site in Hangzhou city, Ru kiln site in Baofeng city and Jingdezhen in Jiangxi province. were analyzed by EDXRF and Strontium isotope analysis.The results show that it is difficult to accurately distinguish whether wood ash or limestone was the source of calcium in glaze according to the Sr isotope ratio data alone. The strontium isotope ratio data of ancient Chinese glaze are comprehensive information of calcareous raw materials and porcelain stone or feldspar raw materials together. The preliminary results of this work indicate that Strontium isotope analysis method is need further studied before applying it to research the Chinese glaze.
引文
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[9]吴隽,何旗航,张茂林,等.唐、五代景德镇蓝田窑青瓷科技研究[J].文物保护与考古科学,2015,27(02):1-5.
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[2]Freestone,I.C.,Leslie,K.A.,Thirlwall,M.and Gorin-Rosen,Y.,Strontium isotopes in the investigation of early glass production:Byzantine and early Islamic glass from the Near East[J]Archaeometry,2003,45,19 32.
[3]Hongjiao Ma,Julian Henderson,Jane Evans.The exploration of Sr isotopic analysis applied to Chinese glazes:part one[J].Journal of Archaeological Science.2014,50(10):551 558.
[4]Ma,H.,Wood,N.,Doherty,C.,et al.New Insights into the Calcium Flux Used in Ancient Longquan and Yue Kilns Based on Strontium IsotopicCompositions[J].Archaeometry,2018 https://doi.org/10.1111/arcm.12420.
[5]熊寥.中国陶瓷古籍集成[M].上海:上海文化出版社,2006.
[6]徐嫦松,李伟东,张文江,等.吉州窑黑釉瓷胎釉原料分析与配方探讨[J].硅酸盐学报,2018,46(06):846-853.
[7]李国桢,郭演仪.中国名瓷工艺基础[M].上海:上海科学技术出版社,1985.
[8]吴军明,罗婷,熊春华,等.釉灰制备原料和工艺对其组成的影响[J].光谱学与光谱分析,2016,36(11):3709-3713.
[9]吴隽,何旗航,张茂林,等.唐、五代景德镇蓝田窑青瓷科技研究[J].文物保护与考古科学,2015,27(02):1-5.
[10]李合,史宁昌,王光尧,等.上林湖后司岙窑址秘色瓷的成分特征研究[J].故宫博物院院刊,2017(06):124-132+1 60.